422 results on '"Dehui Li"'
Search Results
52. Strongly Anisotropic Quasi‐1D BaTiS 3 Chalcogenide Perovskite for Near‐Infrared Polarized Photodetection
- Author
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Feifan Yang, Kanghua Li, Mingzhi Fan, Wendian Yao, Liuchong Fu, Changying Xiong, Shenglin Jiang, Dehui Li, Ming Xu, Chao Chen, Guangzu Zhang, and Jiang Tang
- Subjects
Atomic and Molecular Physics, and Optics ,Electronic, Optical and Magnetic Materials - Published
- 2022
53. The effect of geographic distance on independent directors’ performance from the perspective of inefficient investment
- Author
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Duo Shang, Dongliang Yuan, Dehui Li, and Libo Fan
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Economics and Econometrics - Published
- 2022
54. Phytolith transport and its influence factor in different soil types in northern temperate region
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Lidan Liu, Nannan Li, Guizai Gao, Hongyan Liu, Dehui Li, and Dongmei Jie
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010506 paleontology ,Soil classification ,Context (language use) ,010502 geochemistry & geophysics ,01 natural sciences ,Phytolith ,Soil pH ,Soil water ,Temperate climate ,Environmental science ,Physical geography ,Precipitation ,Chernozem ,0105 earth and related environmental sciences ,Earth-Surface Processes - Abstract
Increasing use is being made of phytoliths for quantitative palaeovegetation and palaeoclimatic reconstruction, and consequently studies of phytolith transport are attracting increasing attention. In this context, we conducted a detailed study of factors affecting the soil phytolith transport in six representative natural soil types in Northeast China. We define a phytolith transport index (T) which indicates that transport rates are the lowest in chernozem and chestnut soils, intermediate in dark brown and albic soils, and obviously higher in black and alluvial soils. Additionally, there are differences in the vertical transport of different phytolith types in the soils; however, the transport characteristics are essentially the same among the different soil types. Transport rates are lowest for tabular and blocky phytoliths, followed by bulliform phytolith. By contrast, the rates for short cell, lanceolate and elongate phytoliths are significantly higher, and, notably, these phytolith types have different size and aspect ratios. The transport of phytoliths is also mainly influenced by mean annual precipitation (MAP), soil pH and soil clay content. Climatic factors, especially MAP, are a more significant factor for phytolith transport than phytolith size and aspect ratio. Overall, our findings are significant for the palaeoenvironmental interpretation of soil phytolith assemblages in topsoils.
- Published
- 2021
55. Nanosized oxide phases in oxide-dispersion-strengthened steel PM2000
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Dehui Li, Jian Lin, Yuan Wang, Yinzhong Shen, Yifeng Chen, Bocong Liu, and Hui Wang
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Fusion ,chemistry.chemical_compound ,Materials science ,chemistry ,Nuclear fission ,fungi ,technology, industry, and agriculture ,Oxide ,Composite material ,Condensed Matter Physics ,Dispersion (chemistry) - Abstract
Oxide-dispersion-strengthened (ODS) steels are promising material candidates for nuclear fission and fusion applications. Nanosized oxide particles in as-rolled ODS steel PM2000 were investigated b...
- Published
- 2021
56. Layer-Number Engineered Momentum-Indirect Interlayer Excitons with Large Spectral Tunability
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Wendian Yao, Dong Yang, Yingying Chen, Junchao Hu, Junze Li, and Dehui Li
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Mechanical Engineering ,General Materials Science ,Bioengineering ,General Chemistry ,Condensed Matter Physics - Abstract
Interlayer excitons (IXs) in type II van der Waals (vdW) heterostructures are equipped with an oriented permanent dipole moment and long lifetime and thus would allow promising applications in excitonic and optoelectronic devices. However, based on the widely studied heterostructures of transition-metal dichalcogenides (TMDs), IX emission is greatly influenced by the lattice mismatch and geometric misalignment between the constituent layers, increasing the complexity of the device fabrication. Here, we report on the robust momentum-indirect IX emission in TMD/two-dimensional (2D) perovskite vdW heterostructures, which were fabricated without considering the orientation arrangement or momentum mismatch. The IXs show a large diffusion coefficient of ∼10 cm
- Published
- 2022
57. Phytolith evidence for changes in the vegetation diversity and cover of a grassland ecosystem in Northeast China since the mid-Holocene
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Guizai Gao, Maolin Wang, Dehui Li, Nannan Li, Jiangyong Wang, Honghao Niu, Meng Meng, Ying Liu, Guihua Zhang, and Dongmei Jie
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Earth-Surface Processes - Published
- 2023
58. Approximate Analytical Solution for Tissue Temperature Distribution in High-Intensity Focused Ultrasound.
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Dehui Li, Guofeng Shen, Jingfeng Bai, and Yazhu Chen
- Published
- 2009
- Full Text
- View/download PDF
59. Acupuncture Combined with Three-Step Analgesic Drug Therapy for Treatment of Cancer Pain: A Systematic Review and Meta-Analysis of Randomised Clinical Trials
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Chunxia Sun, Yifan Su, Huanfang Fan, Na Guo, and Dehui Li
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medicine.medical_specialty ,business.industry ,Nausea ,Analgesic ,Review Article ,Cochrane Library ,030226 pharmacology & pharmacy ,law.invention ,Clinical trial ,Other systems of medicine ,03 medical and health sciences ,0302 clinical medicine ,Complementary and alternative medicine ,Randomized controlled trial ,law ,Meta-analysis ,Internal medicine ,medicine ,Acupuncture ,medicine.symptom ,business ,Cancer pain ,RZ201-999 ,030217 neurology & neurosurgery - Abstract
Objective. The purpose of this study was to systematically evaluate the efficacy and safety of acupuncture combined with the WHO three-step analgesic drug ladder for cancer pain. Methods. The Cochrane Library, PubMed, and CNKI Database of Systematic Reviews were searched. Using the Cochrane Register for Randomized Controlled Trials, the quality of the included literature was evaluated, and the meta-analysis was carried out with RevMan 5.3 software. Results. Compared with three-step analgesia alone, acupuncture combined with three-step analgesia for cancer pain increased pain relief response rates (RR = 1.12, 95% CI: 1.08∼1.17, P < 0.00001 ), reduced NRS score (SMD = −1.10, 95% CI: −1.86∼−0.35, P = 0.004 ), reduced the rate of side effects (RR = 0.45, 95% CI: 0.38∼0.53, P < 0.00001 ), including nausea ( P < 0.00001 ), vomiting ( P = 0.008 ), constipation ( P < 0.00001 ), and dizziness ( P = 0.010 ), reduced the burst pain rate (SMD = −1.38; 95% CI: −2.44∼−0.32, P = 0.01 ), shortened analgesia effect onset time ( P = 0.004 ), and extended the duration of response ( P < 0.0001 ). Conclusion. For the treatment of cancer pain, acupuncture combined with three-step analgesic drugs is better than using only three-step analgesic drugs.
- Published
- 2021
60. [Analysis of prescription and medication rules of traditional Chinese medicine in the treatment of the coronavirus disease 2019 based on traditional Chinese medicine inheritance support platform]
- Author
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Jiao, Liu, Dehui, Li, Jianqiang, Mei, Lei, Wu, Fenqiao, Chen, Yuan, Liu, Xiaomen, Lang, Guodong, Yuan, and Yawei, Zhao
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Adult ,Adolescent ,Infant ,Middle Aged ,COVID-19 Drug Treatment ,Young Adult ,Prescriptions ,Cough ,Child, Preschool ,Humans ,Female ,Medicine, Chinese Traditional ,Child ,Asymptomatic Infections ,Aged ,Drugs, Chinese Herbal - Abstract
To analyze the rules of medication and principles of formulas for the treatment of coronavirus disease 2019 (COVID-19) using the traditional Chinese medicine inheritance support platform (V2.5).The clinical data, including gender, age, clinical symptoms, frequency of traditional Chinese medicine medication and prescription information, of patients with COVID-19 and asymptomatic infection who were admitted to Hebei COVID-19 designated hospital supported by medical team of First Affiliated Hospital of Hebei University of Chinese Medicine from January to March 2021 were collected. The information data were input into the traditional Chinese medicine inheritance support platform (V2.5). The data mining and analysis were realized by the integrated association rules and complex entropy clustering analysis methods of the software, including the analysis of the frequency of each drug use, drug meridian, taste, and prescription rules, and the new prescriptions were developed.A total of 564 patients (564 prescriptions) were enrolled, involving 200 Chinese herbs, including 357 cases of common COVID-19 and 207 cases of asymptomatic infection. The proportion of women with common COVID-19 was high, and the high incidence age group was 51-70 years old. There was no significant difference in gender of asymptomatic infection, and the high incidence age group was 1-20 years old. The main clinical manifestations of most patients were head heavy and cough, followed by low fever and cough with sputum, the main tongue coating and pulse pattern were similar in both types of patients. The frequency of traditional Chinese medicine used in patients with common type of COVID-19 from high to low was liquorice root (326 times), indian bread (264 times), pinellia tuber (263 times), bitter apricot seed (236 times), baical skullcap root (229 times), gypsum (205 times), agastache rugosus (201 times), dried tangerine peel (194 times), ephedra (184 times), and Chinese thorowax root (163 times), while that used by asymptomatic infection were baical skullcap root (174 times), liquorice root (142 times), medicated leaven (137 times), agastache rugosus (127 times), pinellia tuber (114 times), Chinese thorowax root (100 times), officinal magnolia bark (91 times), atractylodes rhizome (89 times), peony root (84 times), and milkvetch root (83 times). The two types of patients were mainly treated with warm, cold and flat drugs, and the nature and taste were mainly pungent, bitter and sweet. The meridian tropism of drugs was mainly lung, spleen and stomach. High frequency drug formulation mainly included drugs for resolving turbidity and detoxification. At the same time, seven new prescriptions for common COVID-19 and four new prescriptions for asymptomatic infection were developed.The primary reason for the COVID-19 occurrence and development is turbidity-toxin and the qi of plague, and resolving turbidity and detoxication are the basic treating principle. On the basis, for patients with common COVID-19, symptomatic treatment such as relieving exterior syndrome, clearing heat, resolving phlegm, and antitussive drugs should be taken into account at the same time, while the treatment of asymptomatic infections should focus more on supporting the body and eliminating the harmful pathogens.
- Published
- 2022
61. Combined Complex Skin Repair in Patient With Extensive Burns: A Case Report
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Dehui Li, Xingxin Gao, Liming Zhang, Yuan Lin, and Min Zhang
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Male ,medicine.medical_specialty ,Body Surface Area ,medicine.medical_treatment ,Transplantation, Autologous ,Epithelium ,030207 dermatology & venereal diseases ,03 medical and health sciences ,0302 clinical medicine ,medicine ,Humans ,In patient ,Skin repair ,Body surface area ,Wound Healing ,integumentary system ,Third-Degree Burn ,business.industry ,Graft Survival ,Rehabilitation ,030208 emergency & critical care medicine ,Skin Transplantation ,Middle Aged ,Surgery ,Transplantation ,Emergency Medicine ,Skin grafting ,Full thickness ,Burns ,business ,Total body surface area - Abstract
Auto-skin grafting is the current treatment of choice for extensive burns. Nevertheless, the lack of donor sites for skin grafting remains one of the greatest limiting factors for the treatment of extensively burned patients. We present the case of a 53-year-old male patient with deep and full thickness burns on 91% of the total body surface area. We used the Meek technique for split-thickness skin graft expansion to treat this patient. In order to obtain sufficient skin for grafting, we repeatedly harvested the same anatomical areas. Acceleration of burn wounds, recipient, and donor site healing was achieved by systemic treatment with recombinant human growth hormone and topical recombinant human epidermal growth factors. This combined, complex treatment modality contributed to the successful skin repair in this patient.
- Published
- 2021
62. Low-Voltage Operated Organic Thin-Film Transistors With Mobility Exceeding 10 cm²/vs
- Author
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Dehui Li, Wei Wang, Meili Xu, Shizhang Li, and Weihao Qi
- Subjects
010302 applied physics ,Materials science ,business.industry ,Gate dielectric ,Dielectric ,01 natural sciences ,Electronic, Optical and Magnetic Materials ,Organic semiconductor ,Hysteresis ,Thin-film transistor ,Logic gate ,0103 physical sciences ,Optoelectronics ,Electrical and Electronic Engineering ,business ,Low voltage ,Voltage - Abstract
In this letter, low-voltage operation and high mobility are simultaneously achieved in the OTFTs based on an elaborately constructed tri-layer gate dielectric. The tri-layer gate dielectric consists of the cross-linked poly(4-vinylphenol) (CL-PVP), polyvinylpyrrolidone (PVPy) and poly(styrene) (PS) films. The ultrathin CL-PVP and PS films prevent the charges transferring and trapping in the PVPy dielectric, which improves the performances. The low trap density at the organic semiconductor/dielectric interface contributes to the low-voltage operation and high mobility in the OTFTs. The OTFTs exhibit promising performances with high mobility exceeding 10 cm2/vs, small subthreshold swing of 185 mV/decade on average, high on/off ratio of $10^{{5}}$ , at low operating voltages below 5 V. The measurements on stability and ageing of the OTFTs indicate that the encapsulation is required for practical application.
- Published
- 2021
63. Genome-wide association studies of body size traits in Tibetan sheep
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Dehui Liu, Xue Li, Lei Wang, Quanbang Pei, Jincai Zhao, De Sun, Qianben Ren, Dehong Tian, Buying Han, Hanjing Jiang, Wenkui Zhang, Song Wang, Fei Tian, Sijia Liu, and Kai Zhao
- Subjects
Tibetan sheep ,Re-sequencing ,GWAS ,Body size traits ,SNP ,Biotechnology ,TP248.13-248.65 ,Genetics ,QH426-470 - Abstract
Abstract Background Elucidating the genetic variation underlying phenotypic diversity will facilitate improving production performance in livestock species. The Tibetan sheep breed in China holds significant historical importance, serving as a fundamental pillar of Qinghai’s animal husbandry sector. The Plateau-type Tibetan sheep, comprising 90% of the province’s population, are characterized by their tall stature and serve as the primary breed among Tibetan sheep. In contrast, Zhashijia sheep exhibit larger size and superior meat quality. These two species provide an excellent model for elucidating the genetic basis of body size variation. Therefore, this study aims to conduct a comprehensive genome-wide association study on these two Tibetan sheep breeds to identify single nucleotide polymorphism loci and regulatory genes that influence body size traits in Tibetan sheep. Result In this study, the phenotypic traits of body weight, body length, body height, chest circumference, chest depth, chest width, waist angle width, and pipe circumference were evaluated in two Tibetan sheep breeds: Plateau-type sheep and Zhashijia Tibetan sheep. Whole genome sequencing generated 48,215,130 high-quality SNPs for genome-wide association study. Four methods were applied and identified 623 SNPs significantly associated with body size traits. The significantly associated single nucleotide polymorphisms identified in this study are located near or within 111 candidate genes. These genes exhibit enrichment in the cAMP and Rap1 signaling pathways, significantly affecting animal growth, and body size. Specifically, the following genes were associated: ASAP1, CDK6, FRYL, NAV2, PTPRM, GPC6, PTPRG, KANK1, NTRK2 and ADCY8. Conclusion By genome-wide association study, we identified 16 SNPs and 10 candidate genes associated with body size traits in Tibetan sheep, which hold potential for application in genomic selection breeding programs in sheep. Identifying these candidate genes will establish a solid foundation for applying molecular marker-assisted selection in sheep breeding and improve our understanding of body size control in farmed animals.
- Published
- 2024
- Full Text
- View/download PDF
64. Independent directors’ geographic distance, high-speed railway, and corporate cash holdings
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Duo Shang, Dongliang Yuan, Dehui Li, and Qi Lin
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Economics and Econometrics - Published
- 2023
65. Epitaxial growth of CsPbBr3-PbS vertical and lateral heterostructures for visible to infrared broadband photodetection
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Qingbo Liu, Hong Zhou, Hongzhi Shen, Lihan Liang, and Dehui Li
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Materials science ,business.industry ,Infrared ,Detector ,Photodetector ,Heterojunction ,02 engineering and technology ,Photodetection ,010402 general chemistry ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Epitaxy ,01 natural sciences ,Atomic and Molecular Physics, and Optics ,0104 chemical sciences ,Broadband ,Optoelectronics ,General Materials Science ,Electrical and Electronic Engineering ,0210 nano-technology ,business ,Perovskite (structure) - Abstract
Owing to their excellent optoelectronic properties, halide perovskite is very promising for photodetectors and other optoelectronic devices. Perovskite heterostructures are considered to be the key components for these devices. However, it is challenging to rationally synthesize those heterostructures. Here, we demonstrate that perovskite can be epitaxially grown on PbS by vapor transport, thereby creating an interesting CsPbBr3-PbS heterostructure. Remarkably, photodetectors based on CsPbBr3-PbS heterostructures exhibit visible to infrared broadband response with room temperature operation up to 2 μm. The room temperature detectivity higher than 1.0 × 109 Jones was obtained in the 1.8- to 2-μm range. Furthermore, the p-n heterojunction exhibits a clear rectifying characteristic and enables detector to operate at zero-bias. Our study provides fundamentally contributes to establish the epitaxial growth perovskite heterostructures and demonstrate a materials platform for efficient perovskite-based optoelectronic devices.
- Published
- 2021
66. 2D perovskite narrowband photodetector arrays
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Lu Li, Jiaqi Ma, Haizhen Wang, Junze Li, and Dehui Li
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Materials science ,Band gap ,business.industry ,Optical communication ,Photodetector ,General Chemistry ,Full width at half maximum ,Wavelength ,Narrowband ,Materials Chemistry ,Optoelectronics ,Quantum efficiency ,Monochromatic color ,business - Abstract
Narrowband photodetectors, which are capable of detecting light within a narrow spectral range, have important applications in the fields of digital cameras, biosensing and artificial vision. In particular, 2D layered perovskites stand out as good candidate materials for narrowband photodetectors due to their prominent properties, such as natural quantum-well structure and tunable bandgap. Although narrowband photodetectors based on 2D perovskites have been presented recently, for some practical applications, including optical communication and imaging, narrowband photodetector arrays need to be prepared, which has not been reported yet. Here, we have demonstrated the fabrication of 12 × 11 narrowband photodetector arrays based on 2D (BA)2PbI4 perovskites to realize imaging for the first time. The as-prepared photodetector exhibits a narrow photo-response peak centered at around 546 nm with a full width at half maximum of 24 nm. Besides, it shows a high external quantum efficiency of 350% and a detectivity of 2.17 × 1011 Jones under 546 nm illumination. Furthermore, the narrowband photodetector arrays can also realize imaging under monochromatic light illumination from the back side of the device with wavelength selection.
- Published
- 2021
67. A photoelectrochemical biofuel cell based on a TiO2 nanotube array fluorine-doped tin oxide photoanode
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Louqun Wang, Lili Ji, Jing Yang, Dehui Li, and Chunping Xiao
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Chemical energy ,Chemical engineering ,Chemistry ,Biofuel ,Tio2 nanotube ,Doping ,Fluorine ,chemistry.chemical_element ,General Chemistry ,Tin oxide ,Biofuel Cells ,Cell based - Abstract
Photoelectrochemical biofuel cells can convert light and chemical energy into electrical energy using a dye-sensitized titania (TiO2) fluorine-doped tin oxide photoanode and a platinum-coated fluorine-doped tin oxide cathode. TiO2 of the photoanode serves both as a support for dyes and as an electron-transporting medium, the structure of which can limit electron trapping and charge transporting and then affect the performance of the photoelectrochemical biofuel cells. TiO2 nanotube array films have been shown to enhance the efficiencies of both charge collection and electron injection, and hence a vertically aligned TiO2 nanotube array is investigated as a conductor for the tetrakis(4-carboxyphenyl)porphyrin dye to construct a new two-compartment photoelectrochemical biofuel cell. The photoelectrochemical biofuel cell containing the TiO2 nanotube array photoanode yields a short-circuit (Isc) current of 110 μA and an open-circuit (Voc) potential of 1010 mV. In contrast, the photovoltaic parameters, Isc and Voc of the photoelectrochemical biofuel cell with the mesoporous TiO2 nanocrystal fluorine-doped tin oxide photoanode, are 96.96 μA and 740 mV, respectively. Photovoltaic measurements show that the maximum incident photon-to-collected electron conversion efficiency was 58% at 430 nm through the spectral range (400–800 nm) for the photoelectrochemical biofuel cell with the TiO2 nanotube array fluorine-doped tin oxide photoanode. These results revealed that the TiO2 nanotube array had great potential for the photoelectrochemical biofuel cells.
- Published
- 2020
68. Application of soil phytoliths to the quantitative characterization of temperate grassland ecosystems: a case study in Northeast China
- Author
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Dehui Li, Guihua Zhang, Jiangyong Wang, Meng Meng, Honghao Niu, Hongyan Liu, Lidan Liu, Nannan Li, Ying Liu, Dongmei Jie, and Guizai Gao
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0106 biological sciences ,Biomass (ecology) ,geography ,geography.geographical_feature_category ,Ecology ,Soil Science ,Plant community ,04 agricultural and veterinary sciences ,Plant Science ,01 natural sciences ,Grassland ,Diversity index ,Abundance (ecology) ,Phytolith ,040103 agronomy & agriculture ,0401 agriculture, forestry, and fisheries ,Environmental science ,Ecosystem ,Species richness ,010606 plant biology & botany - Abstract
Although phytolith analysis is a promising tool for reconstructing the palaeovegetation in grassland ecosystems, no phytolith study has yet attempted to quantitatively reconstruct the corresponding plant community characteristics. Questions remain regarding whether or not soil phytoliths can quantitatively reflect various aspects of grassland physiognomy, and how well modern phytoliths represent the quantitative characteristics of grassland ecosystems. These are important scientific issues in the field of phytolith analysis, which require further research on the modern phytoliths of grassland ecosystems. In order to explore the potential of phytolith analysis in the temperate grassland region, we have for the first time established a modern soil phytolith reference dataset by exploring the relationships between soil phytoliths and plant species inventory data from 77 sites in the Songnen grassland in Northeast China. The results show that phytolith assemblages can clearly distinguish Leymus chinensis grassland, Stipa grassland and mesophytic herb grassland. In addition, we found that the Ic phytolith index could discriminate samples of L. chinensis grassland from the other samples, while the Iph phytolith index proved to be less reliable in the region. In addition, in terms of quantitative plant community characteristics, the soil phytoliths showed a good correspondence with plant community cover and species richness, but not with biomass and diversity index. The transfer functions established in this study can provide reliable estimates of community cover and species richness in the Songnen grassland. In addition, phytoliths are shown to have the potential to reconstruct the taxonomic abundance of the aboveground plant community. This study is a major advance in the application of phytolith analysis to the quantitative estimation of plant community characteristics, and it provides a modern phytolith reference for the quantitative reconstruction of the paleovegetation of grassland ecosystems.
- Published
- 2020
69. The Universal Growth of Ultrathin Perovskite Single Crystals
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Linyi Li, Yantao Yu, Peng Li, Jinxin Liu, Lihan Liang, Luyang Wang, Yu Ding, Xiaocang Han, Jiamin Ji, Shengli Chen, Dehui Li, Pan Liu, Shunping Zhang, Mengqi Zeng, and Lei Fu
- Subjects
Mechanics of Materials ,Mechanical Engineering ,General Materials Science - Abstract
Perovskites have engaged significant attention owing to rich species and remarkable physical properties as well as optoelectronic applications. Compared to bulk counterparts, ultrathin perovskites exhibit more available compositions due to the breaking of bulk lattice limitation. Coupled with crystal lattice relaxation and quantum confinement, infinite intriguing properties of ultrathin perovskites deserve to be explored. Developing ultrathin perovskites with alterable composition and structure is a necessity to fully explore this versatile family. Herein, a universal strategy is conceived via constructing oriented solvent microenvironment induced by the interfacial electric field originated from the charge separation between solid and liquid phases, which is conducive to controlling the precursor distribution and makes crystals preferentially nucleate and grow in the preferentially lateral mode. From layered to nonlayered, organic to inorganic, and toxic to low-toxic lead-free perovskite, a full-range synthesis is achieved of ultrathin perovskites. This work opens up opportunities both for ultrathin perovskite exploration through compositional engineering and for device miniaturization in energy conversion applications.
- Published
- 2022
70. Focus Shift and Phase Correction in Soft Tissues During Focused Ultrasound Surgery.
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Dehui Li, Guofeng Shen, Jingfeng Bai, and Yazhu Chen
- Published
- 2011
- Full Text
- View/download PDF
71. A Study of Heating Duration and Scanning Path in Focused Ultrasound Surgery.
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Dehui Li, Guofeng Shen, Hui Luo, Jingfeng Bai, and Yazhu Chen
- Published
- 2011
- Full Text
- View/download PDF
72. Manipulation of Valley Pseudospin by Selective Spin Injection in Chiral Two-Dimensional Perovskite/Monolayer Transition Metal Dichalcogenide Heterostructures
- Author
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Zeyi Liu, Xiangfeng Duan, Jiaqi Ma, Yingying Chen, Junze Li, and Dehui Li
- Subjects
education.field_of_study ,Materials science ,Spintronics ,business.industry ,Population ,General Engineering ,General Physics and Astronomy ,02 engineering and technology ,010402 general chemistry ,021001 nanoscience & nanotechnology ,Polarization (waves) ,01 natural sciences ,0104 chemical sciences ,Valleytronics ,Monolayer ,Optoelectronics ,General Materials Science ,0210 nano-technology ,business ,education ,Circular polarization ,Excitation ,Perovskite (structure) - Abstract
Monolayer two-dimensional (2D) transition metal dichalcogenides (TMDs) have attracted great interest in spintronics and valleytronics due to the spin-valley locking effect. To efficiently control and manipulate the valley pseudospin is of paramount importance for valley-based electronics and optoelectronics. A variety of strategies have been developed to address the valley pseudospin including optical, electrical, and magnetic methods; nonetheless, they involve either below liquid-nitrogen temperature or an external magnetic field, which increases the cost and complexity of the devices. Here, we report a straightforward way to manipulate valley polarization in monolayer TMDs via selective spin injection in chiral 2D perovskite/monolayer TMD (e.g., MoS2 and WSe2) van der Waals heterostructures without requiring an external magnetic field or specially designed device structures. We show the dangling-bond-free vdW interface can allow an impressive average spin injection efficiency of 78% to produce persistent valley polarization in monolayer MoS2 (WSe2) over 10% from liquid-nitrogen temperature to above 200 K. We attribute the valley polarization of monolayer MoS2 (WSe2) to selective spin injection from chiral 2D perovskites, which can effectively introduce population imbalance between valleys in monolayer MoS2 (WSe2). Our findings provide an alternative strategy to manipulate the valley polarization in TMDs without requiring circularly polarized light excitation, below liquid-nitrogen temperature, or external magnetic field, and thus would promote the development of perovskite-based spintronic and valleytronic devices.
- Published
- 2020
73. An evaluation of soil phytoliths for reconstructing plant communities and palaeoclimate in the northern temperate region
- Author
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Hongyan Liu, Dehui Li, Dongmei Jie, Nannan Li, Lidan Liu, and Guizai Gao
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Topsoil ,Phytolith ,Temperate climate ,Soil Science ,Climate change ,Plant community ,Glacial period ,Precipitation ,Species richness ,Physical geography ,Geology - Abstract
Phytoliths can act as efficient carriers of information about palaeovegetation and palaeoclimatic conditions, but the representativeness of soil phytoliths from palaeoecological sediments has not been fully understood. In this study, phytolith assemblages in topsoils and associated plant communities at 55 sites in Northeast China were compared. The results indicate that samples from herbaceous and woody communities could be reliably differentiated by topsoil phytoliths. Notably, different phytolith types exhibit varying degrees of representational bias in terms of the aboveground plant community. Some morphotypes (e.g., bilobate, rondel and lanceolate) over‐represent the richness of the corresponding plant; some morphotypes, including microhair, conical epidermal, silicified stomata and epidermal phytoliths, under‐represent the parent plant abundance; additional morphotypes (e.g., elongate, saddle and trapeziform sinuate) are consistent with the changes of associated plants. Based on the representational bias, we calibrated the percentages of topsoil phytoliths and established a phytolith‐based transfer function for precipitation in Northeast China. A palaeoclimate reconstruction in the Changbai Mountains (in the eastern part of Northeast China) based on the above phytolith‐based transfer function for precipitation shows that the region has gone through continuous climatic changes since the late glacial period: from cold and dry conditions to warm and dry conditions, then to warm and wet conditions, and finally to cool and dry conditions. The phytolith‐based reconstructed climate changes since the late glacial period correspond well to those reconstructed by other records from the same stratigraphic profile, and our phytolith‐based climatic reconstruction also confirms the reliability of abrupt cold climatic shifts at 8.2, 6.8, 5.6, 4.6 and 4.2 ka. In conclusion, our results provide the basis for the reliability of phytoliths for reconstructing climatic changes in the northern temperate region. HIGHLIGHTS: Calibrating soil phytolith assemblages for any quantitative palaeovegetation reconstruction using phytoliths is necessary. Phytolith morphotypes in topsoils may over‐ or under‐represent or agree with the abundance of modern plant taxa. Phytolith‐based climatic reconstruction corresponds well with the abrupt climate changes evident since the Late Glacial period and other proxy records.
- Published
- 2020
74. Two-dimensional water layer of cube-like or bowl-shaped clusters in a three-dimensional supramolecule (C10H18N)3Fe(CN)6·17H2O
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Dehui Li, Bo Sun, Yanping Miao, and Jing Yang
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Interconnection ,Materials science ,chemistry.chemical_element ,02 engineering and technology ,General Chemistry ,010402 general chemistry ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,01 natural sciences ,Oxygen ,0104 chemical sciences ,Crystallography ,Water layer ,chemistry ,Molecule ,General Materials Science ,Cube ,0210 nano-technology ,Hydrate ,Layer (electronics) - Abstract
Two-dimensional (2D) layer of water molecules has been observed in crystalline hydrate (C10H18N)3Fe(CN)6·17H2O (1). The layer is generated by interconnection of cube-like clusters by two oxygen ato...
- Published
- 2020
75. Giant enhancement of photoluminescence quantum yield in 2D perovskite thin microplates by graphene encapsulation
- Author
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Xue Cheng, Dehui Li, Wancai Li, and Jiaqi Ma
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Materials science ,Photoluminescence ,business.industry ,Graphene ,Quantum-confined Stark effect ,Quantum yield ,Condensed Matter Physics ,Atomic and Molecular Physics, and Optics ,law.invention ,Quantum dot ,law ,Monolayer ,Optoelectronics ,General Materials Science ,Spontaneous emission ,Electrical and Electronic Engineering ,business ,Perovskite (structure) - Abstract
The optoelectronic performances of the layered materials are strongly dependent on the thickness of the samples due to the surface effect. As the size of the samples decreases to few nanometers, the surface depletion field and surface defect density are prominent arising from the large surface to volume ratio. For instance, thin two-dimensional (2D) organic-inorganic hybrid perovskite microplates usually exhibit a rather low photoluminescence quantum yield (PLQY), owning to the strong surface effect. Here, we report that the PLQY can be enhanced as large as 28 times in (iso-BA)2Pbl4 (BA = C4H9NH3) 2D perovskite thin microplates encapsulated by graphene, resulting in that the PLQY is more than 18% for the microplate with a thickness of 6.7 nm at 78 K. As the thickness of the 2D perovskite microplate increases, the enhancement is gradually reduced and finally vanishes. This observation is in striking contrast to that in monolayer transition metal dichalcogenides (TMDs), when the PLQY is quenched by covering a layer of graphene due to the efficient charge transfer. The enhancement of PLQY in 2D perovskites can be mainly ascribed to the reduced quantum confined Stark effect (QCSE) due to the reduced surface depletion field after covering graphene flake, resulting in the enhanced radiative recombination efficiency. Our findings provide a cost-effective approach to enhance the luminescence, which may pave the way toward high performance light emitting devices based on 2D perovskites.
- Published
- 2020
76. Robust Interlayer Coupling in Two-Dimensional Perovskite/Monolayer Transition Metal Dichalcogenide Heterostructures
- Author
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Haizhen Wang, Yingying Chen, Xue Cheng, Jiaqi Ma, Zeyi Liu, Dehui Li, and Junze Li
- Subjects
Coupling ,Van der waals heterostructures ,Materials science ,Condensed matter physics ,Exciton ,General Engineering ,General Physics and Astronomy ,Heterojunction ,02 engineering and technology ,010402 general chemistry ,021001 nanoscience & nanotechnology ,01 natural sciences ,0104 chemical sciences ,Transition metal ,Monolayer ,General Materials Science ,0210 nano-technology ,Science, technology and society ,Perovskite (structure) - Abstract
Interlayer excitons have been extensively studied in monolayer transition metal dichalcogenide (TMD) heterobilayers mainly due to the long lifetime, which is beneficial for a wide range of optoelectronic applications. To date, the majority of investigations of interlayer excitons in TMD heterobilayers have been focusing on the geometric arrangement of structures, spin-valley lifetime, and interlayer valley excitons with interlayer hopping rules. Nevertheless, interlayer excitons in TMD heterobilayers strongly depend on the local atomic registry and coupling strength, which increase the complexity of the device fabrication. Here, we report pronounced interlayer exciton emission in two-dimensional (2D) perovskite/monolayer TMD heterostructures without the need of thermal annealing or specific geometric arrangements, and the interlayer exciton emission is rather general among 2D perovskites and monolayer TMDs. Such interlayer exciton emission completely dominates the emission spectrum at 78 K regardless of the stacking sequence, suggesting the robust interlayer coupling in 2D perovskite/monolayer TMD heterostructures. Furthermore, the interlayer exciton emission shows a large blue-shift with increasing laser intensity due to the repulsive dipole-dipole interaction and can persist above 220 K. Importantly, the interlayer exciton emission also possesses robust circular polarization in chiral 2D perovskite/monolayer WSe
- Published
- 2020
77. Preservation of common soil phytoliths in the northern temperate region: a case study from northeast China
- Author
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Dehui Li, Dongmei Jie, Hongyan Liu, Guizai Gao, Nannan Li, and Lidan Liu
- Subjects
Archeology ,Temperate climate ,Geology ,Physical geography ,China ,Ecology, Evolution, Behavior and Systematics - Published
- 2020
78. Large Optical Anisotropy in Two-Dimensional Perovskite [CH(NH2)2][C(NH2)3]PbI4 with Corrugated Inorganic Layers
- Author
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Ming Xu, Jiaqi Ma, Jun Wang, Meng Xu, Chen Fang, Long Jin, and Dehui Li
- Subjects
Nanostructure ,Optical anisotropy ,Materials science ,Mechanical Engineering ,Physics::Optics ,Halide ,Bioengineering ,02 engineering and technology ,General Chemistry ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Crystal ,Condensed Matter::Materials Science ,Chemical physics ,General Materials Science ,0210 nano-technology ,Polarization (electrochemistry) ,Perovskite (structure) - Abstract
Optical anisotropy plays an indispensable role in a variety of optical components. Organic halide perovskites often rely on artificially oriented nanostructures to enhance optical anisotropy due to...
- Published
- 2020
79. Biexcitons in 2D (iso-BA)2PbI4 perovskite crystals
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Chen Fang, Haizhen Wang, Wancai Li, Hongmei Luo, Dehui Li, and Jiaqi Ma
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Optical anisotropy ,Materials science ,QC1-999 ,02 engineering and technology ,010402 general chemistry ,2d perovskites ,01 natural sciences ,Nanomaterials ,Electrical and Electronic Engineering ,Biexciton ,Quantum well ,Perovskite (structure) ,Condensed Matter::Quantum Gases ,Condensed matter physics ,Condensed Matter::Other ,Physics ,021001 nanoscience & nanotechnology ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,Atomic and Molecular Physics, and Optics ,0104 chemical sciences ,Electronic, Optical and Magnetic Materials ,optical anisotropy ,quantum wells ,biexcitons ,0210 nano-technology ,Biotechnology - Abstract
Two-dimensional (2D) organic-inorganic hybrid perovskites have attracted growing attention recently due to their naturally formed quantum-well structure, unique photoelectric properties and better environmental stability compared to three-dimensional perovskites. The reduced screening and enhanced Coulomb interaction in 2D perovskites result in the formation of excitonic complexes. While the properties of free excitons have been well investigated, studies on biexcitons remain elusive. Here, we report on the biexcitons in 2D (iso-BA)2PbI4 (BA=C4H9NH3) crystals. The biexciton emission can be observed under a very low excitation power density of 6.4 W/cm2 at 78 K. The biexciton exhibits a large biexciton binding energy of 46 meV due to the large exciton binding energy of (iso-BA)2PbI4. Furthermore, the biexcitons exhibit a favorable polarization orientation, resulting in different anisotropy between biexcitons and excitons. Our findings would motivate more studies on biexcitons in 2D perovskites and pave the way for exploiting the many-body physics for biexciton lasing and optical storage devices.
- Published
- 2020
80. Circularly Polarized Luminescence from Chiral Tetranuclear Copper(I) Iodide Clusters
- Author
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Dehui Li, Guangda Niu, Xu-Feng Luo, Yuhao Liu, You-Xuan Zheng, Junze Li, Peipei Du, Jiang Tang, Liang Gao, Zewen Xiao, Bing Xia, Li Yao, and Chao Chen
- Subjects
Circular dichroism ,Photoluminescence ,Materials science ,chemistry.chemical_element ,02 engineering and technology ,010402 general chemistry ,021001 nanoscience & nanotechnology ,01 natural sciences ,Copper ,Spectral line ,0104 chemical sciences ,Organic molecules ,chemistry.chemical_compound ,Crystallography ,chemistry ,General Materials Science ,Physical and Theoretical Chemistry ,Enantiomer ,0210 nano-technology ,Copper(I) iodide ,Luminescence - Abstract
Circularly polarized luminescent (CPL) materials are promising in applications such as 3D displays and quantum communication. Hybrid organic-inorganic copper(I) iodides have been rapidly developed due to their intense photoluminescence and structural diversity; nevertheless, the reported Cu-I clusters rarely show CPL activities. In this study, we introduced chiral organic molecules R/S-methylbenzylammonium (R/S-MBA) into Cu-I inorganic skeletons to achieve chiral tetranuclear (R/S-MBA)4Cu4I4 clusters with intense orange luminescence and CPL activity at room temperature. These enantiomeric (R/S-MBA)4Cu4I4 clusters show oppositely signed circular dichroism (CD) signals, which agree well with their simulated electronic CD spectra. The crystallization-induced helical arrangement of (R/S-MBA)4Cu4I4 clusters and their largely distorted polynuclear configuration demonstrate a new platform for the study of chiral-related properties.
- Published
- 2020
81. Reversible luminescent humidity chromism of organic–inorganic hybrid PEA2MnBr4 single crystals
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Wanru Gao, Liang Gao, Huan Liu, Meiying Leng, Dehui Li, Guangda Niu, Junze Li, Jiang Tang, and Zhixiang Hu
- Subjects
Inorganic Chemistry ,Diffraction ,Detection limit ,chemistry.chemical_compound ,Materials science ,chemistry ,Chromism ,Chemical engineering ,Humidity ,Relative humidity ,Selectivity ,Luminescence ,Toluene - Abstract
Organic–inorganic hybrids have drawn great attention for gas sensors due to their high sensitivity, good selectivity and acceptable stability at room temperature. There are two main approaches by which organic–inorganic hybrids convert gas information to electric or optical signals (vapochromism). Here, we have reported a new organic–inorganic hybrid PEA2MnBr4 for humidity detection by luminescent visible chromism. PEA2MnBr4 single crystals were grown by the solution method and determined by single-crystal X-ray diffraction. Luminescent humidity chromism was found on PEA2MnBr4 from green emission at the water-desorption state to pink emission at the water-adsorption state within 18 s at a relative humidity of 38% RH. This obviously visible chromism was further used to check the water content in toluene with a low detection limit between 0.02 and 0.05 vol%.
- Published
- 2020
82. Digital Transformation and Slack Resource Reconstruction: How Companies Promote Innovation in Digital Era
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Dehui Li and Lijun Pan
- Published
- 2022
83. Application of a Topsoil Phytolith Dataset for Quantitative Paleoclimate Reconstruction in Northeast China
- Author
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Lina Song, Dongmei Jie, Guizai Gao, Lidan Liu, Hongyan Liu, Dehui Li, and Ying Liu
- Subjects
History ,Polymers and Plastics ,Business and International Management ,Industrial and Manufacturing Engineering - Published
- 2022
84. Economic-Environment Equilibrium Strategy Based Production Quota Allocation Towards Coal Industry Structure Optimization: Case Study from China
- Author
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Kejing Shu, Dehui Li, and Yi Lu
- Published
- 2022
85. A chain-type diamine strategy towards strongly anisotropic triiodide of DMEDA·I6
- Author
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Wanru Gao, Guangda Niu, Peng Xu, Dehui Li, Junze Li, Li Yao, Liang Gao, Jiang Tang, and Shiyou Chen
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Materials science ,02 engineering and technology ,010402 general chemistry ,021001 nanoscience & nanotechnology ,Linear dichroism ,Dichroic glass ,01 natural sciences ,0104 chemical sciences ,Ion ,chemistry.chemical_compound ,Electron transfer ,Effective mass (solid-state physics) ,chemistry ,Chemical physics ,General Materials Science ,Triiodide ,0210 nano-technology ,Anisotropy ,Single crystal - Abstract
Linearly bonded triiodide chains with fairly small distance between the adjacent iodine ions feature a facile electron transfer and highly anisotropic properties. Here, we demonstrate a novel strategy towards a new one-dimensional linear triiodide DMEDA·I6, using chain-type N,N′-dimethyl-ethanediamine (DMEDA) cation to coordinate triiodine ions. This triiodide has the shortest distance between adjacent I3 and good linearity. An estimated electronic band gap of 1.36 eV indicates its semiconducting properties. 100 fold differences both in polarization-sensitive absorption and effective mass were achieved by simulation, with directions parallel and perpendicular to the a-axis of DMEDA·I6. The DME-DA·I6 single crystal-based photodetectors show a good switching characteristic and a distinct polarization-sensitive photoresponse with linear dichroic photodetection ratio of about 1.9. Strongly anisotropic features and semiconducting properties of DMEDA·I6 make this triiodide system an interesting candidate for polarization related applications.
- Published
- 2019
86. Xihuang Pill Inhibits The Development of DMBA Combined With Oestrogen- And Progesterone-Induced Precancerous Breast lesions In Rats By The PI3K/AKT/mTOR Signaling Pathway
- Author
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Dehui Li, Yi-ting Gu, Jing-fei Dong, Jiao Liu, Huanfang Fan, Chunxia Sun, Yifan Su, and Na Guo
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business.industry ,Pill ,MTOR signaling pathway ,Cancer research ,Medicine ,DMBA ,business ,Protein kinase B ,PI3K/AKT/mTOR pathway - Abstract
Background:To study the inhibitory effect of Xihuang pill on the development of DMBA combined with oestrogen- and progesterone-induced breast precancerous lesions in rats by the PI3K/AKT/mTOR signaling pathway and to explore the effect of Xihuang pill in preventing and treating breast cancer. Method: Establishment of a rat model of precancerous breast lesions with DMBA combined with oestrogen and progesterone sequential induction for 10 weeks. Xihuang pill was administered continuously by gavage for 4 weeks. Rat breast tissue was stained with haematoxylin-eosin (HE). The pathomorphological changes were observed with a light microscope. TUNEL staining was used to detect cell apoptosis in breast tissue. Western blotting was used to detect the protein expression of P-PI3K, P-AKT (S473), P-AKT (T308), PTEN, P-tuberin/TSC2, P-tuberin (p-S939), p-mTOR, and P-4E-BP1 in breast tissues. qRT-PCR was used to detect the gene expression of PTEN mRNA and VEGF mRNA. Immunohistochemistry was used to detect the protein expression of P-S6, p-p70s6k and VEGF.Result:Compared with the disease model group, the low-, middle- and high-dose Xihuang pill groups could significantly reduce the degree of breast pathology, and the number of apoptotic precancerous breast lesion cells increased with increasing Xihuang pill dose. The expression levels of P-PI3K, P-AKT (S473), P-AKT (T308), p-mTOR, P-4E-BP1, p-S6, p-p70S6K, VEGF protein and VEGF mRNA dropped with increasing Xihuang pill dose. The expression levels of PTEN, P-tuberin/TSC2, P-tuberin (p-S939) protein and PTEN mRNA increased with increasing Xihuang pill dose. Conclusion:Xihuang pill can promote the apoptosis of precancerous breast lesion cells, reduce the proliferation of vascular endothelial cells, and then inhibit the progression of precancerous breast lesions. Its mechanism is probably associated with the regulation of the PI3K/AKT/mTOR pathway related protein expression.
- Published
- 2021
87. Two-Dimensional Hybrid Perovskite-Based van der Waals Heterostructures
- Author
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Haizhen Wang, Jiaqi Ma, and Dehui Li
- Subjects
Van der waals heterostructures ,Materials science ,business.industry ,Band gap ,Photodetector ,Heterojunction ,law.invention ,law ,Optoelectronics ,General Materials Science ,Physical and Theoretical Chemistry ,business ,High absorption ,Perovskite (structure) ,Diode ,Light-emitting diode - Abstract
Two-dimensional (2D) hybrid perovskites, as newly emerging materials, have become the center of attention in optoelectronic fields within a few years because of their unique optoelectronic properties, including tunable bandgap, long carrier diffusion length, and high absorption coefficient. 2D perovskite-based van der Waals heterostructures via integration of 2D perovskites with other layered materials provide new platforms for many optoelectronic devices with prominent performance, such as photodetectors, light-emitting diodes (LEDs), and phototransistors. In this Perspective, the unique properties of 2D perovskites will be first introduced to explore why this material is attractive and popular. Subsequently, various types of heterostructures based on 2D perovskites will be illustrated, including the heterostructure construction approaches as well as their optical and optoelectronic applications. Finally, potential research directions based on 2D perovskite heterostructures are also proposed.
- Published
- 2021
88. Full-Stokes Polarimeter Based on Chiral Perovskites with Chirality and Large Optical Anisotropy
- Author
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Haizhen Wang, Lihan Liang, Jiaqi Ma, Dehui Li, and Chen Fang
- Subjects
Physics ,business.industry ,Photodetector ,Polarimeter ,General Chemistry ,Polarizer ,Polarization (waves) ,Waveplate ,law.invention ,Biomaterials ,law ,Optoelectronics ,General Materials Science ,business ,Anisotropy ,Circular polarization ,Biotechnology ,Perovskite (structure) - Abstract
Full-Stokes polarimeters, equipped with the capability of discriminating light polarization states, can find important applications in various optical and optoelectronic devices. Nevertheless, currently most full-Stokes polarimeters require complex and bulky optical elements or optical metasystems integrated with metasurfaces, which can increase the cost and cause energy loss. Here, the anisotropy of chiral 2D perovskite single crystals is explored and the full-Stokes polarimeter based on pure chiral 2D perovskite single crystals is reported. By using optical anisotropy and the ability to distinguish the helicity of the circularly polarized light, chiral 2D perovskite polarimeter integrates the polarizer, waveplate, and photodetector together and thus can be able to discriminate the polarization states of light. The as-fabricated device exhibits a photoresponsivity of 0.136 A W-1 and a detectivity of 1.2 × 1010 Jones. This study provides a paradigm to construct filterless on-chip Stokes polarimeter with great simplicity and low cost.
- Published
- 2021
89. Longer serum phosphorus time in range associated with lower mortality risk among peritoneal dialysis patients: a multicenter retrospective cohort study
- Author
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Zhihao Huo, Dehui Liu, Peiyi Ye, Yuehang Zhang, Lisha Cao, Nirong Gong, Xianrui Dou, Chengfa Ren, Qingyao Zhu, Dan Li, Wei Zhang, Yaozhong Kong, Guobao Wang, and Jun Ai
- Subjects
Peritoneal dialysis ,Serum phosphorus ,Time in range ,All-cause mortality ,Cardiovascular mortality ,Peritoneal dialysis withdrawal ,Diseases of the genitourinary system. Urology ,RC870-923 - Abstract
Abstract Background Relationship between serum phosphorus time in range and mortality risk in peritoneal dialysis (PD) patients remains uncertain. We aimed to evaluate the association between serum phosphorus time in range and all-cause mortality in Chinese PD population. Methods This was a multicenter, retrospective, cohort study of 1,915 patients collected from January 2008 to October 2020 in 4 Chinese centers. Serum phosphorus time in range was estimated as the months during the first year that a patient’s serum phosphorus level was within the target range (defined as 1.13–1.78 mmol/L). The primary outcome was all-cause mortality. The secondary outcomes were cardiovascular (CV) mortality and PD withdrawal. Cox proportional hazards regression model with comprehensive adjustments was used to assess the association. Results The primary outcome occurred in 249 (13.0%) PD patients over a median follow-up of 28 months. Overall, the serum phosphorus time in range was negatively associated with all-cause mortality (per 3-month increments, adjusted HR [aHR], 0.83; 95%CI: 0.75–0.92), CV mortality (per 3-month increments, aHR, 0.87; 95%CI: 0.77–0.99), and PD withdrawal (per 3-month increments, aHR, 0.89; 95%CI: 0.83–0.95). Competing-risk model showed that the relationship of serum phosphorus time in range with all-cause mortality remained stable. None of the variables including demographics, history of diabetes and CV disease, as well as several PD-related and clinical indicators modified this association. Conclusions PD patients with longer serum phosphorus time in range in the first year was negatively associated with all-cause mortality and CV mortality. Our findings highlight the importance of maintaining serum phosphorus levels within 1.13–1.78 mmol/L for PD patients.
- Published
- 2024
- Full Text
- View/download PDF
90. Low‐Power Logic‐in‐Memory Complementary Inverter Based on p‐WSe 2 and n‐WS 2
- Author
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Hongzhi Shen, Junwen Ren, Junchao Hu, Zeyi Liu, Yingying Chen, Xinglin Wen, and Dehui Li
- Subjects
Electronic, Optical and Magnetic Materials - Published
- 2022
91. Application of a topsoil phytolith dataset to quantitative paleoclimate reconstruction in Northeast China
- Author
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Lina Song, Dongmei Jie, Guizai Gao, Lidan Liu, Hongyan Liu, Dehui Li, and Ying Liu
- Subjects
Paleontology ,Oceanography ,Ecology, Evolution, Behavior and Systematics ,Earth-Surface Processes - Published
- 2022
92. Self-Powered Filterless On-Chip Full-Stokes Polarimeter
- Author
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Chen Fang, Dehui Li, Boxuan Zhou, and Junze Li
- Subjects
FOS: Physical sciences ,Bioengineering ,Applied Physics (physics.app-ph) ,symbols.namesake ,Electric field ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,Stokes parameters ,General Materials Science ,Homojunction ,Physics ,Condensed Matter - Mesoscale and Nanoscale Physics ,business.industry ,Mechanical Engineering ,Polarimeter ,Physics - Applied Physics ,General Chemistry ,Sense (electronics) ,Condensed Matter Physics ,Polarization (waves) ,Ray ,symbols ,Optoelectronics ,Photonics ,business ,Optics (physics.optics) ,Physics - Optics - Abstract
The detection of polarization states of light is essential in photonic and optoelectronic devices. Currently, the polarimeters are usually constructed with the help of waveplates or a comprehensive metasurface, which will inevitably increase the fabrication complexity and unnecessary energy loss. Here, we have successfully demonstrated a self-powered filterless on-chip full-Stokes polarimeter based on a single-layer MoS2/few-layer MoS2 homojunction. Combining the built-in electric field enhanced circular photogalvanic effect with the intrinsic optical anisotropy of MoS2 between in-plane and out-of-plane direction, the device is able to conveniently sense four Stokes parameters of incident light at zero bias without requiring an extra filtering layer, and can function in the wavelength range of 650-690 nm with acceptable average errors. Besides, this homojunction device is easy to integrate with silicon-based chips and could have much smaller sizes than metasurface based polarimeters. Our study thus provides an excellent paradigm for high-performance on-chip filterless polarimeters., 22 pages, 4 figures
- Published
- 2021
93. Early effects of crop tree management on undergrowth plant diversity and soil physicochemical properties in a Pinus massoniana plantation
- Author
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Shen Yi, Li Xianwei, Chuan Fan, Lyu Qian, Dehui Li, and Gang Chen
- Subjects
0106 biological sciences ,Pinus massoniana ,010504 meteorology & atmospheric sciences ,Dominant species ,ved/biology.organism_classification_rank.species ,Soil Science ,Plant Science ,010603 evolutionary biology ,01 natural sciences ,Shrub ,General Biochemistry, Genetics and Molecular Biology ,Crop trees ,Forest ecology ,0105 earth and related environmental sciences ,Soil physicochemical properties ,Topsoil ,biology ,Ecology ,ved/biology ,General Neuroscience ,Soil organic matter ,Forestry ,General Medicine ,Understory ,Vegetation ,biology.organism_classification ,Agronomy ,Plant diversity ,Environmental science ,Medicine ,General Agricultural and Biological Sciences ,Undergrowth - Abstract
Background Soil and understory vegetation are vital components of forest ecosystems. Identifying the interaction of plantation management to vegetation and soil is crucial for developing sustainable plantation ecosystem management strategies. As one of the main measures of close-to-nature management of forest plantation, few studies have paid attention to the effect of crop tree management on the soil properties and understory vegetation. Methods A 36-year-old Pinus massoniana plantation in Huaying city, Sichuan Province was taken as the research object to analyse the changes in undergrowth plant diversity and soil physicochemical properties under three different crop tree densities (100, 150, and 200 N/ha). Results Our results showed that the contents of available phosphorus, organic matter and hydrolysable nitrogen in the topsoil increased significantly after crop tree management, while content of available potassium decreased. The composition of shrub and herb layer was richer, and the dominant species were obviously replaced after crop tree management. The Shannon–Wiener index and Richness index of shrub layer, and the diversity of herb layer increased significantly after crop tree management. Herb layer diversity indexes and Richness index of shrub layer were closely related to soil organic matter, available phosphorus, hydrolysable nitrogen, available potassium, soil moisture and bulk density. As the main limiting factors for plant growth, nitrogen, phosphorus and potassium were closely related to plant diversity and to the distribution of the dominant species. At the initial stage of crop tree management, each treatment significantly improved the soil physicochemical properties and plant diversity of Pinus massoniana plantation, and the comprehensive evaluation was 200 N/ha >100 N/ha >150 N/ha >CK. Compared with other treatments, 200 N/ha had the best effect on improving the undergrowth environment of the Pinus massoniana plantation in the initial stage of crop tree management.
- Published
- 2021
94. Acupuncture Relieves Opioid-Induced Constipation in Clinical Cancer Therapy - A Meta-Analysis and Systematic Review
- Author
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Dehui Li, Na Guo, Huanfang Fan, Yingjuan Liu, and Changhui Han
- Subjects
medicine.medical_specialty ,Abdominal pain ,Constipation ,Epidemiology ,Pain ,Review ,Cochrane Library ,law.invention ,Randomized controlled trial ,law ,Internal medicine ,Acupuncture ,medicine ,cancer ,pain ,Cancer ,business.industry ,medicine.disease ,Opioid-induced constipation ,opioid-induced constipation ,meta-analysis ,Meta-analysis ,Functional constipation ,Defecation ,medicine.symptom ,business ,Cancer pain ,acupuncture - Abstract
Cancer pain is a common problem in clinical cancer therapy. Opioid analgesia is one of the most effective drugs for pain relief with satisfying performance besides the side effect of opioid-induced constipation (OIC). Acupuncture, as a Chinese traditional non-invasive intervention, has been applied to clinical cancer pain management and functional constipation therapy. However, only a few studies have adopted this treatment for OIC patients. Due to limited numbers of investigated subjects and variability of application methods, including treatment apparatus, acupoints, durations, and sessions, the interpretation of acupuncture’s therapy effects from single-site randomized clinical trials (RCT) is limited. Therefore, we conducted a meta-analysis by collecting published data from Pubmed, Embase, Cochrane library, and Web of Science. Five RCTs focusing on the application of acupuncture with or without medication in OIC patients were included. An overall remission rate of 86.8% in the acupuncture-treated group was achieved, higher than the control group (78.9%; RR, 1.10, 95% CI [1.03, 1.18]). The symptom scores, reporting on defecation frequency, defecation straining, abdominal pain, defection time, and stool property, in acupuncture groups were lower than control groups with a standardized mean difference (SMD) of −2.21 [−4.15, −0.27]. The quality of life (QOL) for patients in the acupuncture treated group increased compared to the control group with reduced PAC-QOL scores (SMD, −1.02 [−1.78, −0.26]). Referring to the effects from pure acupuncture treatment (SMD, −0.43 [−0.83, −0.03]), the co-intervention of acupuncture and drugs (SMD, −1.77 [−2.51, −1.02]) improved the life quality of patients more remarkably (P < 0.05). Overall, our data confirmed the therapeutic effects of acupuncture in the treatment of OIC. The co-intervention of acupuncture with drugs improves the outcomes of OIC patients better than a single strategy. Combined therapy with both medicine and acupuncture has insightful potential for future clinical cancer patient management on constipation problems.
- Published
- 2021
95. Linking Holocene East Asian monsoon variability to solar forcing and ENSO activity: Multi-proxy evidence from a peatland in Northeastern China
- Author
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Yong Ge, Honghao Niu, Nathalie Dubois, Nannan Li, Arash Sharifi, Dongmei Jie, Guizai Gao, Guihua Zhang, Lidan Liu, Ying Liu, Jiangyong Wang, Hongyan Liu, Frank M. Chambers, Meng Meng, and Dehui Li
- Subjects
Archeology ,Global and Planetary Change ,GB ,Peat ,GE ,Ecology ,Climate oscillation ,QH ,Paleontology ,Climate change ,Centennial ,Climatology ,East Asian Monsoon ,Environmental science ,Proxy (statistics) ,China ,Holocene ,Earth-Surface Processes - Abstract
High-resolution proxy-based paleoenvironmental records derived from peatlands provide important insights into climate changes over centennial to millennial timescales. In this study, we present a composite climatic index (CCI) for the Hani peatland from northeastern China, based on an innovative combination of pollen-spore, phytolith, and grain size data. We use the CCI to reconstruct variations of the East Asian summer monsoon (EASM) intensity during the Holocene. This is accomplished with complete ensemble empirical mode decomposition (CEEMD), REDFIT, and cross-wavelet coherency analysis to reveal the periodicities (frequencies) of the multi-proxy derived CCI sequences and to assess potential external forcing of the EASM. The results showed that periodicities of ca. 300–350, 475, 600, 1075, and 1875 years were present in the Hani CCI sequence. Those periodicities are consistent with previously published periodicities in East Asia, indicating they are a product of external climate controls over an extensive region, rather than random variations caused by peatland-specific factors. Cross-wavelet coherency analysis between the decomposed CCI components and past solar activity reconstructions suggests that variations of solar irradiation are most likely responsible for the cyclic characteristics at 500-year frequency. We propose a conceptual model to interpret how the sun regulates the monsoon climate via coupling with oceanic and atmospheric circulations. It seems that slight solar irradiation changes can be amplified by coupling with ENSO events, which result in a significant impact on the regional climate in the East Asian monsoon area.
- Published
- 2021
96. Thermally Assisted Rashba Splitting and Circular Photogalvanic Effect in Aqueously Synthesized 2D Dion-Jacobson Perovskite Crystals
- Author
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Rui Chen, Haolin Li, Zeyi Liu, Jiaqi Ma, Boxuan Zhou, Junze Li, Dehui Li, Wancai Li, and Lihan Liang
- Subjects
Materials science ,Photoluminescence ,Condensed matter physics ,Spintronics ,Band gap ,Mechanical Engineering ,Bioengineering ,02 engineering and technology ,General Chemistry ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Ferroelectricity ,Valleytronics ,General Materials Science ,0210 nano-technology ,Spectroscopy ,Rashba effect ,Perovskite (structure) - Abstract
Recently, a two-dimensional Dion-Jacobson (DJ) perovskite (AMP)PbI4 (AMP = 4-(aminomethyl)piperidinium) is emerging with remarkable Rashba effect and ferroelectricity. However, the origin of the giant Rashba splitting remains elusive and the current synthetic strategy via slow cooling is time- and power-consuming, hindering its future applications. Here, we report on an economical aqueous method to obtain (AMP)PbI4 crystals and clarify the origin of the giant Rashba effect by temperature- and polarization-dependent photoluminescence (PL) spectroscopy. The strong temperature-dependent PL helicity indicates the thermally assisted structural distortion as the main origin of the Rashba effect, suggesting that valley polarization still preserves at high temperatures. The Rashba effect was further confirmed by the circular photogalvanic effect near the indirect bandgap. Our study not only optimizes the synthetic strategies of this DJ perovskite but also sheds light on its potential applications in room/high-temperature spintronics and valleytronics.
- Published
- 2021
97. Surface depletion field in 2D perovskite microplates: Structural phase transition, quantum confinement and Stark effect
- Author
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Haizhen Wang, Jun Wang, Hongmei Luo, Chen Fang, Shuai Wang, Wancai Li, Junze Li, Dehui Li, and Jiaqi Ma
- Subjects
Phase transition ,Photoluminescence ,Materials science ,Transition temperature ,02 engineering and technology ,010402 general chemistry ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,01 natural sciences ,Atomic and Molecular Physics, and Optics ,Surface energy ,0104 chemical sciences ,symbols.namesake ,Stark effect ,Depletion region ,Chemical physics ,Phase (matter) ,symbols ,General Materials Science ,Electrical and Electronic Engineering ,0210 nano-technology ,Perovskite (structure) - Abstract
Surface depletion field would introduce the depletion region near surface and thus could significantly alter the optical, electronic and optoelectronic properties of the materials, especially low-dimensional materials. Two-dimensional (2D) organic—inorganic hybrid perovskites with van der Waals bonds in the out-of-plane direction are expected to have less influence from the surface depletion field; nevertheless, studies on this remain elusive. Here we report on how the surface depletion field affects the structural phase transition, quantum confinement and Stark effect in 2D (BA)2PbI4 perovskite microplates by the thickness-, temperature- and power-dependent photoluminescence (PL) spectroscopy. Power dependent PL studies suggest that high-temperature phase (HTP) and low-temperature phase (LTP) can coexist in a wider temperature range depending on the thickness of the 2D perovskite microplates. With the decrease of the microplate thickness, the structural phase transition temperature first gradually decreases and then increases below 25 nm, in striking contrast to the conventional size dependent structural phase transition. Based on the thickness evolution of the emission peaks for both high-temperature phase and low-temperature phase, the anomalous size dependent phase transition could probably be ascribed to the surface depletion field and the surface energy difference between polymorphs. This explanation was further supported by the temperature dependent PL studies of the suspended microplates and encapsulated microplates with graphene and boron nitride flakes. Along with the thickness dependent phase transition, the emission energies of free excitons for both HTP and LTP with thickness can be ascribed to the surface depletion induced confinement and Stark effect.
- Published
- 2019
98. Light-Enhanced Ion Migration in Two-Dimensional Perovskite Single Crystals Revealed in Carbon Nanotubes/Two-Dimensional Perovskite Heterostructure and Its Photomemory Application
- Author
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Yutao Li, Tian-Ling Ren, He Tian, Jun Kang, Lin-Wang Wang, Li Ren, Yi Yang, Ye Tian, Guang-Yang Gou, Zhen-Yi Ju, Jiaqi Ma, Dan Xie, Dehui Li, Lian-Mao Peng, Mengxing Sun, Li Ding, and Junze Li
- Subjects
Materials science ,010405 organic chemistry ,business.industry ,General Chemical Engineering ,Heterojunction ,General Chemistry ,Carrier lifetime ,Dielectric ,Carbon nanotube ,010402 general chemistry ,01 natural sciences ,0104 chemical sciences ,Ion ,law.invention ,Chemistry ,Semiconductor ,law ,Vacancy defect ,Chemical Sciences ,Optoelectronics ,Field-effect transistor ,business ,QD1-999 ,Research Article - Abstract
Two-dimensional (2D) hybrid perovskite sandwiched between two long-chain organic layers is an emerging class of low-cost semiconductor materials with unique optical properties and improved moisture stability. Unlike conventional semiconductors, ion migration in perovskite is a unique phenomenon possibly responsible for long carrier lifetime, current–voltage hysteresis, and low-frequency giant dielectric response. While there are many studies of ion migration in bulk hybrid perovskite, not much is known for its 2D counterparts, especially for ion migration induced by light excitation. Here, we construct an exfoliated 2D perovskite/carbon nanotube (CNT) heterostructure field effect transistor (FET), not only to demonstrate its potential in photomemory applications, but also to study the light induced ion migration mechanisms. We show that the FET I–V characteristic curve can be regulated by light and shows two opposite trends under different CNT oxygen doping conditions. Our temperature-dependent study indicates that the change in the I–V curve is probably caused by ion redistribution in the 2D hybrid perovskite. The first principle calculation shows the reduction of the migration barrier of I vacancy under light excitation. The device simulation shows that the increase of 2D hybrid perovskite dielectric constant (enabled by the increased ion migration) can change the I–V curve in the trends observed experimentally. Finally, the so synthesized FET shows the multilevel photomemory function. Our work shows that not only we could understand the unique ion migration behavior in 2D hybrid perovskite, it might also be used for many future memory function related applications not realizable in traditional semiconductors., A two-dimensional perovskite/carbon nanotube heterostructure was constructed not only to study light induced ion migration mechanisms, but also to demonstrate its potential in photomemory applications.
- Published
- 2019
99. Nonlinear optics of two‐dimensional transition metal dichalcogenides
- Author
-
Zibo Gong, Xinglin Wen, and Dehui Li
- Subjects
NLO modulation and enhancement ,Materials science ,Transition metal ,Condensed matter physics ,lcsh:T58.5-58.64 ,lcsh:Information technology ,nonlinear optics ,transition metal dichalcogenides ,lcsh:TA401-492 ,Nonlinear optics ,High Energy Physics::Experiment ,lcsh:Materials of engineering and construction. Mechanics of materials ,nonlinear devices - Abstract
Nonlinear optics (NLO) of transition metal dichalcogenides (TMDs) is promising for the on‐chip photonic and optoelectronic applications. In this review, we will survey the current progress of NLO in TMDs. First, we will brief the basic theory of the NLO in TMDs. Second, several important nonlinear processes in TMDs such as harmonic generation, four‐wave mixing, saturable absorption, and two‐photon absorption will be presented and their potential applications are also discussed. Third, the main strategies to tune, modulate, and enhance the NLO in TMDs are reviewed, including the excitonic effect, symmetry modulation, optical cavity enhancement, valley selection, edge state, and material phase. Finally, we give an outlook regarding some important issues and directions of NLO in TMDs.
- Published
- 2019
100. Aqueous Synthesis of Low-Dimensional Lead Halide Perovskites for Room-Temperature Circularly Polarized Light Emission and Detection
- Author
-
Chen Fang, Shuai Wang, Jiaqi Ma, Jun Wang, Wancai Li, Long Jin, and Dehui Li
- Subjects
Aqueous solution ,Materials science ,business.industry ,General Engineering ,General Physics and Astronomy ,Halide ,02 engineering and technology ,010402 general chemistry ,021001 nanoscience & nanotechnology ,01 natural sciences ,0104 chemical sciences ,chemistry.chemical_compound ,Semiconductor ,chemistry ,Quantum dot ,Optoelectronics ,Dimethylformamide ,General Materials Science ,0210 nano-technology ,business ,Circular polarization ,Perovskite (structure) - Abstract
Low-dimensional lead halide perovskite materials are an emerging class of solution-processable semiconductors with promising potential applications in optoelectronic devices. Unfortunately, it is impossible to synthesize high-crystalline-quality low-dimensional perovskite single crystals without using chemotoxic solutions such as dimethylformamide/dimethyl sulfoxide or applying heating. Herein we report an economical and universal aqueous method to synthesize 2D layered and 1D chain perovskite single crystals at room temperature. The resultant chiral 2D perovskites can efficiently and selectively emit and detect circularly polarized light at room temperature. The as-synthesized 1D perovskite single crystals exhibit strong quantum confinement and enhanced self-trapped states that give efficient warm circularly polarized white-light emission. This aqueous synthetic method is general for other high-quality low-dimensional lead halide perovskite single crystals, and thus our findings would motivate more fundamental investigations on low-dimensional perovskites for potential optoelectronic applications.
- Published
- 2019
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