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We theoretically study an extension of the Dicke model, where the single-particle Hamiltonian has three energy levels in Lambda-configuration, i.e. the excited state is coupled to two non-degenerate ground states via two independent quantized light fields. The corresponding many-body Hamiltonian can be diagonalized in the thermodynamic limit with the help of a generalized Holstein--Primakoff transformation. Analyzing the ground-state energy and the excitation energies, we identify one normal and two superradiant phases, separated by phase transitions of both first and second order. A phase with both superradiant states coexisting is not stable. In addition, in the limit of two degenerate ground states a dark state emerges, which seems to be analogous to the dark state appearing in the well known stimulated Raman adiabatic passage scheme., 9 pages, 6 figures

We discuss the description of full counting statistics in quantum transport with a nonMarkovian master equation. We focus on differences arising from whether charge is considered as a classical or a quantum degree of freedom. These differences manifest themselves in the inhomogeneous term of the master equation which describes initial correlations. We describe the influence on current and in particular, the finite-frequency shotnoise. We illustrate these ideas by studying transport through a quantum dot and give results that include both sequential and cotunneling processes. Importantly, the noise spectra derived from the classical description are essentially frequency-independent and all quantum noise effects are absent. These effects are fully recovered when charge is considered as a quantum degree of freedom., Comment: 12 pages; 3 figures

We suggest that a single-electron transistor continuously monitored by a quantum point contact may function as Maxwell's demon when closed-loop feedback operations are applied as time-dependent modifications of the tunneling rates across its junctions. The device may induce a current across the single-electron transistor even when no bias voltage or thermal gradient is applied. For different feedback schemes, we derive effective master equations and compare the induced feedback current and its fluctuations as well as the generated power. Provided that tunneling rates can be modified without changing the transistor level, the device may be implemented with current technology.

We establish a set of nonequilibrium quantum phase transitions in the Dicke model by considering a monochromatic nonadiabatic modulation of the atom-field coupling. For weak driving the system exhibits a set of sidebands which allow the circumvention of the no-go theorem which otherwise forbids the occurence of superradiant phase transitions. At strong driving we show that the system exhibits a rich multistable structure and exhibits both first- and second-order nonequilibrium quantum phase transitions., 4 pages, 3 Figures, and supplementary material. This new version contains corrected typos, new references and new versions of the figures. Published by Physical Review Letters

We propose a feedback control scheme for generating and stabilizing pure states of transport devices, such as charge qubits, under non-equilibrium conditions. The purification of the device state is conditioned on single electron jumps and leaves a clear signal in the full counting statistics which can be used to optimize control parameters. As an example of our control scheme, we are presenting the stabilization pure transport states in a double quantum dot setup with the inclusion of phonon dephasing., 7 pages, 5 figures

We propose the manipulation of an isolated qubit by a simple instantaneous closed-loop feedback scheme in which a time-dependent electronic detector current is directly back-coupled into qubit parameters. As specific detector model we employ a capacitively coupled single-electron transistor. We demonstrate the stabilization of pure delocalized qubit states above a critical detector-qubit coupling. This electronic purification is independent of the initial qubit state and is accomplished after few electron jumps through the detector. Our simple scheme can be used for the efficient and robust initialization of solid-state qubits in quantum computational algorithms at arbitrary temperatures., 4 pages, 4 figures, supplementary material, with minor modifications to be published by PRL

We present a theory of finite-frequency noise in non-equilibrium conductors. It is shown that Non-Markovian correlations are essential to describe the physics of quantum noise. In particular, we show the importance of a correct treatment of the initial system-bath correlations, and how these can be calculated using the formalism of quantum master equations. Our method is particularly important in interacting systems, and when the measured frequencies are larger that the temperature and applied voltage. In this regime, quantum-noise steps are expected in the power spectrum due to vacuum fluctuations. This is illustrated in the current noise spectrum of single resonant level model and of a double quantum dot --charge qubit-- attached to electronic reservoirs. Furthermore, the method allows for the calculation of the single-time counting statistics in quantum dots, measured in recent experiments., Comment: 9 Pages, 7 Figures. Published version

We describe a method for calculating the counting statistics of electronic transport through nanoscale devices with both sequential and cotunneling contributions. The method is based upon a perturbative expansion of the von Neumann equation in Liouvillian space, with current cumulants calculated from the resulting nonMarkovian master equation without further approximation. As application, we consider transport through a single quantum dot and discuss the effects of cotunneling on noise and skewness, as well as the properties of various approximation schemes., Comment: 11 pages, 6 figures

We study the transport properties of the Fano-Anderson model with a Lorentzian-shaped density of states in one of the electronic reservoirs. We explicitly show that the energy dependence of the density of states can cause non-Markovian effects and that the non-Markovian master equation may fail if these effects are strong. We evaluate the stationary current, the zero frequency current noise and the occupation dynamics of the resonant level by means of a quantum master equation approach within different approximation schemes and compare the results to the exact solution obtained by scattering theory and Green's functions., 9 pages, 6 figures; due to suggestions of a referee we have added an appendix where our kernel is derived in detail; a few typos are corrected

We consider theoretically the transport through the double quantum dot structure of the recent experiment of C. Payette {\it et al.} [Phys. Rev. Lett. {\bf 102}, 026808 (2009)] and calculate stationary current and shotnoise. Three-level mixing gives rise to a pronounced current suppression effect, the character of which charges markedly with bias direction. We discuss these results in connexion with the dark states of coherent population trapping in quantum dots., Comment: 6 pages, 5 figs

We study the relationship between entanglement and parametric resonance in a system of two coupled time-dependent oscillators. As a measure of bipartite entanglement, we calculate the linear entropy for the reduced density operator, from which we study the entanglement dynamics. In particular, we find that the bipartite entanglement increases in time up to a maximal mixing scenario, when the set of auxiliary dynamical parameters are under parametric resonance. Moreover, we obtain a closed relationship between the correlations in the ground state, the localisation of the Wigner function in phase space, and the localisation of the wave function of the total system., Comment: 10 pages, 5 figures

We present a theory of a single-electron transistor exchange-coupled to a localized spin. We show how to gain detailed quantitative knowledge about the attached spin such as spin size, exchange coupling strength, Land\'e g-factor, and spin decay time $T_1$ by utilizing a robust blockade phenomenon of DC magnetotransport with accompanying noise enhancement. Our studies are of particular relevance to spin-resolved scanning single-electron transistor microscopy, electronic transport through nanomagnets, and the effect of hyperfine interaction on transport electrons by surrounding nuclear spins., Comment: 4 pages, 2 figures, revised version

We study transport through a triple quantum dot in a triangular geometry with applied bias such that both singly- and doubly- charged states participate. We describe the formation of electronic dark states -- coherent superpositions that block current flow -- in the system, and focus on the formation of a two-electron dark state. We discuss the conditions under which such a state forms and describe the signatures that it leaves in transport properties such as the differential conductance and shotnoise., Comment: (9 pages, 7 figures), we now consider two different sets of charging energies

We present an adiabatic approach to the design of entangling quantum operations with two electron spins localized in separate InAs/GaAs quantum dots via the Coulomb interaction between optically-excited localized states. Slowly-varying optical pulses minimize the pulse noise and the relaxation of the excited states. An analytic "dressed state" solution gives a clear physical picture of the entangling process, and a numerical solution is used to investigate the error dynamics. For two vertically-stacked quantum dots we show that, for a broad range of dot parameters, a two-spin state with concurrence $C>0.85$ can be obtained by four optical pulses with durations $\sim 0.1 - 1$ ns., 7 pages, 5 figures

We consider the transport through a system of three coupled quantum dots in a perpendicular magnetic field. At zero field, destructive interference can trap an electron in a dark state -- a coherent superposition of dot states that completely blocks current flow. The magnetic field can disrupt this interference giving rise to oscillations in the current and its higher-order statistics as the field is increased. These oscillations have a period of either the flux-quantum or half the flux-quantum, depending on the dot geometry. We give results for the stationary current and for the shotnoise and skewness at zero and finite frequency., 7 pages, 7 figures

We report the demonstration of fast spin state initialization with near unity efficiency in a singly-charged quantum dot by optically cooling an electron spin.

Quantum computation requires a continuous supply of rapidly initialized qubits for quantum error correction. Here, we demonstrate fast spin state initialization with near unity efficiency in a singly charged quantum dot by optically cooling an electron spin. The electron spin is successfully cooled from 5 to 0.06 K at a magnetic field of 0.88 T applied in Voigt geometry. The spin cooling rate is of order ${10}^{9}\text{ }\text{ }{\mathrm{s}}^{\ensuremath{-}1}$, which is set by the spontaneous decay rate of the excited state.

We present a formalism to calculate finite-frequency current correlations in interacting nanoscale conductors. We work within the n-resolved density matrix approach and obtain a multi-time cumulant generating function that provides the fluctuation statistics, solely from the spectral decomposition of the Liouvillian. We apply the method to the frequency-dependent third cumulant of the current through a single resonant level and through a double quantum dot. Our results, which show that deviations from Poissonian behaviour strongly depend on frequency, demonstrate the importance of finite-frequency higher-order cumulants in fully characterizing interactions., Comment: 4 pages, 2 figures, improved figures & discussion. J-ref added

We present a theory of the optical control of the spin of an electron in an InAs quantum dot. We show how two Raman-detuned laser pulses can be used to obtain arbitrary single-qubit rotations via the excitation of an intermediate trion state. Our theory takes into account a finite in-plane hole $g$-factor and hole-mixing. We show that such rotations can be performed to high fidelities with pulses lasting a few tens of picoseconds., Comment: 6 pages, 4 figures; minor changes, J-ref added

We consider the initialization of the spin-state of a single electron trapped in a self-assembled quantum dot via optical pumping of a trion level. We show that with a magnetic field applied perpendicular to the growth direction of the dot, a near-unity fidelity can be obtained in a time equal to a few times the inverse of the spin-conserving trion relaxation rate. This method is several orders-of-magnitude faster than with the field aligned parallel, since this configuration must rely on a slow hole spin-flip mechanism. This increase in speed does result in a limit on the maximum obtainable fidelity, but we show that for InAs dots, the error is very small., Comment: 4 pages, 4 figures

We propose an experiment to observe coherent oscillations in a single quantum dot with the oscillations driven by spin-orbit interaction. This is achieved without spin-polarised leads, and relies on changing the strength of the spin-orbit coupling via an applied gate pulse. We derive an effective model of this system which is formally equivalent to the Jaynes-Cummings model of quantum optics. For parameters relevant to a InGaAs dot, we calculate a Rabi frequency of 2 GHz., Comment: 4 pages, 3 figures Revised version: additional results included on page 4. Fig 3c replaced accordingly. Numerical error in predicted Rabi frequency corrected

We present a fully electronic analogue of coherent population trapping in quantum optics, based on destructive interference of single-electron tunneling between three quantum dots. A large bias voltage plays the role of the laser illumination. The trapped state is a coherent superposition of the electronic charge in two of these quantum dots, so it is destabilized as a result of decoherence by coupling to external charges. The resulting current I through the device depends on the ratio of the decoherence rate Gamma_phi and the tunneling rates. For Gamma_phi --> 0 one has simply I=e Gamma_phi. With increasing Gamma_phi the current peaks at the inverse trapping time. The direct relation between I and Gamma_phi can serve as a means of measuring the coherence time of a charge qubit in a transport experiment., version 2: added results for unequal tunnel/decoherence rates

We describe a mechanism for the production of polarization-entangled microwaves using intraband transitions in a pair of quantum dots. This proposal relies neither on spin-orbit coupling nor on control over electron-electron interactions. The quantum correlation of microwave polarizations is obtained from orbital degrees of freedom in an external magnetic field. We calculate the concurrence of emitted microwave photon pairs and show that a maximally entangled Bell pair is obtained in the limit of weak interdot coupling.

Building on a previous proposal for the entanglement of electron-hole pairs in the Fermi sea, we show how 3 qubits can be entangled without using electron-electron interactions. As in the 2-qubit case, this electronic scheme works even if the sources are in (local) thermal equilibrium -- in contrast to the photonic analogue. The 3 qubits are represented by 4 edge-channel excitations in the quantum Hall effect (2 hole excitations plus 2 electron excitations with identical channel index). The entangler consists of an adiabatic point contact flanked by a pair of tunneling point contacts. The irreducible 3-qubit entanglement is characterized by the tangle, which is expressed in terms of the transmission matrices of the tunneling point contacts. The maximally entangled Greenberger-Horne-Zeilinger (GHZ) state is obtained for channel-independent tunnel probabilities. We show how low-frequency noise measurements can be used to determine an upper and lower bound to the tangle. The bounds become tighter the closer the electron-hole state is to the GHZ state., 8 pages including 4 figures; [2017: fixed broken postscript figures]

It is known that a quantum computer operating on electron-spin qubits with single-electron Hamiltonians and assisted by single-spin measurements can be simulated efficiently on a classical computer. We show that the exponential speed-up of quantum algorithms is restored if single-charge measurements are added. These enable the construction of a CNOT (controlled NOT) gate for free fermions, using only beam splitters and spin rotations. The gate is nearly deterministic if the charge detector counts the number of electrons in a mode, and fully deterministic if it only measures the parity of that number., Comment: 5 pages including 3 figures

We consider a class of generalised single mode Dicke Hamiltonians with arbitrary boson coupling in the pseudo-spin $x$-$z$ plane. We find exact solutions in the thermodynamic, large-spin limit as a function of the coupling angle, which allows us to continuously move between the simple dephasing and the original Dicke Hamiltonians. Only in the latter case (orthogonal static and fluctuating couplings), does the parity-symmetry induced quantum phase transition occur., Comment: 6 pages, 5 figues

For two qubits in a pure state there exists a one-to-one relation between the entanglement measure (the concurrence ${\cal C}$) and the maximal violation ${\cal M}$ of a Bell inequality. No such relation exists for the three-qubit analogue of ${\cal C}$ (the tangle $\tau$), but we have found that numerical data is consistent with a simple set of upper and lower bounds for $\tau$ given ${\cal M}$. The bounds on $\tau$ become tighter with increasing ${\cal M}$, so they are of practical use. The Svetlichny form of the Bell inequality gives tighter bounds than the Mermin form. We show that the bounds can be tightened further if the tangle is replaced by an entanglement monotone that can identify both the W state and the Greenberger-Horne-Zeilinger state., Comment: 3 pages, 2 figures

We investigate the quantum chaotic properties of the Dicke Hamiltonian; a quantum-optical model which describes a single-mode bosonic field interacting with an ensemble of $N$ two-level atoms. This model exhibits a zero-temperature quantum phase transition in the $N \go \infty$ limit, which we describe exactly in an effective Hamiltonian approach. We then numerically investigate the system at finite $N$ and, by analysing the level statistics, we demonstrate that the system undergoes a transition from quasi-integrability to quantum chaotic, and that this transition is caused by the precursors of the quantum phase-transition. Our considerations of the wavefunction indicate that this is connected with a delocalisation of the system and the emergence of macroscopic coherence. We also derive a semi-classical Dicke model, which exhibits analogues of all the important features of the quantum model, such as the phase transition and the concurrent onset of chaos., 51 pages, 15 figures, latex

We demonstrate theoretically that the shot noise produced by a tunnel barrier in a two-channel conductor violates a Bell inequality. The nonlocality is shown to originate from entangled electron-hole pairs created by tunneling events---without requiring electron-electron interactions. The degree of entanglement (concurrence) equals $2({T}_{1}{T}_{2}{)}^{1/2}({T}_{1}+{T}_{2}{)}^{\ensuremath{-}1}$, with ${T}_{1},{T}_{2}\ensuremath{\ll}1$ the transmission eigenvalues. A pair of edge channels in the quantum Hall effect is proposed as an experimental realization.

The Rabi Hamiltonian describes a single mode of electromagnetic radiation interacting with a two-level atom. Using the coupled cluster method, we investigate the time evolution of this system from an initially empty field mode and an unexcited atom. We give results for the atomic inversion and field occupation, and find that the virtual processes cause the field to be squeezed. No anti-bunching occurs., Comment: 25 pages, 8 figures, RevTex

We present a new method for finding isolated exact solutions of a class of non-adiabatic Hamiltonians of relevance to quantum optics and allied areas. Central to our approach is the use of Bogoliubov transformations of the bosonic fields in the models. We demonstrate the simplicity and efficiency of this method by applying it to the Rabi Hamiltonian., Comment: LaTeX, 16 pages, 1 figure. Minor additions and journal ref

The two-photon Rabi Hamiltonian is a simple model describing the interaction of light with matter, with the interaction being mediated by the exchange of two photons. Although this model is exactly soluble in the rotating-wave approximation, we work with the full Hamiltonian, maintaining the non-integrability of the model. We demonstrate that, despite this non-integrability, there exist isolated, exact solutions for this model analogous to the so-called Juddian solutions found for the single-photon Rabi Hamiltonian. In so doing we use a Bogoliubov transformation of the field mode, as described by the present authors in an earlier publication., 15 Pages, 1 Figure, Latex, minor changes

In contrast to the spatial Bell's inequalities, which probe entanglement between spatially-separated systems, the Leggett-Garg inequalities test the correlations of a single system measured at different times. Violation of a genuine Leggett-Garg test implies either the absence of a realistic description of the system or the impossibility of measuring the system without disturbing it. Quantum mechanics violates the inequalities on both accounts and the original motivation for these inequalities was as a test for quantum coherence in macroscopic systems. The last few years has seen a number of experimental tests and violations of these inequalities in a variety of microscopic systems such as superconducting qubits, nuclear spins, and photons. In this article, we provide an introduction to the Leggett-Garg inequalities and review these latest experimental developments. We discuss important topics such as the significance of the non-invasive measurability assumption, the clumsiness loophole, and the role of weak measurements. Also covered are some recent theoretical proposals for the application of Leggett-Garg inequalities in quantum transport, quantum biology and nano-mechanical systems., Comment: 49 pages; 7 figs

Feedback control in quantum transport has been predicted to give rise to several interesting effects, amongst them quantum state stabilisation and the realisation of a mesoscopic Maxwell's daemon. These results were derived under the assumption that control operations on the system be affected instantaneously after the measurement of electronic jumps through it. In this contribution I describe how to include a delay between detection and control operation in the master equation theory of feedback-controlled quantum transport. I investigate the consequences of delay for the state-stabilisation and Maxwell's-daemon schemes. Furthermore, I describe how delay can be used as a tool to probe coherent oscillations of electrons within a transport system and how this formalism can be used to model finite detector bandwidth., Comment: 13 pages, 5 figures

The mechanism used by migratory birds to orientate themselves using the geomagnetic field is still a mystery in many species. The radical pair mechanism, in which very weak magnetic fields can influence certain types of spin-dependent chemical reactions, leading to biologically observable signals, has recently imposed itself as one of the most promising candidates for certain species. This is thanks both to its extreme sensitivity and its capacity to reproduce results from behavioral studies. Still, in order to gain a directional sensitivity, an anisotropic mechanism is needed. Recent proposals have explored the possibility that such an anisotropy is due to the electron-nucleus hyperfine interaction. In this work we explore a different possibility, in which the anisotropy is due to spin-orbit coupling between the electron spin and its angular momentum. We will show how a spin-orbit-coupling-based magnetic compass can have performances comparable with the usually-studied nuclear-hyperfine based mechanism. Our results could thus help researchers actively looking for candidate biological molecules which may host magnetoreceptive functions, both to describe magnetoreception in birds as well as to develop artificial chemical compass systems., Comment: 9 pages, 3 figures

We investigate the second-order von Neumann approach from a diagrammatic point-of-view and demonstrate its equivalence with the resonant tunneling approximation. Investigation of higher-order diagrams shows that the method correctly reproduces the equation of motion for the single-particle reduced density matrix of an arbitrary non-interacting many-body system. This explains why the method reproduces the current exactly for such systems. We go on to show, however, that diagrams not included in the method are needed to calculate exactly higher cumulants of the charge transport. This thorough comparison sheds light on the validity of all these self consistent second-order approaches. We analyze the discrepancy between the noise calculated by our method and the exact Levitov formula for a simple non-interacting quantum dot model. Furthermore we study the noise of the canyon of current suppression in a two-level dot, a phenomenon that requires the inclusion of electron-electron interaction as well as higher-order tunneling processes., Comment: 27 pages, 14 figures

We propose an all-electronic technique to manipulate and control interacting quantum systems by unitary single-jump feedback conditioned on the outcome of a capacitively coupled electrometer and in particular a single-electron transistor. We provide a general scheme to stabilize pure states in the quantum system and employ an effective Hamiltonian method for the quantum master equation to elaborate on the nature of stabilizable states and the conditions under which state purification can be achieved. The state engineering within the quantum feedback scheme is shown to be linked with the solution of an inverse eigenvalue problem. Two applications of the feedback scheme are presented in detail: (i) stabilization of delocalized pure states in a single charge qubit and (ii) entanglement stabilization in two coupled charge qubits. In the latter example we demonstrate the stabilization of a maximally entangled Bell state for certain detector positions and local feedback operations., 23 pages, 6 figures, to be published by New Journal of Physics (2013)

We present a scheme for creating and measuring entanglement between two double quantum dot charge qubits in a transport set-up in which voltage pulses can modify system parameters. Detection of entanglement is performed via the construction of a Bell inequality with current correlation measurements. An essential feature is the use of the internal dynamics of the qubits as the constituent electrons tunnel into the leads to give the single-particle rotations necessary for the Bell measurement., Comment: 5 pages, 3 figures

We consider the Dicke Hamiltonian, a simple quantum-optical model which exhibits a zero-temperature quantum phase transition. We present numerical results demonstrating that at this transition the system changes from being quasi-integrable to quantum chaotic. By deriving an exact solution in the thermodynamic limit we relate this phenomenon to a localisation-delocalisation transition in which a macroscopic superposition is generated. We also describe the classical analogues of this behaviour., 4 pages, 5 figures, minor changes, Journal ref. added

We classify entanglement singularities for various two-mode bosonic systems in terms of catastrophe theory. Employing an abstract phase-space representation, we obtain exact results in limiting cases for the entropy in cusp, butterfly, and two-dimensional catastrophes. We furthermore use numerical results to extract the scaling of the entropy with the non-linearity parameter, and discuss the role of mixing entropies in more complex systems., 7 pages, 3 figures

We present a formalism for studying the behaviour of quantum systems coupled to nonequilibrium environments exhibiting nonGaussian fluctuations. We discuss the role of a qubit as a detector of the statistics of environmental fluctuations, as well as nonMarkovian effects in both weak and strong coupling limits. We also discuss the differences between the influences of classical and quantum environments. As examples of the application of this formalism we study the dephasing and relaxation of a charge qubit coupled to nonequillibrium electron transport through single and double quantum dots., 12 pages, 7 figures; significantly expanded version

We describe an interaction mechanism between electron spins in a vertically-stacked double quantum dot that can be used for controlled two-qubit operations. This interaction is mediated by excitons confined within, and delocalized over, the double dot. We show that gates equivalent to the SQRT-SWAP gate can be obtained in times much less than the exciton relaxation time and that the negative effects of hole-mixing and spontaneous emission do not seriously affect these results., Comment: 12 pages, 3 figures; expanded for clarity + minor changes, J-ref added

We develop a self-consistent version of perturbation theory in Liouville space which seeks to combine the advantages of master equation approaches in quantum transport with the nonperturbative features that a self-consistent treatment brings. We describe how counting fields may be included in a self-consistent manner in this formalism such that the full counting statistics can be calculated. NonMarkovian effects are also incorporated. Several different self-consistent approximations are introduced and we discuss their relative strengths with a simple example., Comment: 11 pages, 2 figures

We construct a class of algebraic invariants for N-qubit pure states based on bipartite decompositions of the system. We show that they are entanglement monotones, and that they differ from the well know linear entropies of the sub-systems. They therefore capture new information on the non-local properties of multipartite systems., 6 pages

The Rabi Hamiltonian is a simple, yet non-trivial model of light-matter interactions. Here we present a brief review of the application of the normal coupled cluster method (NCCM) to this model. We concentrate on the NCCM description of the excitation spectrum and of simple time evolutions of the system, providing a link between the two that limits the accuracy of NCCM dynamical calculations in practice.