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401. Iron-substituted polyoxotungstates as inorganic synzymes: evidence for a biomimetic pathway in the catalytic oxygenation of catechols.

Author

Sartorel A, Carraro M, Scorrano G, Bassil BS, Dickman MH, Keita B, Nadjo L, Kortz U, and Bonchio M

Subjects
Catalysis, Organometallic Compounds chemistry, Oxidation-Reduction, Protocatechuate-3,4-Dioxygenase chemistry, Catechols chemistry, Iron chemistry, Organometallic Compounds metabolism, Protocatechuate-3,4-Dioxygenase metabolism, Tungsten chemistry
Published
2009
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403. Fast catalytic epoxidation with H(2)O(2) and [gamma-SiW(10)O(36)(PhPO)(2)](4-) in ionic liquids under microwave irradiation.

Author

Berardi S, Bonchio M, Carraro M, Conte V, Sartorel A, and Scorrano G

Abstract

Olefin epoxidation by [gamma-SiW10O36(PhPO)2]4- and H2O2 occurs in hydrophobic ionic liquids (ILs), with yields and selectivity up to >99%. The catalytic IL phase is recyclable. Under MW irradiation the reaction occurs with up to 200 turnovers per minute. Simultaneous cooling is instrumental for quantitative H2O2 conversion.

Published
2007
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