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With the progress in the development of optical frequency standards grows the demand for the dissemination of stable optical frequencies. To date, optical fiber links constitute the most promising medium to bridge large geographical distances while still maintaining a high degree of frequency stability and accuracy. We investigated the transfer of an optical frequency along different fiber links during the past years and achieved a fractional instability and uncertainty at a level lower than 10 − 19 using fiber links with lengths of up to almost 2000 km. We give an overview of different techniques and methods that can be used in combination with optical fiber links to achieve a stable frequency transfer. The results of different fiber links are summarized and an outlook of future links is given. [ABSTRACT FROM AUTHOR]

The far-infrared (FIR) regime is one of the few wavelength ranges where no astronomical data with sub-arcsecond spatial resolution exist yet. Neither of the medium-term satellite projects like SPICA, Millimetron or OST will resolve this malady. For many research areas, however, information at high spatial and spectral resolution in the FIR, taken from atomic fine-structure lines, from highly excited carbon monoxide (CO) and especially from water lines would open the door for transformative science. These demands call for interferometric concepts. We present here first results of our feasibility study IRASSI (Infrared Astronomy Satellite Swarm Interferometry) for an FIR space interferometer. Extending on the principal concept of the previous study ESPRIT, it features heterodyne interferometry within a swarm of five satellite elements. The satellites can drift in and out within a range of several hundred meters, thereby achieving spatial resolutions of <0.1 arcsec over the whole wavelength range of 1–6 THz. Precise knowledge on the baselines will be ensured by metrology methods employing laser-based optical frequency combs, for which preliminary ground-based tests have been designed by members of our study team. We first give a motivation on how the science requirements translate into operational and design parameters for IRASSI. Our consortium has put much emphasis on the navigational aspects of such a free-flying swarm of satellites operating in relatively close vicinity. We hence present work on the formation geometry, the relative dynamics of the swarm, and aspects of our investigation towards attitude estimation. Furthermore, we discuss issues regarding the real-time capability of the autonomous relative positioning system, which is an important aspect for IRASSI where, due to the large raw data rates expected, the interferometric correlation has to be done onboard, in quasi-real-time. We also address questions regarding the spacecraft architecture and how a first thermomechanical model is used to study the effect of thermal perturbations on the spacecraft. This will have implications for the necessary internal calibration of the local tie between the laser metrology and the phase centres of the science signals and will ultimately affect the accuracy of the baseline estimations. [ABSTRACT FROM AUTHOR]

We present an echelle spectrograph that is optimized for characterization of frequency combs for astronomical applications (astro-combs). In spite of its very compact and cost-efficient design, it allows viewing the spectrum of a frequency comb in nearly the same way as a full-sized high-resolution echelle spectrograph as used at astronomical observatories. This is of great value for testing and characterizing astro-combs during their assembly phase. The spectrograph can further be utilized to effectfully demonstrate the remarkable capabilities of astro-combs. [ABSTRACT FROM AUTHOR]

We report on a novel architecture for robust mode-locked femtosecond fiber lasers using a nonlinear optical loop mirror with all polarization-maintaining fibers. Due to a nonreciprocal phase shift, the loop mirror can be operated in a compact and efficient reflection mode, offering the possibility to reach high repetition rates and easy implementation of tuning elements. In particular, longitudinal mode spacing and carrier-envelope offset frequency may be controlled in order to operate the laser as an optical frequency comb. We demonstrate femtosecond pulse generation at three different wavelengths (1030, 1565, and 2050 nm) using Ytterbium, Erbium, and co-doped Thulium-Holmium as gain media, respectively. Robust operation is achieved for a wide range of parameters, including repetition rates from 10 to 250 MHz. [ABSTRACT FROM AUTHOR]

Abstract: The interest in new test methods for rubber production has been growing rapidly over the past years. Recent developments in production planning aim to minimize storage times, and hence limit the time available for process control between production steps. New additives such as silica and carbon nanotubes allow for significant improvements in the material quality. Both developments demand new approaches to control the production process where established methods do not work satisfactorily. In this study, we have investigated the capability of terahertz time-domain spectroscopy as a new tool for rubber production testing. Offline measurements of different material families show a strong contrast in the terahertz refractive index. Inline measurements during elastomer extrusion allow for monitoring production processes and the duration of purposely induced material changes in the extruder. This technique helps to improve the quality of the materials and to minimize waste. [Copyright &y& Elsevier]

We have measured the frequency of the extremely narrow 15-25 two-photon transition in atomic hydrogen using a remote cesium fountain clock with the help of a 920 km stabilized optical fiber. With an improved detection method we obtain fls-2s = 2466061413 187018 (11) Hz with a relative uncertainty of 4.5 × 10-15, confirming our previous measurement obtained with a local cesium clock [C. G. Parthey et al, Phys. Rev. Lett. 107, 203001 (2011)]. Combining these results with older measurements, we constrain the linear combinations of Lorentz boost symmetry violation parameters C(TX) = (3.1 ±1.9) × 10-11 and 0.92c(7T) + 0.40c(rz) = (2.6 ±5.3) × 10-11 in the standard model extension framework [D. Colladay, V. A. Kostelecky, Phys. Rev. D. 58, 116002 (1998)]. [ABSTRACT FROM AUTHOR]

We have measured the 1S-2S transition frequency in atomic hydrogen via two-photon spectroscopy on a 5.8 K atomic beam. We obtain f1S-2S = 2466061 413 187 035 (10) Hz for the hyperfine centroid, in agreement with, but 3.3 times better than the previous result [M. Fischer et al., Phys. Rev. Lett. 92, 230802 (2004)]. The improvement to a fractional frequency uncertainty of 4.2 x 10-15 arises mainly from an improved stability of the spectroscopy laser, and a better determination of the main systematic uncertainties, namely, the second order Doppler and ac and dc Stark shifts. The probe laser frequency was phase coherently linked to the mobile cesium fountain clock FOM via a frequency comb. [ABSTRACT FROM AUTHOR]

We report on the first deployment of a ytterbium (Yb) transportable optical lattice clock (TOLC), commercially shipping the clock 3000 km from Boulder, Colorado, to Washington DC. The system, composed of a rigidly mounted optical reference cavity, an atomic physics package, and an optical frequency comb, fully realizes an independent frequency standard for comparisons in the optical and microwave domains. The shipped Yb TOLC was fully operational within 2 days of arrival, enabling frequency comparison with a rubidium (Rb) fountain at the United States Naval Observatory (USNO). To the best of our knowledge, this represents the first deployment of a fully independent TOLC, including the frequency comb, coherently uniting the optical stability of the Yb TOLC to the microwave output of the Rb fountain.

Controlled charge flows are fundamental to many areas of science and technology, serving as carriers of energy and information, as probes of material properties and dynamics 1 and as a means of revealing 2,3 or even inducing 4,5 broken symmetries. Emerging methods for light-based current control 5-16 offer particularly promising routes beyond the speed and adaptability limitations of conventional voltage-driven systems. However, optical generation and manipulation of currents at nanometre spatial scales remains a basic challenge and a crucial step towards scalable optoelectronic systems for microelectronics and information science. Here we introduce vectorial optoelectronic metasurfaces in which ultrafast light pulses induce local directional charge flows around symmetry-broken plasmonic nanostructures, with tunable responses and arbitrary patterning down to subdiffractive nanometre scales. Local symmetries and vectorial currents are revealed by polarization-dependent and wavelength-sensitive electrical readout and terahertz (THz) emission, whereas spatially tailored global currents are demonstrated in the direct generation of elusive broadband THz vector beams 17 . We show that, in graphene, a detailed interplay between electrodynamic, thermodynamic and hydrodynamic degrees of freedom gives rise to rapidly evolving nanoscale driving forces and charge flows under the extremely spatially and temporally localized excitation. These results set the stage for versatile patterning and optical control over nanoscale currents in materials diagnostics, THz spectroscopies, nanomagnetism and ultrafast information processing., (© 2024. The Author(s).)

Mid-infrared frequency combs are nowadays well-appreciated sources for spectroscopy and frequency metrology. Here, a comprehensive approach for characterizing a difference-frequency-generated mid-infrared frequency comb (DFG-comb) both in the time and in the frequency domain is presented. An autocorrelation scheme exploiting mid-infrared two-photon detection is used for characterizing the pulse width and to verify the optimal compression of the generated pulses reaching a pulse duration (FWHM) as low as 196 fs. A second scheme based on mid-infrared heterodyne detection employing two independent narrow-linewidth quantum cascade lasers (QCLs) is used for frequency-narrowing the modes of the DFG-comb down to 9.4 kHz on a 5-ms timescale.

Frequency comb synthesized microwaves have been so far realized with tabletop systems, operated in well-controlled environments. Here, we demonstrate state-of-the-art ultrastable microwave synthesis with a compact rack-mountable apparatus. We present absolute phase noise characterization of a 12 GHz signal using an ultrastable laser at $\sim{194}\;{\rm THz}$∼194THz and an Er:fiber comb divider, obtaining $ - {83}\;{\rm dBc/Hz}$-83dBc/Hz at 1 Hz and $ \lt - {166}\;{\rm dBc/Hz}$<-166dBc/Hz for offsets greater than 5 kHz. Employing semiconductor coating mirrors for the same type of transportable optical frequency reference, we show that $ - {105}\;{\rm dBc/Hz}$-105dBc/Hz at 1 Hz is supported by demonstrating a residual noise limit of division and detection process of $ - {115}\;{\rm dBc/Hz}$-115dBc/Hz at 1 Hz. This level of fidelity paves the way for the deployment of ultrastable photonic microwave oscillators and for operating transportable optical clocks.

We report the measurement of the frequency noise power spectral density (PSD) of a Terahertz (THz) molecular laser (ML) pumped by a mid-infrared (MIR) quantum cascade laser (QCL), and emitting 1 mW at 1.1THz in continuous wave. This is achieved by beating the ML frequency with the 1080 th harmonic of the repetition rate of a 1560 nm frequency comb (FC). We find a frequency noise PSD < 10Hz 2 /Hz (-95dBc/Hz) at 100kHz from the carrier. To demonstrate the effect of the stability of the pump laser on the spectral purity of the THz emission we also measure the frequency noise PSD of a CO 2 -laser-pumped 2.5THz ML, reaching 0.1Hz 2 /Hz (-105dBc/Hz) at 40kHz from the carrier, limited by the frequency noise of the FC harmonic. Finally, we show that it is possible to actively phase-lock the QCL-pumped molecular laser to the FC repetition rate harmonic by controlling the QCL current, demonstrating a sub-Hz linewidth.

Attosecond spectroscopy and precision frequency metrology depend on the stabilization of the carrier-envelope phase (CEP) of mode-locked lasers. Unfortunately, the phase of only a few types of lasers can be stabilized to jitters in the few-hundred millirad range. In a comparative experimental study, we analyze a femtosecond Ti:sapphire laser and three mode-locked fiber lasers. We numerically demodulate recorded time series of the free-running carrier-envelope beat note. Our analysis indicates a correlation between amplitude and frequency fluctuations at low Fourier frequencies for essentially all lasers investigated. While this correlation typically rolls off at frequencies beyond 100 kHz, we see clear indications for a broadband coupling mechanism in one of the fiber lasers. We suspect that the observed coupling mechanism acts to transfer intracavity power fluctuations into excess phase noise. This coupling mechanism is related to the mode-locking mechanism employed and not to the gain medium itself. We further verify this hypothesis by numerical simulations, which identify resonances of the saturable absorber mirror as a possible explanation for the coupling mechanism. Finally, we discuss how to avoid a detrimental influence of such resonances.

We report on the parametric generation of 100 fs sub-6-cycle 40 μJ pulses with the center wavelength at 5.2 μm using a 1 ps 2.1 μm pump laser and a dispersion management scheme based on bulk material. Our optically synchronized amplifier chain consists of a Ho:YAG chirped-pulse amplifier and white-light-seeded optical parametric amplifiers providing simultaneous passive carrier-envelope phase locking of three ultrashort longwave pulses at the pump, signal, and idler wavelengths corresponding, respectively, to 2.1, 3.5, and 5.2 μm. We also demonstrate bandwidth enhancement and efficient control over nonlinear spectral phase in the regime of cascaded χ 2 nonlinearity in ZnGeP 2 .

We have explored the performance of 2 "dark fibers" of a commercial telecommunication fiber link for a remote comparison of optical clocks. These fibers establish a network in Germany that will eventually link optical frequency standards at PTB with those at the Institute of Quantum Optics (IQ) at the Leibniz University of Hanover, and the Max Planck Institutes in Erlangen (MPL) and Garching (MPQ). We demonstrate for the first time that within several minutes a phase coherent comparison of clock lasers at the few 10(-15) level can also be accomplished when the lasers are more than 100 km apart. Based on the performance of the fiber link to the IQ, we estimate the expected stability for the link from PTB to MPQ via MPL that bridges a distance of approximately 900 km.