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The BCS theory has achieved widespread success in describing conventional superconductivity. However, when the length scale reaches the atomic limit, the reduced dimensionality may lead to the quantum breakdown resulting in unpredictable superconducting behaviors. It has been exper imentally evidenced that the critical temperature is strongly enhanced in the monolayer films of FeSe/STO and epitaxial Aluminum. Here, we propose the exciton mechanism of superconductivity as a possible reason for the enhanced superconductivity in hybrid superconductor-semiconductor structures. The exciton-induced Cooper pairing may lead to the larger energy gaps and higher critical temperatures as compared to those caused by the phonon induced superconductivity. A detailed comparison of the theory and experimental results of Ref. 1 reveals the possibility of exciton-induced superconductivity in thin films of Aluminum near the monolayer limit.

The experimental results hinting at the room temperature and ambient pressure superconductivity and magnetic levitation in LK-99 attracted an unprecedented interest. While attempts of other teams to reproduce the reported observations on similar samples failed so far, it seems worthwhile to try building a theoretical model that would explain the ensemble of the available data. One of important features that needs to be explained is an apparent contradiction between an extremely high critical temperature Tc and rather modest critical magnetic field Bc and critical current jc reported for LK-99. We show theoretically, that these data may be quantitatively reproduced assuming the interplay between exciton- and phonon-induced superconductivity, while the conventional BCS or Brinkman-Rice-Bardeen-Cooper-Schriefer (BR-BCS) mechanisms would result in a much higher Bc for the same Tc., Comment: Accepted for publication in Materials Today Communications

We consider bosonic condensates of exciton-polaritons optically confined in elliptical traps. A superposition of two non-degenerated \textit{p}-type states of the condensate oriented along the two main axes of the trap is represented by a point on a Bloch sphere, being considered as an optically tunable qubit. We describe a set of universal single-qubit gates resulting in a controllable shift of the Bloch vector by means of an auxiliary laser beam. Moreover, we consider interaction mechanisms between two neighboring traps that enable designing two-qubit operations such as CPHASE, \textit{i}SWAP, and CNOT gates. Both the single- and two-qubit gates are analyzed in the presence of error sources in the context of polariton traps, such as pure dephasing and spontaneous relaxation mechanisms, leading to a fidelity reduction of the final qubit states and quantum concurrence, as well as the increase of Von Neumann entropy. We also discuss the applicability of our qubit proposal in the context of DiVincenzo's criteria for the realization of local quantum computing processes. Altogether, the developed set of quantum operations would pave the way to the realization of a variety of quantum algorithms in a planar microcavity with a set of optically induced elliptical traps.

We take advantage of the polariton bistability in semiconductor microcavities to estimate the interaction strength between lower exciton-polariton and dark exciton states. We combine the quasiresonant excitation of polaritons and the nominally forbidden two-photon excitation (TPE) of dark excitons in a GaAs microcavity. To this end, we use an ultranarrow linewidth cw laser for the TPE process that allows us to determine the energy of dark excitons with high spectral resolution. Our results evidence a sharp drop in the polariton transmission intensity and width of the hysteresis cycle when the TPE process is resonant with the dark exciton energy, highly compromising the bistability of the polariton condensate. This behavior demonstrates the existence of a small symmetry breaking such as that produced by an effective in-plane magnetic field, allowing us to directly excite the dark reservoir. We numerically reproduce the collapse of the hysteresis cycle with the increasing dark exciton population, treating the evolution of a polariton condensate in a one-mode approximation, coupled to the exciton reservoir via polariton-exciton scattering processes., Comment: 9 pages, 4 figures

Spin or valley degrees of freedom in condensed matter have been proposed as efficient information carriers towards next generation spintronics. It is therefore crucial to develop effective strategies to generate and control spin or valley-locked spin currents, e.g., by exploiting the spin Hall or valley Hall effects. However, the scattering, and rapid dephasing of electrons pose major challenges to achieve macroscopic coherent spin currents and realistic spintronic or valleytronic devices, specifically at room temperature, where strong thermal fluctuations could further obscure the spin flow. Exciton polaritons in semiconductor microcavities being the quantum superposition of excitons and photons, are believed to be promising platforms for spin-dependent optoelectronic or, in short, spin-optronic devices. Long-range spin current flows of exciton polaritons may be controlled through the optical spin Hall effect. However, this effect could neither be unequivocally observed at room temperature nor be exploited for realistic polariton spintronic devices due to the presence of strong thermal fluctuations or large linear spin splittings. Here, we report the observation of room temperature optical spin Hall effect of exciton polaritons with the spin current flow over a distance as large as 60 um in a hybrid organic-inorganic FAPbBr3 perovskite microcavity. We show direct evidence of the long-range coherence at room temperature in the flow of exciton polaritons, and the spin current carried by them. By harnessing the long-range spin-Hall transport of exciton polaritons, we have demonstrated two novel room temperature polaritonic devices, namely the NOT gate and the spin-polarized beam splitter, advancing the frontier of room-temperature polaritonics in perovskite microcavities., Comment: 21 pages, 5 figures

Bosonic condensates of spin-less non-interacting particles confined on a ring cannot propagate circular periodic currents once rotation symmetry of the system is broken. However a persistent current may appear due to inter-particle interactions exceeding some critical strength. In this up-critical regime breaking of the symmetry between the clockwise and anticlockwise rotations takes place. We consider this symmetry-breaking scenario in the case of a spinor condensate of exciton polaritons trapped on a ring split by a potential barrier. Due to the intrinsic symmetry of the effective spin-orbit interaction which stems from the linear splitting between transverse-electric and transverse-magnetic microcavity modes, the potential barrier blocks the circulating current and imposes linear polarization patterns. On the other hand, circularly polarized polaritons form circular currents propagating in opposite directions with equal absolute values of angular momentum. In the presence of inter-particle interactions, the symmetry of clockwise and anticlockwise currents can be broken spontaneously. We describe several symmetry-breaking scenarios which imply either restoration of the global condensate rotation or the onset of the circular polarization in the symmetry-broken state., Comment: 9 pages, 5 figures

We observed a light-induced enhancement of the tunneling current propagating through an array of parallel carbon chains anchored between gold nanoparticles (NPs). In the presence of laser radiation characterized by a wavelength close to the plasmon resonance of the NPs, the current-voltage characteristics of carbon bundle tunnelling junctions demonstrate a pronounced asymmetry between positive and negative bias values. Such an asymmetry is typical for a Schottky junction, in general. The resistance of the tunnel junction decreases with the increase of the optical pumping intensity. We associate the observed effect with an injection of `hot' carriers created in Au NPs due to the decay of the surface plasmons accompanied by the charge transfer to the carbon bundles. The observed phenomenon can be used for non-resonant excitation of excitonic states in low-dimensional carbon-based structures for single-photon emission, as well as for photovoltaic applications., Comment: 8 pages, 2 figures

Concentric ring exciton polariton condensates emerging under non-resonant laser pump in an annular trapping potential support persistent circular currents of polaritons. The trapping potential is formed by a cylindrical micropillar etched in a semiconductor microcavity with embedded quantum wells and a repulsive cloud of optically excited excitons under the pump spot. The symmetry of the potential is subject to external control via manipulation by its pump-induced component. In the manuscript, we demonstrate excitation of concentric ring polariton current states with predetermined vorticity which we trace using interferometry measurements with a spherical reference wave. We also observe the polariton condensate dynamically changing its vorticity during observation, which results in pairs of fork-like dislocations on the time-averaged interferogram coexisting with azimuthally homogeneous photoluminescence distribution in the micropillar.

We study formation of superfluid currents of exciton polaritons in annular polariton condensates in a cylindrical micropillar cavity under the spatially localised nonresonant optical pumping. Since polariton condensates are strongly nonequilibrium systems, the trapping potential for polaritons, formed by the pillar edge and the reservoir of optically induced incoherent excitons, is complex in general case. Its imaginary part includes the spatially distributed gain from the pump and losses of polaritons in the condensate. We show that engineering the gain-loss balance in the micropillar plane gives access to the excited states of the polariton condensate. We demonstrate both theoretically and experimentally formation of vortices in double concentric ring polariton condensates in the complex annular trap potential.

We keep track of the orbital degree of freedom of an exciton polariton condensate, confined in an optical trap, and reveal the stochastic switching of persistent annular polariton currents in the pulse-periodic excitation regime.In an elliptic trap, the low-lying in energy polariton current states are inherent in a two-petalled density distribution and swirling phase. In the stochastic regime, the averaged over multiple excitation pulses density distribution gets homogenised in the azimuthal direction, while the weighted phase extracted from interference experiments experiences two compensating each other jumps, when varying around the center of the trap. Breaking the reciprocity of the system with a supplemental control optical pulse makes it possible to switch the system from the stochastic regime to the deterministic regime of an arbitrary polariton circulation.

It is now routine to make Bose-Einstein condensates of polaritons with long enough lifetime and low enough disorder to travel ballistically for hundreds of microns in quasi-one-dimensional (1D) wires. We present observations of a polariton condensate injected at one point in a quasi-1D ring, with a well-defined initial velocity and direction. A clear precession of the circular polarization is seen, which arises from an effective spin-orbit coupling term in the Hamiltonian. Our theoretical model accurately predicts the experimentally observed behavior, and shows that "zitterbewegung" behavior plays a role in the motion of the polaritons., Comment: accepted by Phys. Rev. B

Recently, split-ring bosonic condensates of exciton polaritons have been proposed for realisation of qubits. We formulate an analytical model of a polariton condensate in a one-dimensional ring split by a delta-function potential. The persistent current is stopped by the potential defect embedded in a scalar condensate of non-interacting particles, however, it reappears in the presence of an up-critical non-linearity. The nonlinear supercurrents are characterised by fractional orbital momenta while their eigenfunctions may feature grey or dark solitons. The coupling between the spin and the orbital angular momentum of a spinor condensate affects persistent currents crucially. We show that the spin-orbit interaction (SOI) induces the net superfluid current in the condensate with a spatially uniform spin polarisation. We also find solutions where the SOI-induced currents of two spin components of the condensate propagate in opposite directions. The corresponding states of spinor condensates obey a combined mirror reflection and the spin-flip symmetry.

Whispering gallery modes in a microwire are characterized by a nearly equidistant energy spectrum. In the strong exciton-photon coupling regime, this system represents a bosonic cascade: a ladder of discrete energy levels that sustains stimulated transitions between neighboring steps. In this work, by using femtosecond angle-resolved spectroscopic imaging technique, the ultrafast dynamics of polaritons in a bosonic cascade based on a one-dimensional ZnO whispering gallery microcavity is explicitly visualized. Clear ladder-form build-up process from higher to lower energy branches of the polariton condensates are observed, which are well reproduced by modeling using rate equations. Moreover, the polariton parametric scattering dynamics are distinguished on a timescale of hundreds of femtoseconds. Our understanding of the femtosecond condensation and scattering dynamics paves the way towards ultrafast coherent control of polaritons at room temperature, which will make it promising for high-speed all-optical integrated applications.

We report on the fabrication of fractal dendrites by laser induced melting of aluminum alloys. We target boron carbide (B4C) that is one of the most effective radiation-absorbing materials which is characterised by a low coefficient of thermal expansion. Due to the high fragility of B4C crystals we were able to introduce its nanoparticles into a stabilization aluminum matrix of AA385.0. The high intensity laser field action led to the formation of composite dendrite structures under the effect of local surface melting. The modelling of the dendrite cluster growth confirms its fractal nature and sheds light on the pattern behavior of the resulting quasicrystal structure., Comment: 8 pages, 3 figures

The emergence of spatial and temporal coherence of light emitted from solid-state systems is a fundamental phenomenon, rooting in a plethora of microscopic processes. It is intrinsically aligned with the control of light-matter coupling, and canonical for laser oscillation. However, it also emerges in the superradiance of multiple, phase-locked emitters, and more recently, coherence and long-range order have been investigated in bosonic condensates of thermalized light, as well as in exciton-polaritons driven to a ground state via stimulated scattering. Here, we experimentally show that the interaction between photons in a Fabry-Perot microcavity and excitons in an atomically thin WSe$_2$ layer is sufficient such that the system enters the hybridized regime of strong light-matter coupling at ambient conditions. Via Michelson interferometry, we capture clear evidence of increased spatial and temporal coherence of the emitted light from the spatially confined system ground-state. The coherence build-up is accompanied by a threshold-like behaviour of the emitted light intensity, which is a fingerprint of a polariton laser effect. Valley-physics is manifested in the presence of an external magnetic field, which allows us to manipulate K and K' polaritons via the Valley-Zeeman-effect. Our findings are of high application relevance, as they confirm the possibility to use atomically thin crystals as simple and versatile components of coherent light-sources, and in valleytronic applications at room temperature., Comment: 13 pages, 4 figures

We reveal a topologically protected persistent oscillatory dynamics of a polariton superfluid, which is driven non-resonantly by a super-Gaussian laser beam in a planar semiconductor microcavity subjected to an external C-shape potential. We find persistent oscillations, characterized by a topological attractor, that are based on the dynamical behavior of small Josephson vortices rotating around the outside edge of the central vortex. The attractor is being formed due to the inverse energy cascade accompanied by the growth of the incompressible kinetic energy. The attractor displays a remarkable stability towards perturbations and it may be tuned by the pump laser intensity to two distinct frequency ranges: 20.16$\pm$0.14 GHz and 48.4$\pm$1.2 GHz. This attractor is bistable due to the chirality of the vortex. The switching between two stable states is achieved by altering the pump power or by adding an extra incoherent Gaussian pump beam.

Linear carbon-based materials such as polyyne and cumulene oligomers provide a versatile platform for nano-physics and engineering. Direct gap quasi-1D polyyne structures are promising for the observation of strong and unusual excitonic eects arising due to the two-dimensional quantum connement. Recently, we reported on the observation of sharp exciton peaks in low temperature photoluminescence spectra of polyyne chains. Here, we analyse the time-resolved optical response of this system. We extend the non-local dielectric response theory to predict the exciton radiative lifetime dependence on the band-gap value and on the length of the chain. A good agreement between the experiment and the theory is achieved., Comment: 4 pages, 4 figures

The emergence of two-dimensional crystals has revolutionized modern solid-state physics. From a fundamental point of view, the enhancement of charge carrier correlations has sparked enormous research activities in the transport- and quantum optics communities. One of the most intriguing effects, in this regard, is the bosonic condensation and spontaneous coherence of many-particle complexes. Here, we find compelling evidence of bosonic condensation of exciton-polaritons emerging from an atomically thin crystal of MoSe2 embedded in a dielectric microcavity under optical pumping. The formation of the condensate manifests itself in a sudden increase of luminescence intensity in a threshold-like manner, and a significant spin-polarizability in an externally applied magnetic field. Spatial coherence is mapped out via highly resolved real-space interferometry, revealing a spatially extended condensate. Our device represents a decisive step towards the implementation of coherent light-sources based on atomically thin crystals, as well as non-linear, valleytronic coherent devices., Comment: Main text: 11 pages, 5 figures, Supplementary Materials: 4 pages, 5 figures

We model generation of vortex modes in exciton-polariton condensates in semiconductor micropillars, arranged into a hexagonal ring molecule, in the presence of TE-TM splitting. This splitting lifts the degeneracy of azimuthally modulated vortex modes with opposite topological charges supported by this structure, so that a number of non-degenerate vortex states characterized by different combinations of topological charges in two polarization components appears. We present a full bifurcation picture for such vortex modes and show that because they have different energies, they can be selectively excited by coherent pump beams with specific frequencies and spatial configurations. At high pumping intensity, polariton-polariton interactions give rise to the coupling of different vortex resonances and a bistable regime is achieved.

Strong spin-orbit coupling and inversion symmetry breaking in transition metal dichalcogenide monolayers yield the intriguing effects of valley-dependent optical selection rules. As such, it is possible to substantially polarize valley excitons with chiral light and furthermore create coherent superpositions of K and K- polarized states. Yet, at ambient conditions dephasing usually becomes too dominant, and valley coherence typically is not observable. Here, we demonstrate that valley coherence is, however, clearly observable for a single monolayer of WSe2, if it is strongly coupled to the optical mode of a high quality factor microcavity. The azimuthal vector, representing the phase of the valley coherent superposition, can be directly manipulated by applying magnetic fields, and furthermore, it sensibly reacts to the polarization anisotropy of the cavity which represents an artificial magnetic field. Our results are in qualitative and quantitative agreement with our model based on pseudospin rate equations, accounting for both effects of real and pseudo-magnetic fields., Comment: 12 Pages, 5 Figures

Recently, we have experimentally observed signatures of sharp exciton peaks in the photoluminescence spectra of bundles of monoatomic carbon chains stabilized by gold nanoparticles and deposited on a glass substrate. Here, we estimate the characteristic energies of excitonic transitions in this complex quasi-one-dimensional nano-system with use of the variational method. We show that the characteristic energy scale for the experimentally observed excitonic fine structure is governed by the interplay between the hopping energy in a Van der Waals quasicrystal formed by parallel carbon chains, the neutral-charged exciton splitting and the positive-negative trion splitting. These three characteristic energies are an order of magnitude lower than the direct exciton binding energy., Comment: 6 pages, 3 figures

We exploit the recent proposals for the light-induced superconductivity mediated by a Bose-Einstein condensate of exciton-polaritons to design a superconducting fiber that would enable long-distance transport of a supercurrent at elevated temperatures. The proposed fiber consists of a conventional core made of a silica glass with the first cladding layer formed by a material sustaining dipole-polarised excitons with a binding energy exceeding 25 meV. To be specific, we consider a perovskite cladding layer of 20 nm width. The second cladding layer is made of a conventional superconductor such as aluminium. The fiber is covered by a conventional coating buffer and by a plastic outer jacket. We argue that the critical temperature for a superconducting phase transition in the second cladding layer may be strongly enhanced due to the coupling of the superconductor to a bosonic condensate of exciton-polaritons optically induced by the evanescent part of the guiding mode confined in the core. The guided light mode would penetrate to the first cladding layer and provide the strong exciton-photon coupling regime. We run simulations that confirm the validity of the proposed concept. The fabrication of superconducting fibers where a high-temperature superconductivity could be controlled by light would enable passing superconducting currents over extremely long distances.

We stabilize monoatomic carbon chains in water by attaching them to gold nanoparticles (NPs) by means of the laser ablation process. Resulting nanoobjects represent pairs of NPs connected by multiple straight carbon chains of several nanometer lengths. If NPs at the opposite ends of a chain differ in size, the structure acquires a dipole moment due to the difference in work functions of the two NPs. We take advantage of the dipole polarisation of carbon chains for ordering them by the external electric field. We deposit them on a glass substrate by the sputtering method in the presence of static electric fields of magnitudes up to 10^5 V/m. The formation of one-dimensional carbyne quasi-crystals deposited on a substrate is evidenced by high-resolution TEM and X-ray diffraction measurements. The original kinetic model describing the dynamics of ballistically flowing nano-dipoles reproduces the experimental diagram of orientation of the deposited chains., Comment: 15 pages, 7 figures

We studied monoatomic linear carbon chains stabilised by gold nanoparticles attached to their ends and deposited on a solid substrate. We observe spectral features of straight chains containing from 8 to 24 atoms. Low temperature PL spectra reveal characteristic triplet fine-structures that repeat themselves for carbon chains of different lengths. The triplet is invariably composed of a sharp intense peak accompanied by two broader satellites situated 15 and 40 meV below the main peak. We interpret these resonances as an edge-state neutral exciton, positively and negatively charged trions, respectively. The time-resolved PL shows that the radiative lifetime of the observed quasiparticles is about 1 ns, and it increases with the increase of the length of the chain. At high temperatures a non-radiative exciton decay channel appears due to the thermal hopping of carriers between parallel carbon chains. Excitons in carbon chains possess large oscillator strengths and extremely low inhomogeneous broadenings., Comment: 23 pages, 5 figures

Superposition states of circular currents of exciton-polaritons mimic the superconducting flux qubits. The phase of a polariton fluid must change by an integer number of $2\pi$, when going around the ring. If one introduces a ${\pi}$-phase delay line in the ring, the fluid is obliged to propagate a clockwise or anticlockwise circular current to reduce the total phase gained over one round-trip to zero or to build it up to $2\pi$. We show that such a $\pi$-delay line can be provided by a dark soliton pinned to a potential well created by a C-shape non-resonant pump-spot. The resulting split-ring polariton condensates exhibit pronounced coherent oscillations passing periodically through clockwise and anticlockwise current states. These oscillations may persist far beyond the coherence time of polariton condensates. The qubits based on split-ring polariton condensates are expected to possess very high figures of merit that makes them a valuable alternative to superconducting qubits. The use of the dipole-polarized polaritons allows to control coherently the state of the qubit with the external electric field. This is shown to be one of the tools for realization of single-qubit logic operations. We propose the design of an $i$SWAP gate based on a pair of coupled polariton qubits. To demonstrate the capacity of the polariton platform for quantum computations, we propose a protocol for the realization of the Deutsch's algorithm with polariton qubit networks., Comment: 18 pages, 15 figures

Spin-orbit coupling is a fundamental mechanism that connects the spin of a charge carrier with its momentum. Likewise, in the optical domain, a synthetic spin-orbit coupling is accessible, for instance, by engineering optical anisotropies in photonic materials. Both, akin, yield the possibility to create devices directly harnessing spin- and polarization as information carriers. Atomically thin layers of transition metal dichalcogenides provide a new material platform which promises intrinsic spin-valley Hall features both for free carriers, two-particle excitations (excitons), as well as for photons. In such materials, the spin of an exciton is closely linked to the high-symmetry point in reciprocal space it emerges from. Here, we demonstrate, that spin, and hence valley selective propagation is accessible in an atomically thin layer of MoSe2, which is strongly coupled to a microcavity photon mode. We engineer a wire-like device, where we can clearly trace the flow, and the helicity of exciton-polaritons expanding along a channel. By exciting a coherent superposition of K and K- tagged polaritons, we observe valley selective expansion of the polariton cloud without neither any applied external magnetic fields nor coherent Rayleigh scattering. Unlike the valley Hall effect for TMDC excitons, the observed optical valley Hall effect (OVHE) strikingly occurs on a macroscopic scale, and clearly reveals the potential for applications in spin-valley locked photonic devices.

The drag of half-light half-mater quasiparticles, exciton-polaritons, by an electric current is a peculiar mechanism of light-matter interaction in solids. While an ideal superfluid is protected from being dragged by its zero viscosity, here we argue that the state of the superfluid polariton condensate formed by a non-resonant optical pumping can be controlled by the electric current. The proposed mechanism is based on the stimulated relaxation of moving uncondensed excitons dragged by the electric current. The stimulated relaxation process favors the formation of a moving condensate in a quantum state that is characterised by the lowest condensation threshold. We also show that the electron-mediated inelastic scattering of the reservoir excitons to the condensate leads to the transfer of a non-zero mean momentum to the electron gas thus contributing to the electric current. We predict the generation of circular electric currents in a micropillar cavity in the presence of a nonresonant laser pumping at normal incidence., Comment: 7 pages, 4 figures

Atomically thin crystals of transition metal dichalcogenides are ideally suited to study the interplay of light-matter coupling, polarization and magnetic field effects. In this work, we investiagte the formation of exciton-polaritons in a MoSe2 monolayer, which is integrated in a fully-grown, monolithic microcavity. Due to the narrow linewidth of the polaritonic resonances, we are able to directly investigate the emerging valley Zeeman splitting of the hybrid light-matter resonances in the presence of a magnetic field. At a detuning of -54.5 meV (13.5 % matter constituent of the lower polariton branch), we find a Zeeman splitting of the lower polariton branch of 0.36 meV, which can be directly associated with an excitonic g factor of 3.94\pm0.13. Remarkably, we find that a magnetic field of 6T is sufficient to induce a notable valley polarization of 15 % in our polariton system, which approaches 30% at 9T. Strikingly, this circular polarization degree of the polariton (ground) state exceeds the polarization of the exciton reservoir for equal magnetic field magnitudes by approximately 50%, as a consequence of enhanced relaxation of bosons in our monolayer-based system., Comment: 8 pages, 4 figures

We show the full control of the polarization dynamics of a propagating exciton-polariton condensate in a planar microcavity by using a magnetic field applied in the Voigt geometry. The change of the spin-beat frequency, the suppression of the optical spin Hall effect and the rotation of the polarization pattern by the magnetic field are theoretically reproduced by accounting for the magneto-induced mixing of exciton-polariton and dark, spin forbidden, exciton states.

The self-trapping of exciton-polariton condensates is demonstrated and explained by the formation of a new polaron-like state. Above the polariton lasing threshold, local variation of the lattice temperature provides the mechanism for an attractive interaction between polaritons. Due to this attraction, the condensate collapses into a small bright spot. Its position and momentum variances approach the Heisenberg quantum limit. The self-trapping does not require either a resonant driving force or a presence of defects. The trapped state is stabilized by the phonon-assisted stimulated scattering of excitons into the polariton condensate. While the formation mechanism of the observed self-trapped state is similar to the Landau-Pekar polaron model, this state is populated by several thousands of quasiparticles, in a strike contrast to the conventional single-particle polaron state.

We synthesize macroscopically long linear carbon chains (carbynes) in a colloidal solution, then deposit them on a surface. The method is based on the formation of carbon threads by laser ablation in a colloid accompanied by the stabilization of resulting linear carbon chains by golden nanoparticles. We observe the signatures of the polyyne allotrope of carbyne in the photoluminescence and Raman spectra of the solutions. We deposit the synthesized carbyne threads on fused quartz glass substrates. The transmission electron microscopy images of the deposited threads with golden nanoparticles attached to their ends demonstrate the straight linear parts of the monoatomic carbon chains varying in length between 8 and 24 carbon atoms. This method paves the way to fabrication of an ultimate one-dimensional crystal: a monoatomic carbon wire., Comment: 13 pages, 5 figures, 1 table, including supplementary materials part at the end of the article

Dark excitons are of fundamental importance for a wide variety of processes in semiconductors, but are difficult to investigate using optical techniques due to their weak interaction with light fields. We reveal and characterize dark excitons injected by non-resonant pulsed excitation in a semiconductor microcavity structure containing InGaAs/GaAs quantum wells by monitoring their interactions with the bright lower polariton mode. We find a surprisingly long dark exciton lifetime of more than 20 ns which is longer than the time delay between two consecutive pulses. This creates a memory effect that we clearly observe through the variation of the time-resolved transmission signal. We propose a rate equation model that provides a quantitative agreement with the experimental data., Comment: 16 pages, 8 figures

We report the optical excitation-dependent output photocurrent characteristics of GaN-based polariton diode lasers operated under reverse-bias at room temperature. The photocurrent demonstrates a non-linear enhancement at an incident optical power of ~ 1.6 mW, which is approximately equivalent to the value of polariton lasing threshold observed when the diodes are operated under forward bias conditions. This is explained in the framework of an Auger-like process of excitonic dissociation into its constituent electron-hole pairs, which can be stimulated by the occupation of the polariton lasing states. The observed effect is a remarkable manifestation of the bosonic final state stimulation in polariton lasers. A model based on the coupled kinetic equations for the free carriers, the excitonic reservoir and the polariton condensate shows a good agreement to the experimental data.

Condensation of bosons into a macroscopic quantum state belongs to the most intriguing phenomena in nature. It was first realized in quantum gases of ultra-cold atoms, but more recently became accessible in open-dissipative, exciton-based solid-state systems at elevated temperatures. Semiconducting monolayer crystals have emerged as a new platform for studies of strongly bound excitons in ultimately thin materials. Here, we demonstrate the formation of a bosonic condensate driven by excitons hosted in an atomically thin layer of MoSe2, strongly coupled to light in a solid-state resonator. The structure is operated in the regime of collective strong coupling, giving rise to hybrid exciton-polariton modes composed of a Tamm-plasmon resonance, GaAs quantum well excitons and two-dimensional excitons confined in a monolayer of MoSe2. Polariton condensation in a monolayer crystal manifests by a superlinear increase of emission intensity from the hybrid polariton mode at injection powers as low as 4.8 pJ/pulse, as well as its density-dependent blueshift and a dramatic collapse of the emission linewidth as a hallmark of temporal coherence. Importantly, we observe a significant spin-polarization in the injected polariton condensate, a fingerprint of the core property of monolayer excitons subject to spin-valley locking. The observed effects clearly underpin the perspective of building novel highly non-linear valleytronic devices based on light-matter fluids, coherent bosonic light sources based on atomically thin materials, and paves the way towards studying materials with unconventional topological properties in the framework of bosonic condensation., Comment: 25 pages, 7 figures

We predict a strong enhancement of the critical temperature in a conventional Bardeen-Cooper-Schrieffer (BCS) superconductor in the presence of a bosonic condensate of exciton-polaritons. The effect depends strongly on the ratio of the cutoff frequencies for phonon and exciton-polariton mediated BCS superconductivity, respectively. We also discuss a possible design of hybrid semiconductor-superconductor structures suitable for the experimental observation of such an effect., Comment: 5 pages, 3 figures, accepted in Phys. Rev. Lett

We study the time evolution of the Optical Spin Hall Effect (OSHE), which occurs when exciton-polaritons undergo resonant Rayleigh scattering. The resulting spin pattern in momentum space is quantified by calculating the degree of circular polarization of the momentum space image for each point in time. We find the degree of circular polarization performing oscillations, which can be described within the framework of the pseudospin model by Kavokin et al. (Ref. 1)., Comment: 6 pages, 4 figures

Strong light matter coupling between excitons and microcavity photons, as described in the framework of cavity quantum electrodynamics, leads to the hybridization of light and matter excitations. The regime of collective strong coupling arises, when various excitations from different host media are strongly coupled to the same optical resonance. This leads to a well-controllable admixture of various matter components in three hybrid polariton modes. Here, we study a cavity device with four embedded GaAs quantum wells hosting excitons that are spectrally matched to the A-valley exciton resonance of a MoSe2 monolayer. The formation of hybrid polariton modes is evidenced in momentum resolved photoluminescence and reflectivity studies. We describe the energy and k-vector distribution of exciton-polaritons along the hybrid modes by a thermodynamic model, which yields a very good agreement with the experiment., Comment: 16 Pages, 5 Figures

Solid state cavity quantum electrodynamics is a rapidly advancing field which explores the frontiers of light-matter coupling. Plasmonic approaches are of particular interest in this field, since they carry the potential to squeeze optical modes to spaces significantly below the diffraction limit1,2, enhancing light-matter coupling. They further serve as an architecture to design ultra-fast, non-linear integrated circuits with smallest footprints3. Transition metal dichalcogenides are ideally suited as the active material in such circuits as they interact strongly with light at the ultimate monolayer limit4. Here, we implement a Tamm-plasmon-polariton structure, and study the coupling to a monolayer of WSe2, hosting highly stable excitons5. Exciton-Polariton formation at room temperature is manifested in the characteristic energy-momentum dispersion relation studied in photoluminescence, featuring an anti-crossing between the exciton and photon modes with a Rabi-splitting of 23.5 meV. Creating polaritonic quasi-particles in plasmonic architectures with atomic monolayers under ambient conditions is a crucial step towards compact, highly non-linear integrated photonic and polaritonic circuits6,7.

We develop the theoretical formalism to calculate second-order correlations in dissipative exciton-polariton system and we propose intensity-intensity correlation experiments to reveal the physics of exciton-light coupling in semiconductor microcavities in the Rabi oscillation regime. We predict a counter intuitive behaviour of the correlator between upper and lower polariton branches: due to the decoherence caused by stochastic exciton-photon conversions this correlator is expected to decrease below 1, while the individual second-order coherence of upper and lower polaritons exhibits non-monotonous bunching., Comment: 4 pages, 3 figures

Exciton-polariton modes arising from interaction between bound excitons in monolayer thin semiconductor sheets and photons in a Fabry-Perot microcavity are considered theoretically. We calculate the dispersion curves, mode lifetimes, Rabi splitting, and Hopfield coefficients of these structures for two nearly 2D semiconductor materials, MoS2 and WS2, and suggest that they are interesting for studying the rich physics associated with the Bose-Einstein condensation of exciton-polaritons. The large exciton binding energy and dipole allowed exciton transitions, in addition to the relatively easily controllable distance between the semiconductor sheets are the advantages of this system in comparison with traditional GaAs or CdTe based semiconductor microcavities. In particular, in order to mimic the rich physical properties of the quantum degenerate mixture of two bosonic species of dilute atomic gases with tunable inter-species interaction , we put forward a structure containing two semiconductor sheets separated by some atomic-scale distance (l) using a nearly 2D dielectric (e.g. h-BN), which offers the possibility of tuning the interaction between two exciton-polariton Bose-Enstein condensates. We show that the dynamics of this novel structure are ruled by two coupled Gross-Pitaevskii equations with the coupling parameter proportional to 1/l.

Recent experiments show that the Nernst-Ettingshausen effect is orders of magnitude stronger than the thermoelectric Seebeck effect in superconductors above the critical temperature. We explain different magnitudes of the two effects accounting for the magnetization current of virtual Cooper pairs. The method allows for detailed understanding of the surprising non-monotonic dependence of the Nernst-Ettingshausen coefficient on the magnetic field., Comment: 6 pages, 1 figure