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8. Materials for hydrogen-based energy storage – past, recent progress and future outlook

Author

Hirscher, M., Yartys, V.A., Baricco, M., Bellosta von Colbe, J., Blanchard, D., Bowman, R.C., Broom, D.P., Buckley, Craig, Chang, F., Chen, P., Cho, Y.W., Crivello, J.C., Cuevas, F., David, W.I.F., de Jongh, P.E., Denys, R.V., Dornheim, M., Felderhoff, M., Filinchuk, Y., Froudakis, G.E., Grant, D.M., Gray, E.M.A., Hauback, B.C., He, T., Humphries, Terry, Jensen, T.R., Kim, S., Kojima, Y., Latroche, M., Li, H.W., Lototskyy, M.V., Makepeace, J.W., Møller, K.T., Naheed, L., Ngene, P., Noréus, D., Nygård, M.M., Orimo, S.I., Paskevicius, Mark, Pasquini, L., Ravnsbæk, D.B., Veronica Sofianos, M., Udovic, T.J., Vegge, T., Walker, G.S., Webb, C.J., Weidenthaler, C., Zlotea, C., Hirscher, M., Yartys, V.A., Baricco, M., Bellosta von Colbe, J., Blanchard, D., Bowman, R.C., Broom, D.P., Buckley, Craig, Chang, F., Chen, P., Cho, Y.W., Crivello, J.C., Cuevas, F., David, W.I.F., de Jongh, P.E., Denys, R.V., Dornheim, M., Felderhoff, M., Filinchuk, Y., Froudakis, G.E., Grant, D.M., Gray, E.M.A., Hauback, B.C., He, T., Humphries, Terry, Jensen, T.R., Kim, S., Kojima, Y., Latroche, M., Li, H.W., Lototskyy, M.V., Makepeace, J.W., Møller, K.T., Naheed, L., Ngene, P., Noréus, D., Nygård, M.M., Orimo, S.I., Paskevicius, Mark, Pasquini, L., Ravnsbæk, D.B., Veronica Sofianos, M., Udovic, T.J., Vegge, T., Walker, G.S., Webb, C.J., Weidenthaler, C., and Zlotea, C.

Abstract

© 2020 The Authors Globally, the accelerating use of renewable energy sources, enabled by increased efficiencies and reduced costs, and driven by the need to mitigate the effects of climate change, has significantly increased research in the areas of renewable energy production, storage, distribution and end-use. Central to this discussion is the use of hydrogen, as a clean, efficient energy vector for energy storage. This review, by experts of Task 32, “Hydrogen-based Energy Storage” of the International Energy Agency, Hydrogen TCP, reports on the development over the last 6 years of hydrogen storage materials, methods and techniques, including electrochemical and thermal storage systems. An overview is given on the background to the various methods, the current state of development and the future prospects. The following areas are covered; porous materials, liquid hydrogen carriers, complex hydrides, intermetallic hydrides, electrochemical storage of energy, thermal energy storage, hydrogen energy systems and an outlook is presented for future prospects and research on hydrogen-based energy storage.

Published
2020

11. Contributor contact details

Author

Kilner, J.A., primary, Skinner, S.J., additional, Irvine, S.J.C., additional, Edwards, P.P., additional, Cowern, N.E.B., additional, Holliman, P.J., additional, Connell, A., additional, Davies, M.L., additional, Carnie, M.J., additional, Watson, T.M., additional, Nicholas, R.J., additional, Tuley, R.S., additional, Wijayantha, U., additional, Yildiz, B., additional, Doong, S.J., additional, Felderhoff, M., additional, Brett, D.J.L., additional, Agante, E., additional, Brandon, N.P., additional, Brightman, E., additional, Brown, R.J.C., additional, Manage, M., additional, Staffell, Iain, additional, Scott, K., additional, Manthiram, A., additional, Zhao, X., additional, Li, W., additional, Preux, N., additional, Rolle, A., additional, Vannier, R.N., additional, Grenier, J.–C., additional, Bassat, J.-M., additional, Mauvy, F., additional, Tao, S.W., additional, Cowin, P.I., additional, Lan, R., additional, Jacobson, A.J., additional, Yu, C., additional, Gong, W., additional, Traversa, E., additional, Fabbri, E., additional, Kiziroglou, M.E., additional, Yeatman, E.M., additional, Scrosati, B., additional, Hassoun, J., additional, Harris, I.R., additional, Jewell, G.W., additional, Chroneos, A., additional, Bishop, C.L., additional, Parfitt, D.C., additional, and Grimes, R.W., additional

Published
2012
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17. Magnesium based materials for hydrogen based energy storage: Past, present and future

Author

Yartys, V. A., Lototskyy, M. V., Akiba, E., Albert, R., Antonov, V. E., Ares, J. R., Baricco, M., Bourgeois, N., Buckley, C. E., Bellosta von Colbe, J. M., Crivello, J. C., Cuevas, F., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Hauback, B. C., Humphries, T. D., Jacob, I., Jensen, T. R., de Jongh, P. E., Joubert, J. M., Kuzovnikov, M. A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V. M., Rabkin, E., Sofianos, M. V., Stuart, A., Walker, G., Wang, Hui, Webb, C. J., Zhu, Min, Yartys, V. A., Lototskyy, M. V., Akiba, E., Albert, R., Antonov, V. E., Ares, J. R., Baricco, M., Bourgeois, N., Buckley, C. E., Bellosta von Colbe, J. M., Crivello, J. C., Cuevas, F., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Hauback, B. C., Humphries, T. D., Jacob, I., Jensen, T. R., de Jongh, P. E., Joubert, J. M., Kuzovnikov, M. A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V. M., Rabkin, E., Sofianos, M. V., Stuart, A., Walker, G., Wang, Hui, Webb, C. J., and Zhu, Min

Abstract

Magnesium hydride owns the largest share of publications on solid materials for hydrogen storage. The “Magnesium group” of international experts contributing to IEA Task 32 “Hydrogen Based Energy Storage” recently published two review papers presenting the activities of the group focused on magnesium hydride based materials and on Mg based compounds for hydrogen and energy storage. This review article not only overviews the latest activities on both fundamental aspects of Mg-based hydrides and their applications, but also presents a historic overview on the topic and outlines projected future developments. Particular attention is paid to the theoretical and experimental studies of Mg-H system at extreme pressures, kinetics and thermodynamics of the systems based on MgH 2 , nanostructuring, new Mg-based compounds and novel composites, and catalysis in the Mg based H storage systems. Finally, thermal energy storage and upscaled H storage systems accommodating MgH 2 are presented.

Published
2019

18. Magnesium based materials for hydrogen based energy storage: Past, present and future

Author

Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Yartys, V. A., Lototskyy, M. V., Akiba, E., Albert, R., Antonov, V. E., Ares, J. R., Baricco, M., Bourgeois, N., Buckley, C. E., Bellosta von Colbe, J. M., Crivello, J. C., Cuevas, F., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Hauback, B. C., Humphries, T. D., Jacob, I., Jensen, T. R., de Jongh, P. E., Joubert, J. M., Kuzovnikov, M. A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V. M., Rabkin, E., Sofianos, M. V., Stuart, A., Walker, G., Wang, Hui, Webb, C. J., Zhu, Min, Inorganic Chemistry and Catalysis, Sub Inorganic Chemistry and Catalysis, Yartys, V. A., Lototskyy, M. V., Akiba, E., Albert, R., Antonov, V. E., Ares, J. R., Baricco, M., Bourgeois, N., Buckley, C. E., Bellosta von Colbe, J. M., Crivello, J. C., Cuevas, F., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Hauback, B. C., Humphries, T. D., Jacob, I., Jensen, T. R., de Jongh, P. E., Joubert, J. M., Kuzovnikov, M. A., Latroche, M., Paskevicius, M., Pasquini, L., Popilevsky, L., Skripnyuk, V. M., Rabkin, E., Sofianos, M. V., Stuart, A., Walker, G., Wang, Hui, Webb, C. J., and Zhu, Min

Published
2019

19. Magnesium based materials for hydrogen based energy storage: Past, present and future

Author

Yartys, V., Lototskyy, M., Akiba, E., Albert, R., Antonov, V., Ares, J., Baricco, M., Bourgeois, N., Buckley, Craig, Bellosta von Colbe, J., Crivello, J., Cuevas, F., Denys, R., Dornheim, M., Felderhoff, M., Grant, D., Hauback, B., Humphries, Terry, Jacob, I., Jensen, T., de Jongh, P., Joubert, J., Kuzovnikov, M., Latroche, M., Paskevicius, Mark, Pasquini, L., Popilevsky, L., Skripnyuk, V., Rabkin, E., Sofianos, M., Stuart, A., Walker, G., Wang, H., Webb, C., Zhu, M., Yartys, V., Lototskyy, M., Akiba, E., Albert, R., Antonov, V., Ares, J., Baricco, M., Bourgeois, N., Buckley, Craig, Bellosta von Colbe, J., Crivello, J., Cuevas, F., Denys, R., Dornheim, M., Felderhoff, M., Grant, D., Hauback, B., Humphries, Terry, Jacob, I., Jensen, T., de Jongh, P., Joubert, J., Kuzovnikov, M., Latroche, M., Paskevicius, Mark, Pasquini, L., Popilevsky, L., Skripnyuk, V., Rabkin, E., Sofianos, M., Stuart, A., Walker, G., Wang, H., Webb, C., and Zhu, M.

Abstract

Magnesium hydride owns the largest share of publications on solid materials for hydrogen storage. The “Magnesium group” of international experts contributing to IEA Task 32 “Hydrogen Based Energy Storage” recently published two review papers presenting the activities of the group focused on magnesium hydride based materials and on Mg based compounds for hydrogen and energy storage. This review article not only overviews the latest activities on both fundamental aspects of Mg-based hydrides and their applications, but also presents a historic overview on the topic and outlines projected future developments. Particular attention is paid to the theoretical and experimental studies of Mg-H system at extreme pressures, kinetics and thermodynamics of the systems based on MgH2, nanostructuring, new Mg-based compounds and novel composites, and catalysis in the Mg based H storage systems. Finally, thermal energy storage and upscaled H storage systems accommodating MgH2 are presented.

Published
2019

20. Future perspectives of thermal energy storage with metal hydrides

Author

Manickam, K., Mistry, P., Walker, G., Grant, D., Buckley, Craig, Humphries, Terry, Paskevicius, Mark, Jensen, T., Albert, R., Peinecke, K., Felderhoff, M., Manickam, K., Mistry, P., Walker, G., Grant, D., Buckley, Craig, Humphries, Terry, Paskevicius, Mark, Jensen, T., Albert, R., Peinecke, K., and Felderhoff, M.

Abstract

Thermochemical energy storage materials have advantage of much higher energy densities compared to latent or sensible heat storage materials. Metal hydrides show good reversibility and cycling stability combined with high enthalpies. They can be used for short and long-term heat storage applications and can increase the overall flexibility and efficiency of solar thermal energy production. Metal hydrides with working temperatures less than 500 °C were in the focus of research and development over the last years. For the new generation of solar thermal energy plants new hydrides materials with working temperatures above 600 °C must be developed and characterized. In addition to thorough research on new metal hydrides, the construction and engineering of heat storage systems at these high temperatures are challenging. Corrosion problems, hydrogen embrittlement and selection of heat transfer fluids are significant topics for future research activities.

Published
2019

22. Magnesium based materials for hydrogen based energy storage: Past, present and future

Author

Yartys, V.A., primary, Lototskyy, M.V., additional, Akiba, E., additional, Albert, R., additional, Antonov, V.E., additional, Ares, J.R., additional, Baricco, M., additional, Bourgeois, N., additional, Buckley, C.E., additional, Bellosta von Colbe, J.M., additional, Crivello, J.-C., additional, Cuevas, F., additional, Denys, R.V., additional, Dornheim, M., additional, Felderhoff, M., additional, Grant, D.M., additional, Hauback, B.C., additional, Humphries, T.D., additional, Jacob, I., additional, Jensen, T.R., additional, de Jongh, P.E., additional, Joubert, J.-M., additional, Kuzovnikov, M.A., additional, Latroche, M., additional, Paskevicius, M., additional, Pasquini, L., additional, Popilevsky, L., additional, Skripnyuk, V.M., additional, Rabkin, E., additional, Sofianos, M.V., additional, Stuart, A., additional, Walker, G., additional, Wang, Hui, additional, Webb, C.J., additional, and Zhu, Min, additional

Published
2019
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25. Mg-based compounds for hydrogen and energy storage

Author

Crivello, J. -C., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Huot, J., Jensen, T. R., de Jongh, P., Latroche, M., Walker, G. S., Webb, C. J., Yartys, V. A., Crivello, J. -C., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Huot, J., Jensen, T. R., de Jongh, P., Latroche, M., Walker, G. S., Webb, C. J., and Yartys, V. A.

Abstract

Magnesium-based alloys attract significant interest as cost-efficient hydrogen storage materials allowing the combination of high gravimetric storage capacity of hydrogen with fast rates of hydrogen uptake and release and pronounced destabilization of the metal–hydrogen bonding in comparison with binary Mg–H systems. In this review, various groups of magnesium compounds are considered, including (1) RE–Mg–Ni hydrides (RE = La, Pr, Nd); (2) Mg alloys with p-elements (X = Si, Ge, Sn, and Al); and (3) magnesium alloys with d-elements (Ti, Fe, Co, Ni, Cu, Zn, Pd). The hydrogenation–disproportionation–desorption–recombination process in the Mg-based alloys (LaMg12, LaMg11Ni) and unusually high-pressure hydrides synthesized at pressures exceeding 100 MPa (MgNi2H3) and stabilized by Ni–H bonding are also discussed. The paper reviews interrelations between the properties of the Mg-based hydrides and p–T conditions of the metal–hydrogen interactions, chemical composition of the initial alloys, their crystal structures, and microstructural state.

Published
2016

26. Mg-based compounds for hydrogen and energy storage

Author

Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Crivello, J. -C., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Huot, J., Jensen, T. R., de Jongh, P., Latroche, M., Walker, G. S., Webb, C. J., Yartys, V. A., Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis, Crivello, J. -C., Denys, R. V., Dornheim, M., Felderhoff, M., Grant, D. M., Huot, J., Jensen, T. R., de Jongh, P., Latroche, M., Walker, G. S., Webb, C. J., and Yartys, V. A.

Published
2016

27. Metal hydrides for concentrating solar thermal power energy storage

Author

Sheppard, D., Paskevicius, M., Humphries, Terry, Felderhoff, M., Capurso, G., Bellosta von Colbe, J., Dornheim, M., Klassen, T., Ward, P., Teprovich, J., Corgnale, C., Zidan, R., Grant, D., Buckley, C., Sheppard, D., Paskevicius, M., Humphries, Terry, Felderhoff, M., Capurso, G., Bellosta von Colbe, J., Dornheim, M., Klassen, T., Ward, P., Teprovich, J., Corgnale, C., Zidan, R., Grant, D., and Buckley, C.

Abstract

The development of alternative methods for thermal energy storage is important for improving the efficiency and decreasing the cost of concentrating solar thermal power. We focus on the underlying technology that allows metal hydrides to function as thermal energy storage (TES) systems and highlight the current state-of-the-art materials that can operate at temperatures as low as room temperature and as high as 1100 °C. The potential of metal hydrides for thermal storage is explored, while current knowledge gaps about hydride properties, such as hydride thermodynamics, intrinsic kinetics and cyclic stability, are identified. The engineering challenges associated with utilising metal hydrides for high-temperature TES are also addressed.

Published
2016

36. The plastic crystalline A15 phase of dimethylaminoalane, [N(CH3)2–AlH2]3.

Author

Ley, M. B., Bernert, T., Ruiz-Fuertes, J., Goddard, R., Farès, C., Weidenthaler, C., and Felderhoff, M.

Subjects
PLASTIC crystals, LITHIUM aluminum hydride, DIMETHYLAMINE, CRYSTAL structure, PHASE transitions, DIFFERENTIAL scanning calorimetry, RAMAN spectra
Abstract

A plastic crystalline phase of dimethylaminoalane has been discovered at T ＞ 332 K. The phase transitions solid – plastic phase – liquid are fully reversible. The plastic crystalline phase exhibits a cubic unit cell, space group Pm3̅n, in which the dimethylaminoalane molecules rotate and adopt a structural arrangement reminiscent of the A15 phase. [ABSTRACT FROM AUTHOR]

Published
2016
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