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Aerosol particles play an important role in the microphysics of clouds and hence in their likelihood to precipitate. In the changing climate already-dry areas such as the United Arab Emirates (UAE) are predicted to become even drier. Comprehensive observations of the daily and seasonal variation in aerosol particle properties in such locations are required, reducing the uncertainty in such predictions. We analyse observations from a 1-year measurement campaign at a background location in the United Arab Emirates to investigate the properties of aerosol particles in this region, study the impact of boundary layer mixing on background aerosol particle properties measured at the surface, and study the temporal evolution of the aerosol particle cloud formation potential in the region. We used in situ aerosol particle measurements to characterise the aerosol particle composition, size, number, and cloud condensation nuclei (CCN) properties; in situ SO2 measurements as an anthropogenic signature; and a long-range scanning Doppler lidar to provide vertical profiles of the horizontal wind and turbulent properties to monitor the evolution of the boundary layer. Anthropogenic sulfate dominated the aerosol particle mass composition in this location. There was a clear diurnal cycle in the surface wind direction, which had a strong impact on aerosol particle total number concentration, SO2 concentration, and black carbon mass concentration. Local sources were the predominant source of black carbon as concentrations clearly depended on the presence of turbulent mixing, with much higher values during calm nights. The measured concentrations of SO2 , instead, were highly dependent on the surface wind direction as well as on the depth of the boundary layer when entrainment from the advected elevated layers occurred. The wind direction at the surface or of the elevated layer suggests that the oil refineries and the cities of Dubai and Abu Dhabi and other coastal conurbations were the remote sources of SO2. We observed new-aerosol-particle formation events almost every day (on 4 d out of 5 on average). Calm nights had the highest CCN number concentrations and lowest κ values and activation fractions. We did not observe any clear dependence of CCN number concentration and κ parameter on the height of the daytime boundary layer, whereas the activation fraction did show a slight increase with increasing boundary layer height due to the change in the shape of the aerosol particle size distribution where the relative portion of larger aerosol particles increased with increasing boundary layer height. We believe that this indicates that size is more important than chemistry for aerosol particle CCN activation at this site. The combination of instrumentation used in this campaign enabled us to identify periods when anthropogenic pollution from remote sources that had been transported in elevated layers was present and had been mixed down to the surface in the growing boundary layer. [ABSTRACT FROM AUTHOR]

One year of ground-based night-time Raman lidar observations has been analysed under the Optimization of Aerosol Seeding In rain enhancement Strategies (OASIS) project, in order to characterize the aerosol particle properties over a rural site in the United Arab Emirates. In total, 1130 aerosol particle layers were detected during the 1-year measurement campaign which took place between March 2018 and February 2019. Several subsequent aerosol layers could be observed simultaneously in the atmosphere up to 11 km. The observations indicate that the measurement site is a receptor of frequent dust events, but predominantly the dust is mixed with aerosols of anthropogenic and/or marine origin. The mean aerosol optical depth over the measurement site ranged at 0.37 ± 0.12 and 0.21 ± 0.11 for 355 and 532 nm, respectively. Moreover, mean lidar ratios of 43 ± 11 sr at a wavelength of 355 nm and 39 ± 10 sr at 532 nm were found. The average linear particle depolarization ratio measured over the course of the campaign was 15 ± 6 % and 19 ± 7 % at the 355 and 532 nm wavelengths, respectively. Since the region is both a source and a receptor of mineral dust, we have also explored the properties of Arabian mineral dust of the greater area of the United Arab of Emirates and the Arabian Peninsula. The observed Arabian dust particle properties were 45 ± 5 (42 ± 5) sr at 355 (532) nm for the lidar ratio, 25 ± 2 % (31 ± 2 %) for the linear particle depolarization ratio at 355 (532) nm, and 0.3 ± 0.2 (0.2 ± 0.2) for the extinction-related Ångström exponent (backscatter-related Ångström exponent) between 355 and 532 nm. This study is the first to report comprehensive optical properties of the Arabian dust particles based on 1-year long observations, using to their fullest the capabilities of a multi-wavelength Raman lidar instrument. The results suggest that the mineral dust properties over the Middle East and western Asia, including the observation site, are comparable to those of African mineral dust with regard to the particle depolarization ratios, but not for lidar ratios. The smaller lidar ratio values in this study compared to the reference studies are attributed to the difference in the geochemical characteristics of the soil originating in the study region compared to northern Africa. [ABSTRACT FROM AUTHOR]

We report initial results from the Optimization of Aerosol Seeding In rain enhancement Strategies (OASIS) field campaign in the United Arab Emirates. Understanding the background aerosol properties is crucial when designing precipitation enhancement strategies. The 1-year OASIS field campaign aimed at characterising the vertical profile of aerosol and the boundary-layer dynamics. The measurement setup comprised in-situ aerosol measurements (DMPS, APS, aethalometer, CCN measurements, filter samples), multi-wavelength lidar (PollyXT), scanning Doppler lidar (Halo Photonics Streamline). Identifying turbulent mixing in the boundary layer enabled extending the information gleaned from the surface measurements into the vertical profile up to the top of the well-mixed layer. The boundary layer exhibited a consistent strong diurnal cycle, with calm conditions at night and a well-mixed convective boundary layer developing during the day to heights of at least 2 km and often reaching 4 km. The surface aerosol concentrations usually decrease during the morning, presumably as a result of dilution into the growing boundary layer, followed by new particle formation. Elevated aerosol layers were also common. A major feature was the presence of low level jets in the wind profile, providing a mechanism for rapid horizontal transport of aerosol, both local and remote. The low-level jets often occurred after sunset, presumably as a response to the collapse of the convective boundary layer. We also identified significant dust events through the combined analysis of boundary layer winds and surface aerosol concentrations, where a rapid increase in aerosol concentrations coincide with wind changes throughout the vertical profile. This indicates air mass changes suggesting long-range transport of aerosol, with possible mechanisms including sea breezes or large-scale synoptic flows. Such flows can potentially generate clouds and convection. [ABSTRACT FROM AUTHOR]

OASIS is a multidisciplinary project aiming at a comprehensive quantification of the role of atmospheric aerosols in efficient precipitation enhancement efforts in the United Arab Emirates (UAE). The projects specific scientific objectives are to: 1) undertake a comprehensive 1-year field campaign (Feb 2018 – Feb 2019) in the UAE employing a multitude of in-situ and lidar instruments to quantify the characteristics and the vertical profile of current background aerosol population as well as the key meteorological drivers of cloud formation in the study region, 2) identify optimal seeding strategies (in terms of e.g., time, location, amount of seeding) by using mesoscale meteorological simulations together with cloud-resolving model simulations with a highly advanced aerosol microphysics description, 3) quantify the characteristics of theoretically optimal ice nucleation seed aerosol by employing a suite of molecular-level simulation methods in order to support future experimental work aiming to develop more efficient ice nuclei, and 4) utilize novel statistical approaches to identify the major sources of uncertainty in prediction of rain enhancement success.This presentation summarizes the main results from the first two project years after the completion of the field campaign and a substantial fraction of the mesoscale, cloud-scale and molecular scale modelling work. Our findings highlight the close connection between the aerosol concentrations and the boundary layer dynamics in the UAE atmosphere, illuminate the optimal seeding strategies in both winter stratocumulus and summer convective cloud cases, and point to surface defects as potential sites for efficient ice nucleation. [ABSTRACT FROM AUTHOR]