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In 2014, we measured activity concentration of radiocesium in the western North Pacific Ocean. In the north of Kuroshio Front high activity concentration of Fukushima-derived radiocesium in surface mixed layer in 2012 had been transported eastward by 2014. In the south of the front we found a radiocesium subsurface maximum in 200-600 m depth, which was similar to that observed in 2012. The subsurface maximum spread southward from 18°N to 15°N between 2012 and 2014, which suggests spreading of Fukushima-derived radiocesium into the whole western subtropical area by 2014 due to formation and subduction of the subtropical mode water. [ABSTRACT FROM AUTHOR]

A robust and rapid method for the determination of natural levels of beryllium (Be) in seawater was developed to facilitate mapping Be concentrations in the ocean. A solid-phase extraction method using a silica gel column was applied for preconcentration and purification of Be in seawater prior to determination of Be concentrations with inductively coupled plasma mass spectrometry (ICP-MS). Be was quantitatively adsorbed onto silica gel from solutions with pH values ranging from 6.3 to 9, including natural seawater. The chelating agent ethylenediamine tetraacetic acid was used to remove other ions in the seawater matrix (Na, Mg, and Ca) that interfere with the ICP-MS analysis. The reproducibility of the method was 3% based on triplicate analyses of natural seawater samples, and the detection limit was 0.4 pmol kg −1 for 250 mL of seawater, which is sufficient for the analysis of seawater in the open ocean. The method was then used to determine the vertical profile of Be in the eastern North Pacific Ocean, which was found to be a recycled-type profile in which the Be concentration increased with depth from the surface (7.2 pmol kg −1 at <200 m) to deep water (29.2 pmol kg −1 from 3500 m to the bottom). [ABSTRACT FROM AUTHOR]