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Afforestation has been initiated in Northeast Asia to improve ecological status. The responses of the regional hydrological cycle to vegetation restoration remain insufficiently explored. This study uses a variety of satellite-derived vegetation variables and hydrological cycle components to scan the eco-hydrological regimes in the Three-North Region of China and Mongolia during the past four decades. We observe that vegetation productivity increases mainly in North China (NC), Northeast China (NEC), Northwest China (NWC), and the north of Inner Mongolia and Mongolia. Precipitation and runoff show a decreasing trend (-0.4 mm/year and - 0.6 mm/year, respectively), yet they are less correlated to the normalized difference vegetation index and leaf area index. Along with increasing vegetation productivity, evapotranspiration increases (0.05 mm/year) obviously in NC and NEC, while root soil moisture (-0.001 m 3 /m 3 /year) and terrestrial water storage (-2.0 mm/year) decrease in NC and parts of NEC and NWC. The correlation coefficient between evapotranspiration and vegetation variables is up to 0.73. Collectively, results imply one potential adverse response of terrestrial water fluxes to increasing vegetation. Independent ecological and hydrological datasets further corroborate our work. Climatic factors (i.e., downward shortwave radiation and air temperature) and human activities (i.e., aerosol optical depth, carbon dioxide, and water withdrawal) substantially affect regional hydrological cycles. Considering the increasing vegetation productivity in the Three-North Region of China and Mongolia is likely to continue in the 21st century based on the Sixth Coupled Model Intercomparison Project (CMIP6) simulations, the terrestrial water fluxes may undergo deficit pressure. Overall, this study comprehensively investigates the vegetation and hydrology interplays, and provides a reference for protecting and improving ecological-hydrological conditions in Northeast Asia., Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2022 Elsevier B.V. All rights reserved.)