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Land surface temperature (LST) is increasingly needed for studying the functioning of the Earth's surface at local to global scale. Radiative transfer (RT) models that simulate top of atmosphere (TOA) radiance are essential tools to derive accurate LST from thermal infrared (TIR) signals of Earth observation (EO) satellites. DART (Discrete Anisotropic Radiative Transfer) is one of the most accurate and comprehensive three-dimensional models that simulate RT in the Earth-atmosphere system. Up to version 5.7.3, the mean absolute error (MAE) of DART atmospheric TIR radiance of six standard atmospheres (USSTD76, TROPICAL, MIDDLATSUM, MIDDLATWIN, SUBARCSUM, SUBARCWIN) over 3.5 μm - 20 μm was 3.1 K compared to the reference atmospheric RT model MODTRAN, which is much larger than the 1 K accuracy needed by most LST applications. Also, the radiance error reached 2.6 K for some TIR bands whereas the noise equivalent differential temperature (NeDT) of satellite TIR sensor is usually less than 0.4 K. Recently, the DART atmospheric RT modelling was greatly improved by (1) introducing the equivalent absorption cross-section of five most absorbing gases (H 2 O, CO 2 , O 3 , CH 4 , N 2 O), and (2) implementing a double-layer thermal emission method. The MAE of DART atmospheric TIR radiance of six standard atmospheres and actual atmospheres over France and the Mediterranean Sea is now better than 1.0 K. The band radiance error is less than 0.2 K in the EO satellite TIR bands. DART is still accurate if the temperature profiles of standard atmospheres are offset by less than 6 K and if the viewing zenith angle is less than 50°. In short, the improved DART meets the requirements of both LST applications, and present and future TIR EO satellite missions. It is already available to scientists (https://dart.omp.eu). • Improvement of DART atmospheric RT modelling in TIR region • Design of a more accurate double-layer thermal emission method • Pre-computation of equivalent absorption cross-section using MODTRAN • New DART accuracy meets LST applications and TIR EO satellite mission requirements [ABSTRACT FROM AUTHOR]