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Distinguishing between natural and anthropogenic controls on the proportions of naturally occurring radioactive materials (NORMs) in the environment is important for water resource management. In this study, the dynamics of uranium (U) and thorium (Th), two of the most prominent NORM elements, were investigated in the Red Deer River basin using monitoring data collected from 2015 to 2018. More than twofold increases in median proportions of total U (from 0.73 to 1.53 µg/L) and Th (from 0.008 to 0.104 µg/L) were observed for sites located downstream of the Steveville badlands, an area of highly erodible bedrock that a ~ 300 km section of the river flows through. Input is highly variable, coinciding mainly with increases in total suspended solids during intense rainstorms in the late summer. In-depth examination of monitoring data through factor analysis, multiple linear regression, mass balance calculations, and land use analysis highlights the importance of erosion and subsequent particle transport along river banks in the badlands area on the distribution of total U and Th, while also revealing that groundwater-surface water interaction affects proportions of dissolved U throughout the river. No significant influence from industry or land use on U and Th export was found, and proportions of U and Th in water and suspended sediment are within the natural ranges expected for surface waters and sediments/soils. Methodology employed in this study provides a basic framework for analysis of environmental monitoring datasets, which can be employed in the absence of radiochemical data to study the fate, transport, and sources of NORMs., (© 2022. Crown.)