1. Ultrafast Demagnetization Excited by Extreme Ultraviolet Light From a Free-Electron Laser
- Author
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Beata Ziaja, Maya Kiskinova, Andre Philippi-Kobs, M. H. Berntsen, Jochen Wagner, Leonard Müller, Robert Frömter, Miltcho B. Danailov, Emanuele Pedersoli, Vladimir Lipp, Michal Stransky, Michele Manfredda, Wojciech Roseker, Flavio Capotondi, Kai Bagschik, Hans Peter Oepen, Matthias Riepp, Gerhard Grübel, and Andreas Scherz
- Subjects
Materials science ,Excited state ,Extreme ultraviolet ,Demagnetizing field ,Free-electron laser ,Atomic physics ,Ultrashort pulse - Abstract
Ultrashort and intense extreme ultraviolet (XUV) and X-ray pulses readily available at free-electron lasers (FELs) enable studying non-linear light−matter interactions on femtosecond timescales. Here, we report on the non-linear fluence dependence of magnetic scattering of Co/Pt multilayers, using FERMI FEL’s 70-fs-long single and double XUV pulses, the latter with a temporal separation of 200 fs, with a photon energy slightly detuned to the Co M2,3 absorption edge. We observe a quenching in magnetic scattering that sets-in already in the non-destructive fluence regime of a few mJ/cm² typically used for FEL-probe experiments on magnetic materials. Calculations of the transient electronic structure in tandem with a phenomenological modeling of the experimental data by means of ultrafast demagnetization unambiguously show that XUV-radiation-induced demagnetization is the dominant mechanism for the quenching in the investigated fluence regime of
- Published
- 2021
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