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To better constrain late Neogene denudation of the Himalayas, we analysed in situ 10Be concentrations in 17 Neogene sediment samples of the Surai section (central Nepal) and two modern sediment samples of the Rapti River. We first refined the depositional ages of the Surai section from 36 new paleomagnetic analyses, five 26Al/10Be burial ages, and, based on the Dynamic Time Warping algorithm, 104 automatically calculated likely magnetostratigraphic correlations. We also traced changing sediment sources using major element and Sr-Nd isotopic data, finding at 4-3 Ma a switch from a large, trans-Himalayan river to a river draining only the Lesser Himalaya and Siwalik piedmont, increasing the contribution of recycled sediments at that time. 10Be concentrations in Neogene sediments range from (1.00 ± 0.36) to (5.22 ± 0.98) × 10³ at g-1 and decrease with stratigraphic age. Based on a flood plain transport model, our refined age model, and assuming a drainage change at 4-3 Ma, we reconstructed 10Be concentrations at the time of deposition. Assuming cosmogenic production rates similar to those of the modern basins, we calculated palaeodenudation rates of 0.9 ± 0.5 to 3.9 ± 2.7 mm a-1 from ca. 6 to 3 Ma in the palaeo-Karnali basin and 0.6 ± 0.2 to 1.6 ± 0.8 mm a-1 since ca. 3 Ma in the palaeo-Rapti basin. Given the uncertainties and similar modern values of ~2 mm a-1, the palaeo-Karnali denudation rates may have been steady at ~1.7 ± 0.3 mm a-1 for the last ca. 6 Ma. A transient acceleration of the denudation in the palaeo-Rapti basin of ~1.5 mm a-1 since ca. 1.5 Ma was likely due to the reworking of older, 10Be-depleted Siwalik sediments in the foreland. If true, this steadiness of the denudation rates may suggest that Quaternary glaciations did not largely affect Himalayan denudation. [ABSTRACT FROM AUTHOR]

We investigate chronology and age uncertainty for the middle to upper Pleistocene lower Bengal Fan using a novel age‐depth modeling approach that factors lithostratigraphic, magnetostratigraphic, biostratigraphic, cyclostratigraphic, and seismic stratigraphic constraints, based on results from the International Ocean Discovery Program Expedition 354 Bengal Fan and analysis of the GeoB97‐020/027 seismic line. The initial chronostratigraphic framework is established using regionally extensive hemipelagic sediment units, and only age‐depth models of fan deposits that respect the superposition of channel‐levee systems between sites are accepted. In doing so, we reconstruct signals of regional sediment accumulation rate and lithogenic sediment input through the perspective of a two‐dimensional ~320 km transect at 8°N that are consistent with more distal and more ambiguous regional records. This chronology allows us to discuss the depositional history of the middle to upper Pleistocene lower Bengal Fan within the context of sea level, climate, and tectonic controls. We hypothesize, based on the timing of accumulation rate changes, that progradation and intensification of the Bengal Fan's channel‐levee system at 8°N was largely driven by increases in sea level amplitude during this time. However, it is also possible this progradation was influenced by changes in Pleistocene climate and increased Himalayan erosion rates, driving greater sediment flux to the fan. Plain Language Summary: Deep sea fans are sediment deposits in the ocean that often form near river systems offshore continental margins. The largest of these, the Bengal Fan in the northern Indian Ocean, contains the most complete record of materials eroded from the Himalayan Mountains and can be used to study the climate and tectonic history of the region. Sediments are moved from the river mouth to the fan in a series of ever‐changing channels that distribute sediments across the fan surface, making it impossible to obtain a complete and continuous record of Himalayan erosion at any one location. International Ocean Discovery Program Expedition 354 drilled a series of seven locations in a transect across the fan to capture a more complete record of where sediment was deposited over the last 1.25 Myr, a time characterized by major changes in Earth's climate system. Here we discuss statistics of sediment deposition from a computer model constrained by observations from those seven sites. The results indicate that the Bengal Fan grew rapidly during a time when global sea level changes, caused by the growth and decay of continental ice sheets, became more intense. Key Points: A novel regional chronostratigraphic model is used to investigate evolution of the lower Bengal Fan over the last 1.25 MyrSeven IODP site chronologies are constrained by lithostratigraphic, magnetostratigraphic, biostratigraphic, cyclostratigraphic, and seismic stratigraphic constraintsGrowth and intensification of channel‐levee systems at 8°N correspond to increases in the amplitude of Pleistocene sea level changes [ABSTRACT FROM AUTHOR]

A sedimentological and geochemical study was carried out to explore the origin of arsenic contamination in sediments in Nawalparasi district, in the western Terai of Nepal. The investigation tools include major, trace and rare earth element analyses of core sediments, as well as C datings, and O, C isotopic analyses on mollusk shells. The results show that black schists from the Lesser Himalaya highly contributed to the detrital input in Parasi during the Pleistocene-Holocene transition because of focused erosion related to rapid uplift and high rainfall along the Main Central Thrust zone. In addition, aquifer silts, sands, and most of the brown clays underwent a certain degree of chemical weathering and physical reworking, and show possible inputs from the Siwaliks during the Late Holocene. A possible correlation between late Quaternary climate regimes and the concentration of arsenic in sediments is suspected, with arsenic preferentially concentrated during the drier periods of the last 25 kyr BP. The process of arsenic eluviations in sandy and silty sediments can explain the lower arsenic concentrations in sediments during humid periods. During the drier periods, seasonal precipitation was smaller and temperature was lower, leading to wet (less evaporative) soils in swampy environments. This environment favoured the development of aquatic plants and bacteria growing within in the moist land areas, enhancing the strong weathering of initially suspended load particles (micas and clays), which were preferentially deposited in quiet hydraulic environments. These sorting and weathering processes presumably allowed the arsenic to be concentrated in the finest sediment fraction. [ABSTRACT FROM AUTHOR]

Abstract: Continental chemical weathering is central in Earth''s surface biogeochemical cycles as it redistributes elements across reservoirs such as the crust and the oceans. However the evolution of weathering through time and its response to external forcing such as changes in climate remain poorly constrained. In this work, a composite sediment record from the Bay of Bengal is used to document the evolution of chemical weathering in the Himalayan system (Himalayan range and Indo-Gangetic floodplain), the world largest sediment conveyor to the oceans, since the Last Glacial Maximum (LGM). The degree of weathering of the sediments is documented using mobile to immobile ratios such as K/Si and H2O+/Si as well as detrital calcite abundance. Robust weathering proxies are derived by correcting the chemical composition of sediment for sorting effects that occur during transport and deposition. The Bay of Bengal record is also further compared to the chemical composition of modern river sediments from the Ganga and Brahmaputra basin. Weathering proxies all indicate that the sediments exported by the Ganga and Brahmaputra Rivers became increasingly weathered over the past ∼21kyr, whereas, Sr, Nd and major elements suggest a constant sediment provenance in the system over the last 21kyr. These changes in the degree of weathering of the sediments show that the weathering flux exported by the system to the Indian Ocean during the LGM was significantly lower than at present and demonstrate that chemical weathering in continental scale basins such as the Ganga and Brahmaputra responds to Late Quaternary climate changes. [Copyright &y& Elsevier]

Abstract: We present an extensive river sediment dataset covering the Ganga basin from the Himalayan front downstream to the Ganga mainstream in Bangladesh. These sediments were mainly collected over several monsoon seasons and include depth profiles of suspended particles in the river water column. Mineral sorting is the first order control on the chemical composition of river sediments. Taking into account this variability we show that sediments become significantly depleted in mobile elements during their transit through the floodplain. By comparing sediments sampled at the Himalayan front with sediments from the Ganga mainstream in Bangladesh it is possible to budget weathering in the floodplain. Assuming a steady state weathering regime in the floodplain, the weathering of Himalayan sediments in the Gangetic floodplain releases ca. (189±92)×109 and (69±22)×109 mol/yr of carbonate bound Ca and Mg to the dissolved load, respectively. Silicate weathering releases (53±18)×109 and (42±13)×109 mol/yr of Na and K while the release of silicate Mg and Ca is substantially lower, between ca. 0 and 20×109 mol/yr. Additionally, we show that sediment hydration, [H2O+], is a sensitive tracer of silicate weathering that can be used in continental detrital environments, such as the Ganga basin. Both [H2O+] content and the D/H isotopic composition of sediments increases during floodplain transfer in response to mineral hydrolysis and neoformations associated to weathering reactions. By comparing the chemical composition of river sediments across the floodplain with the composition of the eroded Himalayan source rocks, we suggest that the floodplain is the dominant location of silicate weathering for Na, K and [H2O+]. Overall this work emphasizes the role of the Gangetic floodplain in weathering Himalayan sediments. It also demonstrates how detrital sediments can be used as weathering tracers if mineralogical and chemical sorting effects are properly taken into account. [Copyright &y& Elsevier]

Abstract: We use the evolution of river sediment characteristics and sedimentary Corg from the Himalayan range to the delta to study the transport of Corg in the Ganga–Brahmaputra system and especially its fate during floodplain transit. A detailed characterisation of both mineral and organic particles for a sampling set of river sediments allows taking into account the sediment heterogeneity characteristic of such large rivers. We study the relationships between sediment characteristics (mineralogy, grain size, specific area) and Corg content in order to evaluate the controls on Corg loading. Contributions of C3 and C4 plants are estimated from Corg stable isotopic composition (δ13Corg). We use the evolution of δ13Corg values from the Himalayan range to the delta in order to study the fate of Corg during floodplain transit. Ganga and Brahmaputra sediments define two distinct linear relations with specific area. In spite of 4–5 times higher specific area, Ganga sediments have similar Corg content, grain size and mineralogy as Brahmaputra sediments, indicating that specific area does not exert a primary control on Corg loading. The general correlation between the total Corg content and Al/Si ratio indicates that Corg loading is mainly related to: (1) segregation of organic particles under hydrodynamic forces in the river, and (2) the ability of mineral particles to form organo-mineral aggregates. Bed and suspended sediments have distinct δ13Corg values. In bed sediments, δ13Corg values are compatible with a dominant proportion of fossil Corg derived from Himalayan rocks erosion. Suspended sediments from Himalayan tributaries at the outflow of the range have low δ13Corg values (−24.8‰ average) indicating a dominant proportion of C3 plant inputs. In the Brahmaputra basin, δ13Corg values of suspended sediments are constant along the river course in the plain. On the contrary, suspended sediments of the Ganga in Bangladesh have higher δ13Corg values (−22.4‰ to −20.0‰), consistent with a significant contribution of C4 plant derived from the floodplain. Our data indicate that, during the plain transit, more than 50% of the recent biogenic Corg coming from the Himalaya is oxidised and replaced by floodplain Corg. This renewal process likely occurs during successive deposition-erosion cycles and river course avulsions in the plain. [Copyright &y& Elsevier]

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[1] Sources and fluxes of particulate organic carbon (OC) in the Ganga-Brahmaputra river system were estimated from 13C/12C ratios of bedrocks, soils, bank and suspended river sediments from a Himalayan watershed (Narayani, Nepal), and the Bangladesh floodplain. In the watershed of the Narayani, OC δ13C values for bank and suspended sediments have similar values and narrow ranges, with a mean of about -24.2‰ at the base of the Himalayas. On the Bangladesh floodplain, bank and suspended sediments are enriched in 13C (δ13C about -22.5‰) relative to those collected at the base of the Himalayas. The OC exported at the base of the Himalayan range is estimated to include about 15% from the 13C enriched C4 biomass while the C4 contribution is about 25% of the OC exported by the Ganga and Brahmaputra. A calculated total OC flux of 0.65 × 1012 molC yr-1 is exported to the ocean or trapped in the plain. In sediments of the Ganga and Brahmaputra, the clay-size fraction is depleted in 13C (<2.6‰) relative to the bulk sediment. Possible explanations are that either the organic matter associated with clays is largely inherited from the Himalayan watersheds, or, and considered more likely, the clays and coarser sediments sample different OC pools, possibly with different ages (the growth of C4 crops has dramatically increased since the mid twentieth century), on the floodplain. The OC budget of the actual Ganga-Brahmaputra system is broadly comparable to that derived from the Quaternary sediments of the Bengal fan that represents about 10% of the global OC contribution to the continental margins. [ABSTRACT FROM AUTHOR]

The Bangladesh lowlands are traversed by the largest sediment flux on the planet. Detritus generated mostly in Himalayan highlands and conveyed through the Ganga–Brahmaputra rivers and Meghna estuary reaches the Bay of Bengal, where it forms a composite deltaic system. This study integrates the vast existing database on Ganga–Brahmaputra sediments of all grain sizes from clay to sand with new petrographic, mineralogical, and geochemical data on estuarine and shallow-marine sands. A large spectrum of compositional signatures was used to: (i) assess the relative supply of the Ganga and Brahmaputra rivers to estuarine and shelfal sediments; (ii) define the compositional variability of estuarine sediments and the impact exerted by hydraulic sorting and climate-related chemical weathering on provenance signals; (iii) define the compositional variability of shelf sediments and the potential hydrodynamic segregation of fast-settling heavy minerals in coastal environments and of slow-settling platy micas on low-energy outer-shelf floors; (iv) consider the potential additional mud supply from the western subaerial part of the delta formerly built by the Ganga River; and (v) draw a preliminary mineralogical comparison between fluvio-deltaic sediments and turbidites of the Bengal–Nicobar deep-sea fan, thus tracing sediment dispersal across the huge sedimentary system extending from Tibet to the equatorial Indian Ocean. All investigated mineralogical and geochemical parameters, as well as Sr and Nd isotope ratios and clay–mineral assemblages, showed a clear prevalence in sediment supply from the Brahmaputra (60–70%) over the Ganga (30–40%). Heavy-mineral suites and Sr and Nd isotope fingerprints of Bengal shelf sediments are nearly identical to those of the Brahmaputra River and Meghna estuary, also because the Brahmaputra carries almost twice as many Ca-plagioclase grains and heavy minerals including epidote than the Ganga, and these minerals control the large majority of the Sr and Nd budgets. The experience gained in modern settings can be directly extrapolated only to the recent past, because sediments older than the late Pleistocene and buried more than a few hundred meters begin to lose less durable ferromagnesian minerals by selective chemical dissolution, which makes quantitative estimates progressively less robust in more deeply buried older strata. [ABSTRACT FROM AUTHOR]

This article illustrates a multi-technique frontier approach for the provenance study of silt-size sediments. The mineralogical composition of low-density and heavy-mineral fractions of four samples of fine to very coarse silt deposited on the Bengal shelf was analyzed separately for six different grain-size classes by combining grain counting under an optical microscope, Raman spectroscopy, and X-ray diffraction. The geochemical composition was determined on both bulk-sediment samples and on their <5-μm classes. Such a "multiple-window" approach allowed capturing the full mineralogical information contained in each sample, as well as the size-dependent intra-sample variability of all compositional parameters. The comparison between grain-size distributions obtained by different methods highlighted a notable fallacy of laser granulometry, which markedly overestimated the size of the finest mode represented by fine silt and clay. As a test case, we chose to investigate sediments of the Bengal shelf, where detritus is fed from the Meghna estuary, formed by the joint Ganga and Brahmaputra Rivers and representing the largest single entry point of sediment in the world's oceans. The studied samples show the typical fingerprint of orogenic detritus produced by focused erosion of collision orogens. Bengal shelf silt is characterized by a feldspatho-quartzose (F-Q) composition with a Q/F ratio decreasing from 3.0 to 1.7 with increasing grain size, plagioclase prevailing over K-feldspar, and rich transparent-heavy-mineral assemblages including mainly amphibole with epidote, and minor garnet and pyroxene. Such a detrital signature compares very closely with Brahmaputra suspended load, but mineralogical and geochemical parameters, including the anomalous decrease of the Q/F ratio with increasing grain size, consistently indicate more significant Ganga contribution for cohesive fine silt. The accurate quantitative characterization of different size fractions of Bengal shelf sediments represents an essential step to allow comparison of compositional signatures characterizing different segments of this huge source-to-sink system, from fluvial and deltaic sediments of the Himalayan foreland basin and Bengal shelf to the Bengal Fan. [ABSTRACT FROM AUTHOR]

An unambiguous Neogene and Quaternary sequence of clastic sedimentation in the middleBengal fan has been retrieved by IODP Expedition 354. The Sr-Nd isotopic fingerprint ofsilicate fraction, turbiditic sediments have clear Himalayan origin. The turbidites&#x2019; chemicalcomposition showed virtually no differences with the modern Himalayan riversediments, with no significant variation through time1. In details, however, theisotope geochemistry defines a systematic consistent with subtle variations in thecomposition of the sources of the sediments. Mineralogical effects, such as nuggetseffects and the predominance of some heavy minerals in the isotopic budget ofsome elements2 and sedimentological sorting3 are also prone to modify the Sr-Ndisotopic fingerprint of deep-sea turbidites. In the Bay of Bengal, such effects generateanti-correlated changes but the extend on ɛNd is rather small, at most 1ɛg???? betweencoarsest and fine layers within the same tubidite. The analysis of 75 samples ofcoarse silt across the transect cored by Exp. 354 at 8˚ N and U1444 hole from byExp. 353 at 14˚ N define temporal changes that are insensitive to the samplinglocation and attribute to changes in the tectonic regime in the Himalayan range.In particular, the activation of the MBT and associated exhumation of the LesserHimalayan sequence (LHS) is marked by a drop in the ɛNd by up to 2.1ɛg???? startingaround 7.6Ma. The rise in the proportion of LHS material is then stopped around6.0Ma, likely to correspond to the activation of the MCT1 in the range. For theolder period, only one record from U1451 is available and might be more subject tochanges in the sediment supply within the Bengal Fan. Nevertheless, the middleMiocene is dominated by material derived from the high Himalayan crystalline seriesrelated to exhumation along the MCT with rising contribution through time (until∼10Ma) of the Trans-Himalaya batholith and the significant erosion of the southernTibet. 1) France-Lanord, C., Spiess, V., Klaus, A., Schwenk, T., Expedition 354Scientists. (2016). http://doi.org/10.14379 /iodp.proc.354.2016. 2) Garçon et al.(2014) https://doi.org/10.1016/j.chemgeo.2013.11.018. 3) McLennan et al. (1989)https://doi.org/10.1038/337547a0 [ABSTRACT FROM AUTHOR]

Abstract: Sediments carried in suspension represent a fundamental part of fluvial transport. Nonetheless, largely because of technical problems, they have been hitherto widely neglected in provenance studies. In order to determine with maximum possible precision the mineralogy of suspended load collected in vertical profiles from water surface to channel bottom of Rivers Ganga and Brahmaputra, we combined Raman spectroscopy with traditional heavy-mineral and X-ray diffraction analyses, carried out separately on low-density and dense fractions of all significant size classes in each sample (multiple-window approach). Suspended load resulted to be a ternary mixture of dominant silt enriched in phyllosilicates, subordinate clay largely derived from weathered floodplains, and sand mainly produced by physical erosion and mechanical grinding during transport in Himalayan streams. Sediment concentration and grain size increase steadily with water depth. Whereas absolute concentration of clay associated with Fe-oxyhydroxides and organic matter is almost depth-invariant, regular mineralogical and consequently chemical changes from shallow to deep load result from marked increase of faster-settling, coarser, denser, or more spherical grains toward the bed. Such steady intersample compositional variability can be modeled as a mixture of clay, silt and sand modes with distinct mineralogical and chemical composition. With classical formulas describing sediment transport by turbulent diffusion, absolute and relative concentrations can be predicted at any depth for each textural mode and each detrital component. Based on assumptions on average chemistry of detrital minerals and empirical formulas to calculate their settling velocities, the suspension-sorting model successfully reproduces mineralogy and chemistry of suspended load at different depths. Principal outputs include assessment of contributions by each detrital mineral to the chemical budget, and calibration of dense minerals too rare to be precisely estimated by optical or Raman analysis but crucial in both detrital-geochronology and settling-equivalence studies. Hydrodynamic conditions during monsoonal discharge could also be evaluated. Understanding compositional variability of suspended load is a fundamental pre-requisite to correctly interpret mineralogical and geochemical data in provenance analysis of modern and ancient sedimentary deposits, to accurately assess weathering processes, sediment fluxes and erosion patterns, and to unambiguously evaluate the effects of anthropogenic modifications on the natural environment. [Copyright &y& Elsevier]

Abstract: This study investigates the natural processes that control concentration of detrital minerals and consequently chemical elements in river sand. The novelty of our approach consists in the systematic integration of detailed textural, petrographical, mineralogical and chemical data, and in the quantitative description and modeling of relationships among mineralogical and chemical variables for each sample and each grain-size class in each sample. Bed sediment in transit in the largest sedimentary system on Earth chiefly consists of fine-grained lithofeldspathoquartzose sand including rich amphibole–epidote–garnet suites, mixed with minor very-fine-grained-sand to silt subpopulations containing less heavy minerals and representing intermittent suspension. Mineralogical and particularly chemical differences between Ganga and Brahmaputra bedload are orders of magnitude less than both intersample variability associated with selective-entrainment effects and intrasample variability associated with settling-equivalence effects. Any provenance interpretation of mineralogical, chemical, or detrital-geochronology datasets therefore requires quantitative understanding of hydraulically controlled compositional variability. Mineralogical and chemical, intrasample and intersample variability can be deduced with simple equations and numerical solutions. The underlying assumptions on the chemical composition of detrital minerals, as well as the possible pitfalls, uncertainties and approximations involved are discussed. Principal results include calibration of rare REE-bearing ultradense minerals, ill-determined by optical analyses but crucial in both detrital-geochronology and settling-equivalence studies, and assessment of progressively changing concentration for any detrital component with increasing intensity of selective-entrainment effects. Contributions by each mineral group to the chemical budget were inferred with sufficient precision and accuracy. Although complex because of diverse controlling factors including provenance, weathering and anthropogenic pollution, mineralogical and consequently chemical variability of fluvial sediments can be quantitatively predicted. This path, difficult because of insufficient information but far from hopeless, shall eventually lead to more accurate calculation of sediment fluxes and chemical budgets, as well as to a deeper understanding of sedimentary geochemistry and fluvial sedimentology. [Copyright &y& Elsevier]

Abstract: Neoproterozoic glacial and post-glacial sediments from the Volta Basin (West Africa) form a stratigraphic ‘Triad’ of tillites, carbonates and cherts. The carbonates that cap the tillites were studied in detail at Bwipe (Ghana), in the western part of the basin. They are made of finely-laminated dolostones with well-preserved sedimentary features, suggesting that dolomite formation was penecontemporaneous of deposition in a warm, arid peritidal environment, with microbial activity. Rare-earth element distribution display seawater-like patterns. Redox-sensitive trace elements indicate suboxic conditions. High Ba/Al ratios can be related to high organic productivity. δ 13C values are nearly constant at −3.7‰ and δ 18OPDB are about −6‰. 87Sr/86Sr ratios range between 0.7061 and 0.7073. The δ 13C signatures are nearly similar to those of coeval cap dolostones from the northern part of the Basin. The dolostones change upwards to limestones with secondary textures, as well as more negative δ 13C and higher 87Sr/86Sr ratio. Therefore, only the dolostones witness the post-glacial conditions in seawater. It is proposed that, due to a bloom of microbial productivity following ice thaw, organic matter likely accumulated at the water–sediment interface and was consumed by sulphate-reducing bacteria, leading to the precipitation of δ 13C-negative dolomite. This microbially mediated model is supported by present-day field evidence from hypersaline lagoons in Brazil and by previously published culture experiments. It is consistent with the sedimentological and geochemical data from the Ghana cap dolostones and can be applied to other Neoproterozoic cap dolostones worldwide. [Copyright &y& Elsevier]

Re-Os analyses were performed on suspended loads and coarser grained bank sediments of the Brahmaputra River system. Re and Os concentrations of these sediments vary from 7 to 1154 ppt and from 3 to 173 ppt, respectively. 187Os/188Os ratios range from 0.178 to 6.8, and thus vary from nearly mantle to very radiogenic crustal values. Nevertheless, most of the sediments have 187Os/188Os ratios less than 1.5, and nearly all of the samples of the Brahmaputra main channel have ratios less than 1.2. Thus, as previously suggested, the Brahmaputra is much less radiogenic than the Ganga. The Siang River, the northern extension of the Brahmaputra, is quite radiogenic in Os despite receiving sediments from the Tsangpo River, which flows along a suture zone with ultramafic outcrops. The Brahmaputra main channel has a fairly constant 187Os/188Os ratio even though its tributaries contribute sediments with very heterogeneous Os isotopic compositions. These data, along with the corresponding Nd isotopic compositions, suggest that about 60–90% of the sediment in the Brahmaputra system is derived from Himalayan formations (Higher Himalaya and Lesser Himalaya) whereas 10–40% comes from ophiolite-bearing sequences, perhaps eastern equivalents of those of the Transhimalayan Plutonic Belt. Os data also confirm previously published Sr and Nd results, indicating that about half of the sediments delivered to the Brahmaputra are supplied by the Siang River, while the Himalayan and the eastern tributaries account for 40 and 10%, respectively.The lower 187Os/188Os of the Brahmaputra River compared to that of the Ganga is due to two factors. One is the more limited presence of the Lesser Himalaya and hence the lower black shale content of the eastern Himalaya. The other is the non-radiogenic Os supplied by the eastern and southern tributaries, reflecting the presence of mantle-derived lithologies in this region. Despite the lower sediment supply from these tributaries, they contribute greatly to the Os budget of the Brahmaputra River. This study indicates that the Brahmaputra River has little effect on the present-day seawater Os budget. However, reconsideration of this budget suggests that the Ganga, which provides the most radiogenic Os of major rivers studied to date, may have significant impact on the marine Os isotopic composition. The Indo-Asian collision cannot be excluded as an important cause of the increase in the marine 187Os/188Os over the past 16 million years until the contributions of all of the rivers draining the Himalayan Tibetan Plateau are known. [Copyright &y& Elsevier]

Atmospheric CO 2 and global climate are closely coupled. Since 800 ka CO 2 concentrations have been up to 50% higher during interglacial compared to glacial periods. Because of its dependence on temperature, humidity, and erosion rates, chemical weathering of exposed silicate minerals was suggested to have dampened these cyclic variations of atmospheric composition. Cooler and drier conditions and lower non-glacial erosion rates suppressed in situ chemical weathering rates during glacial periods. However, using systematic variations in major element geochemistry, Sr–Nd isotopes and clay mineral records from Ocean Drilling Program Sites 1143 and 1144 in the South China Sea spanning the last 1.1 Ma, we show that sediment deposited during glacial periods was more weathered than sediment delivered during interglacials. We attribute this to subaerial exposure and weathering of unconsolidated shelf sediments during glacial sealevel lowstands. Our estimates suggest that enhanced silicate weathering of tropical shelf sediments exposed during glacial lowstands can account for ∼9% of the carbon dioxide removed from the atmosphere during the glacial and thus represent a significant part of the observed glacial–interglacial variation of ∼80 ppmv. As a result, if similar magnitudes can be identified in other tropical shelf-slope systems, the effects of increased sediment exposure and subsequent silicate weathering during lowstands could have potentially enhanced the drawdown of atmospheric CO 2 during cold stages of the Quaternary. This in turn would have caused an intensification of glacial cycles. [ABSTRACT FROM AUTHOR]

Abstract: In order to reveal particulate organic carbon (POC) source and mode of transport in the largest river basin on Earth, we sampled the main sediment-laden tributaries of the Amazon system (Solimões, Madeira and Amazon) during two sampling campaigns, following vertical depth-profiles. This sampling technique takes advantage of hydrodynamic sorting to access the full range of solid erosion products transported by the river. Using the Al/Si ratio of the river sediments as a proxy for grain size, we find a general increase in POC content with Al/Si, as sediments become finer. However, the sample set shows marked variability in the POC content for a given Al/Si ratio, with the Madeira River having lower POC content across the measured range in Al/Si. The POC content is not strongly related to the specific surface area (SSA) of the suspended load, and bed sediments have a much lower POC/SSA ratio. These data suggest that SSA exerts a significant, yet partial, control on POC transport in Amazon River suspended sediment. We suggest that the role of clay mineralogy, discrete POC particles and rock-derived POC warrant further attention in order to fully understand POC transport in large rivers. To examine the source of POC in the Amazon Basin in more detail, we use radiocarbon (14C) content and the stable isotope composition (δ13C) of POC. 14C activity demonstrates that rock-derived POC is a significant component of river bed sediments and contributes to POC across the river depth-profiles of suspended sediments. We estimate that the flux of rock-derived POC may reach 10% of the total POC export by the Amazon River. After correcting for rock-derived POC input, we find that POC from the terrestrial biosphere (biospheric POC) is mostly sourced from C3-plants. Higher biospheric POC δ13C values in the Madeira River (by 0.5–1‰) are best explained by a small (<5%) contribution of C4-grasses from Bolivian savannas. Finally, we use 14C to estimate the mean age of biospheric POC exported from the Amazon Basin. The data show that biospheric POC is younger in the Solimões River (1120years) than in the Madeira River (2850 years). These ages are much younger than the corresponding estimates of sediment residence time in the basin, suggesting that lowland areas and/or young POC from above-ground biomass may contribute disproportionately to the biomarker signals in terrigenous sediments of the Amazon delta. [Copyright &y& Elsevier]

Abstract: The Himalayas represent the archetype of mountain building due to active continental collision and are considered in many studies as the locus of intense interactions between climate, denudation and tectonics. Estimates of modern denudation rates across the entire range remain, however, relatively sparse. In this study, in situ-produced cosmogenic 10Be concentrations were measured in detritic quartz in order to determine basin-scale denudation rates for the central part of the Himalayan range. River sand was sampled over several years in the main trans-Himalayan rivers, from the Himalayan front to the Ganga outlet in Bangladesh. The calculated 10Be denudation rates of the trans-Himalayan river basins range from 0.5 to 2.4mmyr−1 (average 1.3mmyr−1) and vary by up to a factor of 3 between sampling years. These denudation rates strongly contrast with the 0.007mmyr−1 denudation rate of southern tributary basins draining the Indian craton. This work also shows that in the Ganga basin, no systematic evolution of average 10Be concentrations is observed during floodplain transfer, implying that distal samples can be used to estimate the integrated denudation rate of the whole central Himalayan range. Samples from the Ganga in Bangladesh display remarkably low variability in 10Be concentration, implying an average Himalayan denudation rate of 1.0–1.1mmyr−1. However, within the floodplain, several samples suggest a recent perturbation of sediment transport dynamics with a recent increase in the relative sediment contribution from southern tributaries. The Himalayan sediment flux, deduced from the 10Be denudation rate of the range, is 610±230Mtyr−1. This flux is consistent, within uncertainty, with sediment fluxes derived from sediment gauging. The similarity of the two flux estimates suggests that Himalayan erosion fluxes have remained stable over the last centuries, even if the large uncertainties associated with each method hamper more precise assessments. [Copyright &y& Elsevier]

Abstract: This study uses 238U–234U–230Th disequilibria in river sediments in order to constrain the transfer times of sediments in alluvial plains of rivers from Himalaya and the Gangetic plain. From the observed distributions we infer sediment transfer times of about 100 ka in the Gangetic plain for rivers taking their source in the Himalayan chain, and longer transfer of about 160–250 ka for foothill-fed rivers. This difference is probably related to the difference in the sediment transport dynamics of these two types of rivers. [Copyright &y& Elsevier]