1. Engineering the thermal conductivity along an individual silicon nanowire by selective helium ion irradiation
- Author
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Olga S. Ovchinnikova, Alex Belianinov, Raymond R. Unocic, Dan Liu, Matthew J. Burch, Jie Chen, Hanfang Hao, John T. L. Thong, Liyan Zhu, Daniel S. Pickard, Baowen Li, Yunshan Zhao, and Songkil Kim
- Subjects
Materials science ,Science ,Nanowire ,FOS: Physical sciences ,General Physics and Astronomy ,chemistry.chemical_element ,Nanotechnology ,02 engineering and technology ,01 natural sciences ,Article ,General Biochemistry, Genetics and Molecular Biology ,Thermal conductivity ,0103 physical sciences ,Thermal ,Irradiation ,010306 general physics ,Helium ,Condensed Matter - Materials Science ,Multidisciplinary ,business.industry ,Scattering ,Materials Science (cond-mat.mtrl-sci) ,General Chemistry ,021001 nanoscience & nanotechnology ,Amorphous solid ,chemistry ,Scattering rate ,Optoelectronics ,0210 nano-technology ,business - Abstract
The ability to engineer the thermal conductivity of materials allows us to control the flow of heat and derive novel functionalities such as thermal rectification, thermal switching and thermal cloaking. While this could be achieved by making use of composites and metamaterials at bulk length-scales, engineering the thermal conductivity at micro- and nano-scale dimensions is considerably more challenging. In this work, we show that the local thermal conductivity along a single Si nanowire can be tuned to a desired value (between crystalline and amorphous limits) with high spatial resolution through selective helium ion irradiation with a well-controlled dose. The underlying mechanism is understood through molecular dynamics simulations and quantitative phonon-defect scattering rate analysis, where the behaviour of thermal conductivity with dose is attributed to the accumulation and agglomeration of scattering centres at lower doses. Beyond a threshold dose, a crystalline-amorphous transition was observed., Manipulating the flow of heat at the nanoscale is difficult because it requires the ability to tune the thermal properties of tiny structures. Here, the authors locally change the thermal conductivity of an individual silicon nanowire by irradiating it with helium ions.
- Published
- 2017