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Fundamental questions in chemistry and physics may never be answered due to the exponential complexity of the underlying quantum phenomena. A desire to overcome this challenge has sparked a new industry of quantum technologies with the promise that engineered quantum systems can address these hard problems. A key step towards demonstrating such a system will be performing a computation beyond the capabilities of any classical computer, achieving so-called quantum supremacy. Here, using 9 superconducting qubits, we demonstrate an immediate path towards quantum supremacy. By individually tuning the qubit parameters, we are able to generate thousands of unique Hamiltonian evolutions and probe the output probabilities. The measured probabilities obey a universal distribution, consistent with uniformly sampling the full Hilbert-space. As the number of qubits in the algorithm is varied, the system continues to explore the exponentially growing number of states. Combining these large datasets with techniques from machine learning allows us to construct a model which accurately predicts the measured probabilities. We demonstrate an application of these algorithms by systematically increasing the disorder and observing a transition from delocalized states to localized states. By extending these results to a system of 50 qubits, we hope to address scientific questions that are beyond the capabilities of any classical computer.

Statistical mechanics is founded on the assumption that all accessible configurations of a system are equally likely. This requires dynamics that explore all states over time, known as ergodic dynamics. In isolated quantum systems, however, the occurrence of ergodic behavior has remained an outstanding question. Here, we demonstrate ergodic dynamics in a small quantum system consisting of only three superconducting qubits. The qubits undergo a sequence of rotations and interactions and we measure the evolution of the density matrix. Maps of the entanglement entropy show that the full system can act like a reservoir for individual qubits, increasing their entropy through entanglement. Surprisingly, these maps bear a strong resemblance to the phase space dynamics in the classical limit; classically chaotic motion coincides with higher entanglement entropy. We further show that in regions of high entropy the full multi-qubit system undergoes ergodic dynamics. Our work illustrates how controllable quantum systems can investigate fundamental questions in non-equilibrium thermodynamics.

We report the first electronic structure calculation performed on a quantum computer without exponentially costly precompilation. We use a programmable array of superconducting qubits to compute the energy surface of molecular hydrogen using two distinct quantum algorithms. First, we experimentally execute the unitary coupled cluster method using the variational quantum eigensolver. Our efficient implementation predicts the correct dissociation energy to within chemical accuracy of the numerically exact result. Second, we experimentally demonstrate the canonical quantum algorithm for chemistry, which consists of Trotterization and quantum phase estimation. We compare the experimental performance of these approaches to show clear evidence that the variational quantum eigensolver is robust to certain errors. This error tolerance inspires hope that variational quantum simulations of classically intractable molecules may be viable in the near future., Comment: 13 pages, 7 figures. This revision is to correct an error in the coefficients of identity in Table 1

The discovery of topological phases in condensed matter systems has changed the modern conception of phases of matter. The global nature of topological ordering makes these phases robust and hence promising for applications. However, the non-locality of this ordering makes direct experimental studies an outstanding challenge, even in the simplest model topological systems, and interactions among the constituent particles adds to this challenge. Here we demonstrate a novel dynamical method to explore topological phases in both interacting and non-interacting systems, by employing the exquisite control afforded by state-of-the-art superconducting quantum circuits. We utilize this method to experimentally explore the well-known Haldane model of topological phase transitions by directly measuring the topological invariants of the system. We construct the topological phase diagram of this model and visualize the microscopic evolution of states across the phase transition, tasks whose experimental realizations have remained elusive. Furthermore, we developed a new qubit architecture that allows simultaneous control over every term in a two-qubit Hamiltonian, with which we extend our studies to an interacting Hamiltonian and discover the emergence of an interaction-induced topological phase. Our implementation, involving the measurement of both global and local textures of quantum systems, is close to the original idea of quantum simulation as envisioned by R. Feynman, where a controllable quantum system is used to investigate otherwise inaccessible quantum phenomena. This approach demonstrates the potential of superconducting qubits for quantum simulation and establishes a powerful platform for the study of topological phases in quantum systems.

Progress in superconducting qubit experiments with greater numbers of qubits or advanced techniques such as feedback requires faster and more accurate state measurement. We have designed a multiplexed measurement system with a bandpass filter that allows fast measurement without increasing environmental damping of the qubits. We use this to demonstrate simultaneous measurement of four qubits on a single superconducting integrated circuit, the fastest of which can be measured to 99.8% accuracy in 140ns. This accuracy and speed is suitable for advanced multi-qubit experiments including surface code error correction., Comment: Five figures

A major challenge in the field of quantum computing is the construction of scalable qubit coupling architectures. Here, we demonstrate a novel tuneable coupling circuit that allows superconducting qubits to be coupled over long distances. We show that the inter-qubit coupling strength can be arbitrarily tuned over nanosecond timescales within a sequence that mimics actual use in an algorithm. The coupler has a measured on/off ratio of 1000. The design is self-contained and physically separate from the qubits, allowing the coupler to be used as a module to connect a variety of elements such as qubits, resonators, amplifiers, and readout circuitry over long distances. Such design flexibility is likely to be essential for a scalable quantum computer., Comment: 9 manuscript pages, 4 manuscript figures, 3 supplementary information pages, 4 supplementary figures

Entanglement is one of the key resources required for quantum computation, so experimentally creating and measuring entangled states is of crucial importance in the various physical implementations of a quantum computer. In superconducting qubits, two-qubit entangled states have been demonstrated and used to show violations of Bell's Inequality and to implement simple quantum algorithms. Unlike the two-qubit case, however, where all maximally-entangled two-qubit states are equivalent up to local changes of basis, three qubits can be entangled in two fundamentally different ways, typified by the states $|\mathrm{GHZ}> = (|000> + |111>)/\sqrt{2}$ and $|\mathrm{W}> = (|001> + |010> + |100>)/\sqrt{3}$. Here we demonstrate the operation of three coupled superconducting phase qubits and use them to create and measure $|\mathrm{GHZ}>$ and $|\mathrm{W}>$ states. The states are fully characterized using quantum state tomography and are shown to satisfy entanglement witnesses, confirming that they are indeed examples of three-qubit entanglement and are not separable into mixtures of two-qubit entanglement., Comment: 9 pages, 5 figures. Version 2: added supplementary information and fixed image distortion in Figure 2.

We analyze the crosstalk error mechanism in measurement of two capacitively coupled superconducting flux-biased phase qubits. The damped oscillations of the superconducting phase after the measurement of the first qubit may significantly excite the second qubit, leading to its measurement error. The first qubit, which is highly excited after the measurement, is described classically. The second qubit is treated both classically and quantum-mechanically. The results of the analysis are used to find the upper limit for the coupling capacitance (thus limiting the frequency of two-qubit operations) for a given tolerable value of the measurement error probability., Comment: 16 pages, Revtex; minor changes in the text and figures