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Engineered dissipative reservoirs have the potential to steer many-body quantum systems toward correlated steady states useful for quantum simulation of high-temperature superconductivity or quantum magnetism. Using up to 49 superconducting qubits, we prepared low-energy states of the transverse-field Ising model through coupling to dissipative auxiliary qubits. In one dimension, we observed long-range quantum correlations and a ground-state fidelity of 0.86 for 18 qubits at the critical point. In two dimensions, we found mutual information that extends beyond nearest neighbors. Lastly, by coupling the system to auxiliaries emulating reservoirs with different chemical potentials, we explored transport in the quantum Heisenberg model. Our results establish engineered dissipation as a scalable alternative to unitary evolution for preparing entangled many-body states on noisy quantum processors.

Undesired coupling to the surrounding environment destroys long-range correlations on quantum processors and hinders the coherent evolution in the nominally available computational space. This incoherent noise is an outstanding challenge to fully leverage the computation power of near-term quantum processors. It has been shown that benchmarking Random Circuit Sampling (RCS) with Cross-Entropy Benchmarking (XEB) can provide a reliable estimate of the effective size of the Hilbert space coherently available. The extent to which the presence of noise can trivialize the outputs of a given quantum algorithm, i.e. making it spoofable by a classical computation, is an unanswered question. Here, by implementing an RCS algorithm we demonstrate experimentally that there are two phase transitions observable with XEB, which we explain theoretically with a statistical model. The first is a dynamical transition as a function of the number of cycles and is the continuation of the anti-concentration point in the noiseless case. The second is a quantum phase transition controlled by the error per cycle; to identify it analytically and experimentally, we create a weak link model which allows varying the strength of noise versus coherent evolution. Furthermore, by presenting an RCS experiment with 67 qubits at 32 cycles, we demonstrate that the computational cost of our experiment is beyond the capabilities of existing classical supercomputers, even when accounting for the inevitable presence of noise. Our experimental and theoretical work establishes the existence of transitions to a stable computationally complex phase that is reachable with current quantum processors.

An important measure of the development of quantum computing platforms has been the simulation of increasingly complex physical systems. Prior to fault-tolerant quantum computing, robust error mitigation strategies are necessary to continue this growth. Here, we study physical simulation within the seniority-zero electron pairing subspace, which affords both a computational stepping stone to a fully correlated model, and an opportunity to validate recently introduced ``purification-based'' error-mitigation strategies. We compare the performance of error mitigation based on doubling quantum resources in time (echo verification) or in space (virtual distillation), on up to $20$ qubits of a superconducting qubit quantum processor. We observe a reduction of error by one to two orders of magnitude below less sophisticated techniques (e.g. post-selection); the gain from error mitigation is seen to increase with the system size. Employing these error mitigation strategies enables the implementation of the largest variational algorithm for a correlated chemistry system to-date. Extrapolating performance from these results allows us to estimate minimum requirements for a beyond-classical simulation of electronic structure. We find that, despite the impressive gains from purification-based error mitigation, significant hardware improvements will be required for classically intractable variational chemistry simulations., Comment: 10 pages, 13 page supplementary material, 12 figures. Experimental data available at https://doi.org/10.5281/zenodo.7225821

The discovery of topological order has revolutionized the understanding of quantum matter in modern physics and provided the theoretical foundation for many quantum error correcting codes. Realizing topologically ordered states has proven to be extremely challenging in both condensed matter and synthetic quantum systems. Here, we prepare the ground state of the toric code Hamiltonian using an efficient quantum circuit on a superconducting quantum processor. We measure a topological entanglement entropy near the expected value of $\ln2$, and simulate anyon interferometry to extract the braiding statistics of the emergent excitations. Furthermore, we investigate key aspects of the surface code, including logical state injection and the decay of the non-local order parameter. Our results demonstrate the potential for quantum processors to provide key insights into topological quantum matter and quantum error correction., Comment: 6 pages 4 figures, plus supplementary materials

A promising approach to study condensed-matter systems is to simulate them on an engineered quantum platform. However, achieving the accuracy needed to outperform classical methods has been an outstanding challenge. Here, using eighteen superconducting qubits, we provide an experimental blueprint for an accurate condensed-matter simulator and demonstrate how to probe fundamental electronic properties. We benchmark the underlying method by reconstructing the single-particle band-structure of a one-dimensional wire. We demonstrate nearly complete mitigation of decoherence and readout errors and arrive at an accuracy in measuring energy eigenvalues of this wire with an error of ~0.01 rad, whereas typical energy scales are of order 1 rad. Insight into this unprecedented algorithm fidelity is gained by highlighting robust properties of a Fourier transform, including the ability to resolve eigenenergies with a statistical uncertainty of 1e-4 rad. Furthermore, we synthesize magnetic flux and disordered local potentials, two key tenets of a condensed-matter system. When sweeping the magnetic flux, we observe avoided level crossings in the spectrum, a detailed fingerprint of the spatial distribution of local disorder. Combining these methods, we reconstruct electronic properties of the eigenstates where we observe persistent currents and a strong suppression of conductance with added disorder. Our work describes an accurate method for quantum simulation and paves the way to study novel quantum materials with superconducting qubits.

Quantum algorithms offer a dramatic speedup for computational problems in machine learning, material science, and chemistry. However, any near-term realizations of these algorithms will need to be heavily optimized to fit within the finite resources offered by existing noisy quantum hardware. Here, taking advantage of the strong adjustable coupling of gmon qubits, we demonstrate a continuous two-qubit gate set that can provide a 3x reduction in circuit depth as compared to a standard decomposition. We implement two gate families: an iSWAP-like gate to attain an arbitrary swap angle, $\theta$, and a CPHASE gate that generates an arbitrary conditional phase, $\phi$. Using one of each of these gates, we can perform an arbitrary two-qubit gate within the excitation-preserving subspace allowing for a complete implementation of the so-called Fermionic Simulation, or fSim, gate set. We benchmark the fidelity of the iSWAP-like and CPHASE gate families as well as 525 other fSim gates spread evenly across the entire fSim($\theta$, $\phi$) parameter space achieving purity-limited average two-qubit Pauli error of $3.8 \times 10^{-3}$ per fSim gate., Comment: 20 pages, 17 figures

The interplay of interactions and strong disorder can lead to an exotic quantum many-body localized (MBL) phase. Beyond the absence of transport, the MBL phase has distinctive signatures, such as slow dephasing and logarithmic entanglement growth; they commonly result in slow and subtle modification of the dynamics, making their measurement challenging. Here, we experimentally characterize these properties of the MBL phase in a system of coupled superconducting qubits. By implementing phase sensitive techniques, we map out the structure of local integrals of motion in the MBL phase. Tomographic reconstruction of single and two qubit density matrices allowed us to determine the spatial and temporal entanglement growth between the localized sites. In addition, we study the preservation of entanglement in the MBL phase. The interferometric protocols implemented here measure affirmative correlations and allow us to exclude artifacts due to the imperfect isolation of the system. By measuring elusive MBL quantities, our work highlights the advantages of phase sensitive measurements in studying novel phases of matter., Comment: 5+28 pages, 5+22 figures, updated version

We demonstrate diabatic two-qubit gates with Pauli error rates down to $4.3(2)\cdot 10^{-3}$ in as fast as 18 ns using frequency-tunable superconducting qubits. This is achieved by synchronizing the entangling parameters with minima in the leakage channel. The synchronization shows a landscape in gate parameter space that agrees with model predictions and facilitates robust tune-up. We test both iSWAP-like and CPHASE gates with cross-entropy benchmarking. The presented approach can be extended to multibody operations as well., Comment: Main text: 6 pages, 4 figures. Supplementary: 2 pages, 2 figures

We develop a high speed on-chip flux measurement using a capacitively shunted SQUID as an embedded cryogenic transducer and apply this technique to the qualification of a near-term scalable printed circuit board (PCB) package for frequency tunable superconducting qubits. The transducer is a flux tunable LC resonator where applied flux changes the resonant frequency. We apply a microwave tone to probe this frequency and use a time-domain homodyne measurement to extract the reflected phase as a function of flux applied to the SQUID. The transducer response bandwidth is 2.6 GHz with a maximum gain of $\rm 1200^\circ/\Phi_0$ allowing us to study the settling amplitude to better than 0.1%. We use this technique to characterize on-chip bias line routing and a variety of PCB based packages and demonstrate that step response settling can vary by orders of magnitude in both settling time and amplitude depending on if normal or superconducting materials are used. By plating copper PCBs in aluminum we measure a step response consistent with the packaging used for existing high-fidelity qubits.

Complex integrated circuits require multiple wiring layers. In complementary metal-oxide-semiconductor (CMOS) processing, these layers are robustly separated by amorphous dielectrics. These dielectrics would dominate energy loss in superconducting integrated circuits. Here we demonstrate a procedure that capitalizes on the structural benefits of inter-layer dielectrics during fabrication and mitigates the added loss. We separate and support multiple wiring layers throughout fabrication using SiO$_2$ scaffolding, then remove it post-fabrication. This technique is compatible with foundry level processing and the can be generalized to make many different forms of low-loss multi-layer wiring. We use this technique to create freestanding aluminum vacuum gap crossovers (airbridges). We characterize the added capacitive loss of these airbridges by connecting ground planes over microwave frequency $\lambda/4$ coplanar waveguide resonators and measuring resonator loss. We measure a low power resonator loss of $\sim 3.9 \times 10^{-8}$ per bridge, which is 100 times lower than dielectric supported bridges. We further characterize these airbridges as crossovers, control line jumpers, and as part of a coupling network in gmon and fuxmon qubits. We measure qubit characteristic lifetimes ($T_1$'s) in excess of 30 $\mu$s in gmon devices.

Statistical mechanics is founded on the assumption that a system can reach thermal equilibrium, regardless of the starting state. Interactions between particles facilitate thermalization, but, can interacting systems always equilibrate regardless of parameter values\,? The energy spectrum of a system can answer this question and reveal the nature of the underlying phases. However, most experimental techniques only indirectly probe the many-body energy spectrum. Using a chain of nine superconducting qubits, we implement a novel technique for directly resolving the energy levels of interacting photons. We benchmark this method by capturing the intricate energy spectrum predicted for 2D electrons in a magnetic field, the Hofstadter butterfly. By increasing disorder, the spatial extent of energy eigenstates at the edge of the energy band shrink, suggesting the formation of a mobility edge. At strong disorder, the energy levels cease to repel one another and their statistics approaches a Poisson distribution - the hallmark of transition from the thermalized to the many-body localized phase. Our work introduces a new many-body spectroscopy technique to study quantum phases of matter.

Fundamental questions in chemistry and physics may never be answered due to the exponential complexity of the underlying quantum phenomena. A desire to overcome this challenge has sparked a new industry of quantum technologies with the promise that engineered quantum systems can address these hard problems. A key step towards demonstrating such a system will be performing a computation beyond the capabilities of any classical computer, achieving so-called quantum supremacy. Here, using 9 superconducting qubits, we demonstrate an immediate path towards quantum supremacy. By individually tuning the qubit parameters, we are able to generate thousands of unique Hamiltonian evolutions and probe the output probabilities. The measured probabilities obey a universal distribution, consistent with uniformly sampling the full Hilbert-space. As the number of qubits in the algorithm is varied, the system continues to explore the exponentially growing number of states. Combining these large datasets with techniques from machine learning allows us to construct a model which accurately predicts the measured probabilities. We demonstrate an application of these algorithms by systematically increasing the disorder and observing a transition from delocalized states to localized states. By extending these results to a system of 50 qubits, we hope to address scientific questions that are beyond the capabilities of any classical computer.

We present a fabrication process for fully superconducting interconnects compatible with superconducting qubit technology. These interconnects allow for the 3D integration of quantum circuits without introducing lossy amorphous dielectrics. They are composed of indium bumps several microns tall separated from an aluminum base layer by titanium nitride which serves as a diffusion barrier. We measure the whole structure to be superconducting (transition temperature of 1.1$\,$K), limited by the aluminum. These interconnects have an average critical current of 26.8$\,$mA, and mechanical shear and thermal cycle testing indicate that these devices are mechanically robust. Our process provides a method that reliably yields superconducting interconnects suitable for use with superconducting qubits.

Josephson junctions form the essential non-linearity for almost all superconducting qubits. The junction is formed when two superconducting electrodes come within $\sim$1 nm of each other. Although the capacitance of these electrodes is a small fraction of the total qubit capacitance, the nearby electric fields are more concentrated in dielectric surfaces and can contribute substantially to the total dissipation. We have developed a technique to experimentally investigate the effect of these electrodes on the quality of superconducting devices. We use $\lambda$/4 coplanar waveguide resonators to emulate lumped qubit capacitors. We add a variable number of these electrodes to the capacitive end of these resonators and measure how the additional loss scales with number of electrodes. We then reduce this loss with fabrication techniques that limit the amount of lossy dielectrics. We then apply these techniques to the fabrication of Xmon qubits on a silicon substrate to improve their energy relaxation times by a factor of 5.

By analyzing the dissipative dynamics of a tunable gap flux qubit, we extract both sides of its two-sided environmental flux noise spectral density over a range of frequencies around $2k_BT/h \approx 1\,\rm{GHz}$, allowing for the observation of a classical-quantum crossover. Below the crossover point, the symmetric noise component follows a $1/f$ power law that matches the magnitude of the $1/f$ noise near $1\,{\rm{Hz}}$. The antisymmetric component displays a 1/T dependence below $100\,\rm{mK}$, providing dynamical evidence for a paramagnetic environment. Extrapolating the two-sided spectrum predicts the linewidth and reorganization energy of incoherent resonant tunneling between flux qubit wells., Comment: paper + supplement

Many superconducting qubit systems use the dispersive interaction between the qubit and a coupled harmonic resonator to perform quantum state measurement. Previous works have found that such measurements can induce state transitions in the qubit if the number of photons in the resonator is too high. We investigate these transitions and find that they can push the qubit out of the two-level subspace, and that they show resonant behavior as a function of photon number. We develop a theory for these observations based on level crossings within the Jaynes-Cummings ladder, with transitions mediated by terms in the Hamiltonian that are typically ignored by the rotating wave approximation. We find that the most important of these terms comes from an unexpected broken symmetry in the qubit potential. We confirm the theory by measuring the photon occupation of the resonator when transitions occur while varying the detuning between the qubit and resonator.

The intriguing many-body phases of quantum matter arise from the interplay of particle interactions, spatial symmetries, and external fields. Generating these phases in an engineered system could provide deeper insight into their nature and the potential for harnessing their unique properties. However, concurrently bringing together the main ingredients for realizing many-body phenomena in a single experimental platform is a major challenge. Using superconducting qubits, we simultaneously realize synthetic magnetic fields and strong particle interactions, which are among the essential elements for studying quantum magnetism and fractional quantum Hall (FQH) phenomena. The artificial magnetic fields are synthesized by sinusoidally modulating the qubit couplings. In a closed loop formed by the three qubits, we observe the directional circulation of photons, a signature of broken time-reversal symmetry. We demonstrate strong interactions via the creation of photon-vacancies, or "holes", which circulate in the opposite direction. The combination of these key elements results in chiral groundstate currents, the first direct measurement of persistent currents in low-lying eigenstates of strongly interacting bosons. The observation of chiral currents at such a small scale is interesting and suggests that the rich many-body physics could survive to smaller scales. We also motivate the feasibility of creating FQH states with near future superconducting technologies. Our work introduces an experimental platform for engineering quantum phases of strongly interacting photons and highlight a path toward realization of bosonic FQH states., Comment: in Nature Physics (2016)

We present a method to optimize qubit control parameters during error detection which is compatible with large-scale qubit arrays. We demonstrate our method to optimize single or two-qubit gates in parallel on a nine-qubit system. Additionally, we show how parameter drift can be compensated for during computation by inserting a frequency drift and using our method to remove it. We remove both drift on a single qubit and independent drifts on all qubits simultaneously. We believe this method will be useful in keeping error rates low on all physical qubits throughout the course of a computation. Our method is O(1) scalable to systems of arbitrary size, providing a path towards controlling the large numbers of qubits needed for a fault-tolerant quantum computer, Comment: 8 pages with supplemental, 7 figures

A major challenge in quantum computing is to solve general problems with limited physical hardware. Here, we implement digitized adiabatic quantum computing, combining the generality of the adiabatic algorithm with the universality of the digital approach, using a superconducting circuit with nine qubits. We probe the adiabatic evolutions, and quantify the success of the algorithm for random spin problems. We find that the system can approximate the solutions to both frustrated Ising problems and problems with more complex interactions, with a performance that is comparable. The presented approach is compatible with small-scale systems as well as future error-corrected quantum computers., Comment: Main text: 7 pages, 5 figures. Supplementary: 12 pages, 9 figures

Leakage errors occur when a quantum system leaves the two-level qubit subspace. Reducing these errors is critically important for quantum error correction to be viable. To quantify leakage errors, we use randomized benchmarking in conjunction with measurement of the leakage population. We characterize single qubit gates in a superconducting qubit, and by refining our use of Derivative Reduction by Adiabatic Gate (DRAG) pulse shaping along with detuning of the pulses, we obtain gate errors consistently below $10^{-3}$ and leakage rates at the $10^{-5}$ level. With the control optimized, we find that a significant portion of the remaining leakage is due to incoherent heating of the qubit., Comment: 10 pages, 10 figures including supplement; fixed typos in metadata

We introduce a frequency-multiplexed readout scheme for superconducting phase qubits. Using a quantum circuit with four phase qubits, we couple each qubit to a separate lumped-element superconducting readout resonator, with the readout resonators connected in parallel to a single measurement line. The readout resonators and control electronics are designed so that all four qubits can be read out simultaneously using frequency multiplexing on the one measurement line. This technology provides a highly efficient and compact means for reading out multiple qubits, a significant advantage for scaling up to larger numbers of qubits., Comment: 4 pages, 4 figures

We find that stray infrared light from the 4 K stage in a cryostat can cause significant loss in superconducting resonators and qubits. For devices shielded in only a metal box, we measured resonators with quality factors Q = 10^5 and qubits with energy relaxation times T_1=120 ns, consistent with a stray light-induced quasiparticle density of 170-230 \mu m^{-3}. By adding a second black shield at the sample temperature, we found about an order of magnitude improvement in performance and no sensitivity to the 4 K radiation. We also tested various shielding methods, implying a lower limit of Q = 10^8 due to stray light in the light-tight configuration., Comment: 4 pages, 4 figures

A major challenge in the field of quantum computing is the construction of scalable qubit coupling architectures. Here, we demonstrate a novel tuneable coupling circuit that allows superconducting qubits to be coupled over long distances. We show that the inter-qubit coupling strength can be arbitrarily tuned over nanosecond timescales within a sequence that mimics actual use in an algorithm. The coupler has a measured on/off ratio of 1000. The design is self-contained and physically separate from the qubits, allowing the coupler to be used as a module to connect a variety of elements such as qubits, resonators, amplifiers, and readout circuitry over long distances. Such design flexibility is likely to be essential for a scalable quantum computer., Comment: 9 manuscript pages, 4 manuscript figures, 3 supplementary information pages, 4 supplementary figures

Entanglement is one of the key resources required for quantum computation, so experimentally creating and measuring entangled states is of crucial importance in the various physical implementations of a quantum computer. In superconducting qubits, two-qubit entangled states have been demonstrated and used to show violations of Bell's Inequality and to implement simple quantum algorithms. Unlike the two-qubit case, however, where all maximally-entangled two-qubit states are equivalent up to local changes of basis, three qubits can be entangled in two fundamentally different ways, typified by the states $|\mathrm{GHZ}> = (|000> + |111>)/\sqrt{2}$ and $|\mathrm{W}> = (|001> + |010> + |100>)/\sqrt{3}$. Here we demonstrate the operation of three coupled superconducting phase qubits and use them to create and measure $|\mathrm{GHZ}>$ and $|\mathrm{W}>$ states. The states are fully characterized using quantum state tomography and are shown to satisfy entanglement witnesses, confirming that they are indeed examples of three-qubit entanglement and are not separable into mixtures of two-qubit entanglement., Comment: 9 pages, 5 figures. Version 2: added supplementary information and fixed image distortion in Figure 2.