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Entanglement in a many-particle system can enable measurement sensitivities beyond that achievable by only classical correlations. For an ensemble of spins, all-to-all interactions are known to reshape the quantum projection noise, leading to a form of entanglement known as spin squeezing. Here, we demonstrate spin squeezing with strictly short-range contact interactions. In particular, working with ultracold lithium atoms in optical lattices, we utilize superexchange interactions to realize a nearest-neighbor anisotropic Heisenberg model. We investigate the resulting quench dynamics from an initial product state in both one and three dimensions. In 1D, we observe $1.9^{+0.7}_{-0.5}$ dB of spin squeezing in quantitative agreement with theory. However, in 3D, we observe a maximum of $2.0^{+0.7}_{-0.7}$ dB of squeezing, over an order of magnitude smaller than that expected. We demonstrate that this discrepancy arises from the presence of a finite density of holes; both the motion of the holes as well as direct coupling between spin and density qualitatively alter the spin dynamics. Our observations point to the importance of understanding the complex interplay between motional and spin degrees of freedom in quantum simulators.

A Thouless pump is a slowly driven one-dimensional band insulator which pumps charge at a quantised rate. Previous work showed that pumping persists in weakly disordered chains, and separately in clean chains at finite drive frequency. We study the interplay of disorder and finite frequency, and show that the pump rate always decays to zero due to non-adiabatic transitions between the instantaneous eigenstates. However, the decay is slow, occurring on a time-scale that is exponentially large in the period of the drive. In the adiabatic limit, the band gap in the instantaneous spectrum closes at a critical disorder strength above which pumping ceases. We predict the scaling of the pump rate around this transition from a model of scattering between rare states near the band edges. Our predictions can be experimentally tested in ultracold atomic and photonic platforms., Comment: 11 pages, 7 figures

Ergodicity, the central tenet of statistical mechanics, requires that an isolated system will explore all of its available phase space permitted by energetic and symmetry constraints. Mechanisms for violating ergodicity are of great interest for probing non-equilibrium matter and for protecting quantum coherence in complex systems. For decades, polyatomic molecules have served as an intriguing and challenging platform for probing ergodicity breaking in vibrational energy transport, particularly in the context of controlling chemical reactions. Here, we report the observation of rotational ergodicity breaking in an unprecedentedly large and symmetric molecule, 12C60. This is facilitated by the first ever observation of icosahedral ro-vibrational fine structure in any physical system, first predicted for 12C60 in 1986. The ergodicity breaking exhibits several surprising features: first, there are multiple transitions between ergodic and non-ergodic regimes as the total angular momentum is increased, and second, they occur well below the traditional vibrational ergodicity threshold. These peculiar dynamics result from the molecules' unique combination of symmetry, size, and rigidity, highlighting the potential of fullerenes to uncover emergent phenomena in mesoscopic quantum systems.

Quasiperiodically driven fermionic systems can support topological phases not realized in equilibrium. The fermions are localized in the bulk, but support quantized energy currents at the edge. These phases were discovered through an abstract classification, and few microscopic models exist. We develop a coupled layer construction for tight-binding models of these phases in $d\in\{1,2\}$ spatial dimensions, with any number of incommensurate drive frequencies $D$. The models exhibit quantized responses associated with synthetic two- and four-dimensional quantum Hall effects in the steady state. A numerical study of the phase diagram for $(d+D) = (1+2)$ shows: (i) robust topological and trivial phases separated by a sharp phase transition; (ii) charge diffusion and a half-integer energy current between the drives at the transition; and (iii) a long-lived topological energy current which remains present when weak interactions are introduced., Comment: 15 pages, 11 figures; (v2) published version

The dynamical phase diagram of interacting disordered systems has seen substantial revision over the past few years. Theory must now account for a large prethermal many-body localized (MBL) regime in which thermalization is extremely slow, but not completely arrested. We derive a quantitative description of these dynamics in short-ranged one-dimensional systems using a model of successive many-body resonances. The model explains the decay timescale of mean autocorrelators, the functional form of the decay - a stretched exponential - and relates the value of the stretch exponent to the broad distribution of resonance timescales. The Jacobi method of matrix diagonalization provides numerical access to this distribution, as well as a conceptual framework for our analysis. The resonance model correctly predicts the stretch exponents for several models in the literature. Successive resonances may also underlie slow thermalization in strongly disordered systems in higher dimensions, or with long-range interactions., Comment: 7 pages, 3 figures + 9 pages, 9 figures; (v2) additional appendix on the absence of rare region effects, new numerical data for Heisenberg model autocorrelation functions and Floquet model decimated element distributions, other clarifications and corrections

The striking nonlinear effects exhibited by cavity QED systems make them a powerful tool in modern condensed matter and atomic physics. A recently discovered example is the quantized pumping of energy into a cavity by a strongly-coupled, periodically-driven spin. We uncover a remarkable feature of these energy pumps: they coherently translate, or boost, a quantum state of the cavity in the Fock basis. Current optical cavity and circuit QED experiments can realize the required Hamiltonian in a rotating frame. Boosting thus enables the preparation of highly-excited non-classical cavity states in near-term experiments., Comment: 6 pages, 4 figures + 6 pages, 6 figures; (v2) Clarifications on experimental considerations, including an additional appendix on the lab frame evolution

Sufficient disorder is believed to localize static and periodically-driven interacting chains. With quasiperiodic driving by $D$ incommensurate tones, the fate of this many-body localization (MBL) is unknown. We argue that randomly disordered MBL exists for $D=2$, but not for $D\geq 3$. Specifically, a putative two-tone driven MBL chain is neither destabilized by thermal avalanches seeded by rare thermal regions, nor by the proliferation of long-range many-body resonances. For $D\geq 3$, however, sufficiently large thermal regions have continuous local spectra and slowly thermalize the entire chain. En route, we generalize the eigenstate thermalization hypothesis to the quasiperiodically-driven setting, and verify its predictions numerically. Two-tone driving enables new topological orders with edge signatures; our results suggest that localization protects these orders indefinitely., Comment: 15 pages, 4 figures + 6 pages, 4 figures; (v2) Clarifications on synthetic localization

Entanglement is the central resource in adiabatic quantum transport. Dephasing affects the availability of that resource by biasing trajectories, driving transitions between success and failure. This depletion of entanglement is important for the practical implementation of quantum technologies. We present a new perspective on the failure of adiabatic computation by understanding the failure of adiabatic transport as a dynamical phase transition. These ideas are demonstrated in a toy model of adiabatic quantum transport in a two spin system.

We derive a topological classification of the steady states of $d$-dimensional lattice models driven by $D$ incommensurate tones. Mapping to a unifying $(d+D)$-dimensional localized model in frequency space reveals anomalous localized topological phases (ALTPs) with no static analog. While the formal classification is determined by $d+D$, the observable signatures of each ALTP depend on the spatial dimension $d$. For each $d$, with $d+D=3$, we identify a quantized circulating current, and corresponding topological edge states. The edge states for a driven wire ($d=1$) function as a quantized, nonadiabatic energy pump between the drives. We design concrete models of quasiperiodically driven qubits and wires that achieve ALTPs of several topological classes. Our results provide a route to experimentally access higher dimensional ALTPs in driven low-dimensional systems., Comment: 6 pages, 3 figures + 13 pages, 5 figures

A finite length ferromagnetic chain with opposite spin polarisation imposed at its two ends is one of the simplest frustrated spin models. In the clean classical limit the domain wall inserted on account of the boundary conditions resides with equal probability on any one of the bonds, and the degeneracy is precisely equal to the number of bonds. If quantum mechanics is introduced via a transverse field, the domain wall will behave as a particle in a box, and prefer to be nearer the middle of the chain rather than the ends. A simple characteristic of a real quantum annealer is therefore which of these limits obtains in practice. Here we have used the ferromagnetic chain with antiparallel boundary spins to test a real flux qubit quantum annealer and discover that contrary to both expectations, the domain walls found are non-uniformly distributed on account of effective random longitudinal fields present notwithstanding tuning carried out to zero out such fields when the couplings between qubits are nominally zero. We present a simple derivation of the form of the distribution function for the domain walls, and show also how the effect we have discovered can be used to determine the strength of the effective random fields (noise) characterising the annealer. The noise measured in this fashion is smaller than what is seen during the single qubit tuning process, but nonetheless qualitatively affects the outcome of the simulation performed by the annealer., Comment: 14 pages, 9 figures plus supplemental material, title change in v2 and v3, accepted in npj Quantum Information, arXiv matches accepted version

Quasi-periodically driven quantum systems are predicted to exhibit quantized topological properties, in analogy with the quantized transport properties of topological insulators. We use a single nitrogen-vacancy center in diamond to experimentally study a synthetic quantum Hall effect with a two-tone drive. We measure the evolution of trajectories of two quantum states, initially prepared at nearby points in synthetic phase space. We detect the synthetic Hall effect through the predicted overlap oscillations at a quantized fundamental frequency proportional to the Chern number, which characterizes the topological phases of the system. We further observe half-quantization of the Chern number at the transition between the synthetic Hall regime and the trivial regime, and the associated concentration of local Berry curvature in synthetic phase space. Our work opens up the possibility of using driven qubits to design and study higher-dimensional topological insulators and semi-metals in synthetic dimensions.

A spin strongly driven by two harmonic incommensurate drives can pump energy from one drive to the other at a quantized average rate, in close analogy with the quantum Hall effect. The pumping rate is a non-zero integer in the topological regime, while the trivial regime does not pump. The dynamical transition between the regimes is sharp in the zero-frequency limit and is characterized by a Dirac point in a synthetic band structure. We show that the pumping rate is {\em half-integer} quantized at the transition and present universal Kibble-Zurek scaling functions for energy transfer processes. Our results adapt ideas from quantum phase transitions, quantum information and topological band theory to non-equilibrium dynamics, and identify qubit experiments to observe the universal linear and non-linear response of a Dirac point in synthetic dimensions., Comment: 10 pages, 8 figures

We study quantum phase transitions in transverse-field Ising spin chains in which the couplings are random but hyperuniform, in the sense that their large-scale fluctuations are suppressed. We construct a one-parameter family of disorder models in which long-wavelength fluctuations are increasingly suppressed as a parameter $\alpha$ is tuned. For $\alpha = 0$, one recovers the familiar infinite-randomness critical point. For $0 < \alpha < 1$, we find a line of infinite-randomness critical points with continuously varying critical exponents; however, the Griffiths phases that flank the critical point at $\alpha = 0$ are absent at any $\alpha > 0$. When $\alpha > 1$, randomness is a dangerously irrelevant perturbation at the clean Ising critical point, leading to a state we call the critical Ising insulator. In this state, thermodynamics and equilibrium correlation functions behave as in the clean system. However, all finite-energy excitations are localized, thermal transport vanishes, and autocorrelation functions remain finite in the long-time limit. We characterize this line of hyperuniform critical points using a combination of perturbation theory, renormalization-group methods, and exact diagonalization., Comment: 20 pages, 22 figures

Few level quantum systems driven by $n_\mathrm{f}$ incommensurate fundamental frequencies exhibit temporal analogues of non-interacting phenomena in $n_\mathrm{f}$ spatial dimensions, a consequence of the generalisation of Floquet theory in frequency space. We organise the fundamental solutions of the frequency lattice model for $n_\mathrm{f}=2$ into a quasi-energy band structure and show that every band is classified by an integer Chern number. In the trivial class, all bands have zero Chern number and the quasi-periodic dynamics is qualitatively similar to Floquet dynamics. The topological class with non-zero Chern bands has dramatic dynamical signatures, including the pumping of energy from one drive to the other, chaotic sensitivity to initial conditions, and aperiodic time dynamics of expectation values. The topological class is however unstable to generic perturbations due to exact level crossings in the quasi-energy spectrum. Nevertheless, using the case study of a spin in a quasi-periodically varying magnetic field, we show that topological class can be realised at low frequencies as a pre-thermal phase, and at finite frequencies using counter-diabatic tools., Comment: 22 Pages, 15 Figures

We study ground states and elementary excitations of a system of bosonic atoms and diatomic Feshbach molecules trapped in a one-dimensional optical lattice using exact diagonalization and variational Monte Carlo methods. We primarily study the case of an average filling of one boson per site. In agreement with bosonization theory, we show that the ground state of the system in the thermodynamic limit corresponds to the Pfaffian-like state when the system is tuned towards the superfluid-to-Mott insulator quantum phase transition. Our study clarifies the possibility of the creation of exotic Pfaffian-like states in realistic one-dimensional systems. We also present preliminary evidence that such states support non-Abelian anyonic excitations that have potential application for fault-tolerant topological quantum computation., Comment: 10 pages, 10 figures. Matching the version published Phys.Rev.B

We derive a microscopic model for dissipative dynamics in a system of mutually interacting qubits coupled to a thermal bath that generalises the dissipative model of Landau-Lifschitz-Gilbert to the case of anisotropic bath couplings. We show that the dissipation acts to bias the quantum trajectories towards a reduced phase space. This model applies to a system of superconducting flux qubits whose coupling to the environment is necessarily anisotropic. We study the model in the context of the D-Wave computing device and show that the form of environmental coupling in this case produces dynamics that are closely related to several models proposed on phenomenological grounds., Comment: 12 pages, 10 figures

Subtracting photons from a two-mode squeezed state is a well-known method to increase entanglement. We analyse different strategies of local photon subtraction from a two-mode squeezed state in terms of entanglement gain and success probability. We develop a general framework that incorporates imperfections and losses in all stages of the process: before, during, and after subtraction. By combining all three effects into a single efficiency parameter, we provide analytical and numerical results for subtraction strategies using photon-number-resolving and threshold detectors. We compare the entanglement gain afforded by symmetric and asymmetric subtraction scenarios across the two modes. For a given amount of loss, we identify an optimised set of parameters, such as initial squeezing and subtraction beam splitter transmissivity, that maximise the entanglement gain rate. We identify regimes for which asymmetric subtraction of different Fock states on the two modes outperforms symmetric strategies. In the lossless limit, subtracting a single photon from one mode always produces the highest entanglement gain rate. In the lossy case, the optimal strategy depends strongly on the losses on each mode individually, such that there is no general optimal strategy. Rather, taking losses on each mode as the only input parameters, we can identify the optimal subtraction strategy and required beam splitter transmissivities and initial squeezing parameter. Finally, we discuss the implications of our results for the distillation of continuous-variable quantum entanglement., Comment: 13 pages, 11 figures. Updated version for publication

Interferometry with quantum light is known to provide enhanced precision for estimating a single phase. However, depending on the parameters involved, the quantum limit for the simultaneous estimation of multiple parameters may not attainable, leading to trade-offs in the attainable precisions. Here we study the simultaneous estimation of two parameters related to optical interferometry: phase and loss, using a fixed number of photons. We derive a trade-off in the estimation of these two parameters which shows that, in contrast to single-parameter estimation, it is impossible to design a strategy saturating the quantum Cramer-Rao bound for loss and phase estimation in a single setup simultaneously. We design optimal quantum states with a fixed number of photons achieving the best possible simultaneous precisions. Our results reveal general features about concurrently estimating Hamiltonian and dissipative parameters, and has implications for sophisticated sensing scenarios such as quantum imaging., Comment: 9 pages, 6 figures