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The Aristarchus plateau represents one of the most complex volcanic provinces on the lunar surface and is host to the largest pyroclastic deposit on the Moon. Lunar pyroclastic deposits offer a window into the Moon’s interior and represent a valuable resource to support a sustained human presence. We present a new analysis of the Aristarchus pyroclastic deposit using Mini-RF bistatic radar data at wavelengths of 4.2 and 12.6 cm. Building on previous Earth-based Arecibo Observatory radar studies at 12.6 and 70 cm, we place further constraints on the spatial extent of the pyroclastic deposit and investigate the clast size distribution and provenance of foreign material distributed within the formation. Concentrations of blocky material >0.5 cm in diameter and suspended within the upper decimeters of the pyroclastic deposit are associated with potential buried mare flows along the rim of Vallis Schröteri and discrete pockets of primary material ejected by the Aristarchus impact. Unraveling the deposit from nonpyroclastic materials and the surrounding landscape creates new constraints with which to reconstruct the volcanic history of the region. From a future mission perspective, the identification of primary Aristarchus material distributed across the plateau offers an opportunity to sample diverse volcanic lithologies within an area that could be sampled by a single Commercial Lunar Payload Services mission. In terms of lunar resource in situ utilization, such ejected material also represents a contaminant; thus, radar data provide an invaluable tool to identify pristine pyroclastic material for mission planners.