Search

In this paper, an experimental study on generation of nanoparticle various sizes using Ti:sapphire laser pulses, is reported. Nanoparticle formation in plasma plumes of metals like silver and copper, expanding in vacuum, has been studied using stretched pulses of 300 ps duration [subnanoseconds (sub-ns)] from a Ti:sapphire laser. It has been compared with the nanoparticle formation (of the same materials) when compressed pulses of 45 fs duration were used under similar focusing conditions. Nanoparticle formation is observed at intensities as high as 2×1016 W/cm2. The structural analysis of the nanoparticle deposition on a silicon substrate showed that, using 45 fs pulses, smaller nanoparticles of average size ∼20 nm were generated, whereas on using the sub-ns pulses, larger particles were produced. Also, the visible light transmission and reflection from the nanoparticle film of Ag on glass substrate showed surface plasmon resonance (SPR). The SPR curves of the films of nanoparticles deposited by femtosecond pulses were always broader and reflection/transmission was always smaller when compared with the films formed using the sub-ns pulses, indicating smaller size particle formation by ultrashort pulses. Thus, it has been demonstrated that variation in the laser pulse duration of laser offers a simple tool for varying the size of the nanoparticles generated in plasma plumes. [ABSTRACT FROM AUTHOR]

The morphologies of the fullerene targets and the ablated fullerenes to determine the optimal conditions of excitation of the C60-containing targets have been analyzed. The optimization of fullerene-containing plasma conditions allowed the enhanced harmonic generation in these plasmas using laser radiation of different wavelengths, pulse durations, and phase modulation. A comparison between the harmonic generation in single-atom/ion-containing plasmas (using bulk carbon, silver, and indium targets) and fullerene-rich plasma plumes showed better conversion efficiency for the latter medium. The influence of phase modulation of the fundamental radiation in fullerene plasmas on the spectral properties of harmonics has been studied. [ABSTRACT FROM AUTHOR]

The dependence of the high-order harmonic intensity on the laser focal spot position in laser produced plasma plumes is experimentally studied. High order harmonics up to the 59th order (λ∼13.5 nm) were generated by focusing 48 fs laser pulses from a Ti:sapphire laser system in silver plasma plume produced using 300 ps uncompressed laser radiation as the prepulse. The intensity of harmonics nearly vanished when the best focus was located in the plume center, whereas it peaked on either side with unequal intensity. The focal spot position corresponding to the peak harmonic intensity moved away from the plume center for higher order harmonics. The results are explained in terms of the variation of phase mismatch between the driving laser beam and harmonics radiation produced, relativistic drift of electrons, and defocusing effect due to radial ionization gradient in the plasma for different focal spot positions. [ABSTRACT FROM AUTHOR]

An experimental study on hard x-ray Bremsstrahlung radiation due to fast electron generation from a planar solid copper target irradiated by 150 mJ, 45 fs Ti:sapphire laser pulses at I∼1018 W/cm2 is reported. Angular distribution of the hard x-ray dose rate (hν≥40 keV) is observed to be strongly forward peaked in the direction of target normal with a measured peak value of 40 μSv/h, at a distance of 500 mm from the target. Two sources of this radiation, one at the laser irradiated target and the other at the chamber wall facing the target, are inferred from the measurements of angular distribution and distance dependence of the x-ray dose rate. [ABSTRACT FROM AUTHOR]

An experimental study of parametric dependence of space-resolved x-ray line emission from laser-produced magnesium plasma expanding in a helium background gas has been performed for different pressures up to 125 mbar. A strong enhancement in MgXI He-α resonance (1s² ¹S[sub 0]-1 s2p ¹P[sub 1] at 9.17 Å) and intercombination (1s² ¹S[sub 0]-1 s2p ³P[sub 1] at 9.23 Å) line emission is observed in the expansion region extending up to ∼6 mm from the target. At the optimum background gas pressure of about 40 mbar, there is an order of magnitude increase in the x-ray line intensity compared to that observed for a gas pressure of few mbar. The results of measurements of the distance of the peak emission region from the target and width of the emission zone for different pressures are presented, and the role of the background gas for the observed behavior is discussed. [ABSTRACT FROM AUTHOR]

A diagnostic system to detect electrical faults inside a coaxial high current discharge device is presented here. This technique utilizes two biconical antennas picking up electromagnetic radiation from the discharge device, a voltage divider sensing input voltage, and a Rogowski coil measuring the main discharge current. A computer program then analyses frequency components in these signals and provides information as to whether the discharge event was normal or any breakdown fault occurred inside the coaxial device. The diagnostic system is developed for a 450 kV and 50 kA capillary discharge plasma setup. For the setup various possible faults are analyzed by electrical simulation, followed by experimental results. In the case of normal discharge through the capillary load the dominant frequency is ∼4 MHz. Under faulty conditions, the peak in magnitude versus frequency plot of the antenna signal changes according to the fault position which involves different paths causing variation in the equivalent circuit elements. [ABSTRACT FROM AUTHOR]

The Laser Plasma Division at the Centre for Advanced Technology is engaged in a variety of research and development activities on laser-plasma interaction with special emphasis on laser-matter interaction at ultra-high intensities. An important aspect of our future work is studies in laser-plasma based acceleration using an elaborate infrastructural set-up of ultra-fast laser and plasma diagnostic systems and recently acquired 10TW, 50fs Ti:Sapphire laser system. This paper presents outline of the planned studies in this field. [ABSTRACT FROM AUTHOR]

Experimental measurements of ablation parameters in a KrF laser produced aluminum plasma are presented for the laser intensity range of 10[sup 11]-10[sup 13] W/cm². Plasma created from large focal spots shows single broad ion current pulses as compared to two groups of ions observed from small focal spots. Detailed analysis of the velocity distributions of emitted ions is carried out to understand this behavior and its effect on measurements of the ablation parameters. Scalings with laser intensity of the mass ablation rate (m ∼ I[sup 0.42, sub L]) and of the ablation pressure (P[sub a] ∼ I[sup 0.81, sub L) 8 - IL') giving m = 1.5 × 10[sup 5] g cm[sup -2] sec[sup -1] and P[sup a] = 5.5 Mbar at a laser intensity of 10[sup 13] W/cm² are obtained. The results are found to be in good agreement with the predictions of a plasma ablation model based on inverse bremsstrahlung dominated absorption. [ABSTRACT FROM AUTHOR]

The dynamics of ultrashort laser plasmas demand single shot temporal measurements on fast time scales. We describe a method to record the plasma expansion on picosecond (ps) timescales continuously over hundreds of ps, in single shot. The method uses the chirp of a Ti:sapphire laser as a time-resolved optical diagnostic tool. Using this technique, the evolution of the plasma expansion had been recorded with ps time resolutions, by probing with a chirped laser pulse of 200 ps duration. A peak expansion velocity of 1.8×107 cm/s is observed and its evolution in time is obtained for ∼300 ps. [ABSTRACT FROM AUTHOR]