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The combinations of artificial intelligence and lasers provide powerful ways to form smart light sources with ground-breaking functions. Here, a Raman fiber laser (RFL) with reconfigurable and programmable spectra in an ultra-wide bandwidth is developed based on spectral-spatial manipulation of light in multimode fiber (MMF). The proposed fiber laser uses nonlinear gain from cascaded stimulated Raman scattering, random distributed feedback from Rayleigh scattering, and point feedback from an MMF-based smart spectral filter. Through wavefront shaping controlled by a genetic algorithm, light of selective wavelength(s) can be focused in the MMF, forming the filter that, together with the active part of the laser, actively shape the output spectrum with a high degree of freedom. We achieved arbitrary spectral shaping of the cascaded RFL (e.g., continuously tunable single-wavelength and multi-wavelength laser with customizable linewidth, mode separation, and power distribution) from the 1st- to the 3rd-order Stokes emission by adjusting the pump power and auto-optimization of the smart filter. Our research uses artificial-intelligence controlled light manipulation in a fiber platform with multi-eigenmodes and nonlinear gain, mapping the spatial control into the spectral domain as well as extending the linear control of light in MMF to active light emission, which is of great significance for applications in optical communication, sensing, and spectroscopy., Comment: 10 pages,6 figures

Refractive index enhancement is crucial in the field of lithography, imaging, optical communications, solar devices and many more. We present a review of advancements in the process of designing high refractive index metamaterials, starting from quantum coupling and photonic bandgap materials to metamaterials utilizing deep subwavelength coupling to achieve ever-high values of refractive index. A crisp and critical impression of each scheme are presented. The understanding of evolution of material design from intrinsic electronic states manipulation to meta-atoms design is not only fascinating but prerequisite to developing successful devices and applications.

Using metasurfaces to control the wave propagation at will has been very successful over the broad electromagnetic spectrum in recent years. By encoding specially designed abrupt changes of electromagnetic parameters into metasurfaces, such as phase and amplitude, nearly arbitrary control over the output wavefronts could be realized. Constituted by a single- or fewlayer of planar structures, metasurfaces are straightforward in design and fabrication, thus promising many realistic applications. Moreover, such control concept can be further extended to the surface wave regime. In this review, we present our recent progress on metasurfaces capable of tailoring the propagation of both free-space and surface terahertz waves. Following an introduction of the basic concept and theory, a number of unique terahertz metasurfaces are presented, showing the ability in devising ultra-thin and compact functional terahertz components.

Ultrasensitive terahertz sensing of highly absorptive aqueous solutions remains challenging due to strong absorption of water in the terahertz regime. Here, we experimentally demonstrate a cost-effective metamaterial-based sensor integrated with terahertz time-domain spectroscopy for highly absorptive water-methanol mixture sensing. This metamaterial has simple asymmetric wire structures that support multiple resonances including a fundamental Fano resonance and higher order dipolar resonance in the terahertz regime. Both the resonance modes have strong intensity in the transmission spectra which we exploit for detection of the highly absorptive water-methanol mixtures. The experimentally characterized sensitivities of the Fano and dipole resonances for the water-methanol mixtures are found to be 160 and 305 GHz/RIU, respectively. This method provides a route for readily available metamaterial-assisted terahertz spectroscopy for ultrasensitive sensing of highly absorptive chemical and biochemical materials with multiple resonances and high accuracy.

We report extensive enhancement in the refractive index of artificially designed metamaterials by exploiting the deep subwavelength coupling in a free-standing, thin-film metal-dielectric-metal checkboard structure. A record high refractive index of 77.02+43.22i is obtained at terahertz frequencies. The detailed investigations reveal that the enhancement of the effective refractive index of the structure via deep subwavelength coupling in a bilayer design is governed by a power law, which is an effective and simpler approach to design high index metamaterial. The approach relies on deep subwavelength coupling to obtain extremely high refractive index values that can lead to many practical applications in the field of imaging, lithography, design of delay lines and interferometers.

Losses are ubiquitous and unavoidable in nature inhibiting the performance of most optical processes. Manipulating losses to adjust the dissipation of photons is analogous to braking a running car that is as important as populating photons via a gain medium. Here, we introduce the transient loss boundary into a photon populated cavity that functions as a photon brake and probe photon dynamics by engineering the brake timing and brake strength. Coupled cavity photons can be distinguished by stripping one photonic mode through controlling the loss boundary, which enables the transition from a coupled to an uncoupled state. We interpret the transient boundary as a perturbation by considering both real and imaginary parts of permittivity, and the dynamic process is modelled with a temporal two-dipole oscillator, one with the natural resonant polarization and the other with a frequency-shift polarization. The model unravels the underlying mechanism of concomitant coherent spectral oscillations and generation of tone-tuning cavity photons in the braking process. By synthesizing the temporal loss boundary into a photon populated cavity, a plethora of interesting phenomena and applications are envisioned such as the observation of quantum squeezed states, low-loss nonreciprocal waveguides and ultrafast beam scanning devices., Comment: 18 pages,5 figures,accepted in Nature Communications

Superluminal tunneling of light through a barrier has attracted broad interest in the last several decades. Despite the observation of such phenomena in various systems, it has been under intensive debate whether the transmitted light truly carry the information of the original pulse. Here we report observation of anomalous time response for terahertz electromagnetic pulses passing through thin metal films, with the pulse shape of the transmitted beam faithfully resembling that of the incident beam. A causal theoretical analysis is developed to explain the experiments, though the theory of Special Relativity may confront a challenge in this exceptional circumstance. These findings may facilitate future applications in high-speed optical communication or signal transmission, and may reshape our fundamental understanding about the tunneling of light., Comment: 16 pages, 9 figures. To be submitted to PHYSICAL REVIEW LETTERS

Recent breakthroughs in solid-state photonic quantum technologies enable generating and detecting single photons with near-unity efficiency as required for a range of photonic quantum technologies. The lack of methods to simultaneously generate and control photons within the same chip, however, has formed a main obstacle to achieving efficient multi-qubit gates and to harness the advantages of chip-scale quantum photonics. Here we propose and demonstrate an integrated voltage-controlled phase shifter based on the electro-optic effect in suspended photonic waveguides with embedded quantum emitters. The phase control allows building a compact Mach-Zehnder interferometer with two orthogonal arms, taking advantage of the anisotropic electro-optic response in gallium arsenide. Photons emitted by single self-assembled quantum dots can be actively routed into the two outputs of the interferometer. These results, together with the observed sub-microsecond response time, constitute a significant step towards chip-scale single-photon-source de-multiplexing, fiber-loop boson sampling, and linear optical quantum computing., Comment: 7 pages, 4 figues + supplementary information

Manipulating the polarisation of light is crucial for sensing and imaging applications. One such aspect in particular is selective transmission of one circular polarisation (spin) when light is transmitted through a medium or a device. However, most present methods of achieving this have relatively low efficiency and selectivity, whilst high selectivity examples rely on lossy and complex three-dimensional helical or multilayer structures. Here, we propose a dielectric metamaterial approach for achieving spin-selective transmission of electromagnetic waves, utilizing spin-controlled constructive or destructive interference between two Pancharatnam-Berry (PB) phases in conjunction with propagative dynamic phase. The dielectric metamaterial, consisting of monolithic silicon herringbone structures, exhibits a broadband operation in the terahertz regime whilst obtaining a spin-selective efficiency upwards of 60%. Such a device is robust and is not easily degraded by errors in fabrication., Comment: 15 pages, 4 figures, Advanced Materials, first published: 14 September 2016

We propose and experimentally demonstrate that a metasurface consisting of Pancharatnam-Berry phase optical elements can enable the full control of optical spin-to-orbital angular momentum conversion. Our approach relies on the critical interference between the transmission and reflection upon the metasurfaceto create actively tunable and controllable conversion with a high output via coherent control of the two incident beams. The introduced control methodology is general and could be an important step toward the development of functional optical devices for practical applications., Comment: 22 pages, 4 figures

Metamaterials based on effective media have achieved a lot of unusual physics (e.g. negative refraction and invisibility cloaking) owing to their abilities to tailor the effective medium parameters that do not exist in nature. Recently, coding metamaterials have been suggested to control electromagnetic waves by designing the coding sequences of digital elements '0' and '1', which possess opposite phase responses. Here, we propose the concept of anisotropic coding metamaterial at terahertz frequencies, in which coding behaviors in different directions are dependent on the polarization status of terahertz waves. We experimentally demonstrate an ultrathin and flexible polarization-controlled anisotropic coding metasurface functioning in the terahertz regime using specially- designed coding elements. By encoding the elements with elaborately-designed digital sequences (in both 1 bit and 2 bits), the x- and y-polarized reflected waves can be deflected or diffused independently in three dimensions. The simulated far-field scattering patterns as well as near-electric-field distributions are given to illustrate the bifunctional performance of the encoded metasurface, which show good agreement to the measurement results. We further demonstrate the abilities of anisotropic coding metasurface to generate beam splitter and realize anomalous reflection and polarization conversion simultaneously, providing powerful controls of differently-polarized terahertz waves. The proposed method enables versatile beam behaviors under orthogonal polarizations using a single metasurface, and hence will promise interesting terahertz devices.

We experimentally study the effect of near field coupling on the transmission of light in terahertz metasurfaces, possessing slightly distinctive SRR resonances. Our results show that the interplay between the strengths of electric and magnetic dipoles, modulates the amplitude of resulting electromagnetically induced transmission, probed under different types of asymmetries in the coupled system. We employ a two-particle model to theoretically study the influence of the near field coupling between bright and quasi-dark modes on the transmission properties of the coupled system and we find an excellent agreement with our observed results. Adding to the enhanced transmission characteristics, our results provide a deeper insight into the metamaterial analogues of atomic electromagnetically induced transparency and offer an approach to engineer slow light devices, broadband filters and attenuators at terahertz frequencies.

High quality factor resonances are extremely promising for designing ultra-sensitive refractive index label-free sensors since it allows intense interaction between electromagnetic waves and the analyte material. Metamaterial and plasmonic sensing has recently attracted a lot of attention due to subwavelength confinement of electromagnetic fields in the resonant structures. However, the excitation of high quality factor resonances in these systems has been a challenge. We excite an order of magnitude higher quality factor resonances in planar terahertz metamaterials that we exploit for ultrasensitive sensing. The low-loss quadrupole and Fano resonances with extremely narrow linewidths enable us to measure the minute spectral shift caused due to the smallest change in the refractive index of the surrounding media. We achieve sensitivity levels of 7.75 x 10^3 nm/ RIU with quadrupole and 5.7 x 10^4 nm/ RIU with the Fano resonances which could be further enhanced by using thinner substrates. These findings would facilitate the design of ultrasensitive real time chemical and biomolecular sensors in the fingerprint region of the terahertz regime., Comment: 10 pages, 6 figures

Invisibility cloaking not only catches the human imagination, but also promises fascinating applications in optics and photonics. By manipulating electromagnetic waves with metamaterials, researchers have been able to realize electromagnetic cloaking in the microwave, terahertz and optical regimes. Nevertheless, the complex design and fabrication process, narrow bandwidth, and high intrinsic losses in the metamaterial-based cloaks have imposed intractable limitations on their realistic applications. Seeking new approaches to overcome these perceived disadvantages is in progress. Here by using uniform sapphire crystal, we demonstrate the first homogenous invisibility cloak functioning at terahertz frequencies. The terahertz invisibility device features a large concealed volume, low loss, and broad bandwidth. In particular, it is capable of hiding objects with a dimension nearly an order of magnitude larger than that of its lithographic counterpart, but without involving complex and time-consuming cleanroom processing. Such homogenous invisibility cloaks may lead to novel terahertz photonic devices potentially used in medicine, radars, and communications., Comment: 17 pages, 7 figures

The invisibility cloak has been a long-standing dream for many researchers over the decades. The introduction of transformational optics has revitalized this field by providing a general method to design material distributions to hide the subject from detection. By transforming space and light propagation, a three-dimensional (3D) object is perceived as having a reduced number of dimensions, in the form of points, lines, and thin sheets, making it "undetectable" judging from the scattered field. Although a variety of cloaking devices have been reported at microwave and optical frequencies, the spectroscopically important Terahertz (THz) domain remains unexplored. Moreover, due to the difficulties in fabricating cloaking devices that are optically large in all three dimensions, hiding realistic 3D objects has yet to be demonstrated. Here, we report the first experimental demonstration of a 3D THz cloaking device fabricated using a scalable Projection Microstereolithography process. The cloak operates at a broad frequency range between 0.3 and 0.6 THz, and is placed over an {\alpha}- lactose monohydrate absorber with rectangular shape. Characterized using angularresolved reflection THz time-domain spectroscopy (THz-TDS), the results indicate that the THz invisibility cloak has successfully concealed both the geometrical and spectroscopic signatures of the absorber, making it undetectable to the observer.

We study ways to enhance the sensitivity and dynamic tuning range of the fundamental inductor-capacitor (LC) resonance in split ring resonators (SRRs) by controlling the aspect ratio of the SRRs and their substrate thickness. We conclude that both factors can significantly affect the LC resonance. We show that metafilms consisting of low height SRRs on a thin substrate are most sensitive to changes in their dielectric environment and thus show excellent potential for sensing applications., Comment: 4 pages with 4 figures

We investigate the response of terahertz metamaterials made of split-ring resonators depending on the unit cell density. It is shown that the fundamental resonance has its highest Q factor for a period of one-third the resonance wavelength. Increasing or decreasing the period from that optimal period reduces the Q factor. All observations are explained by understanding radiative coupling as the dominant loss mechanism at low densities, whereas the strong inter SRR coupling enhances non-radiative losses at high densities. Our results allow designing metamaterials with adjustable Q factors and possibly suggesting that an optimal package density exists to induce the strongest dispersion., Comment: 7 pages, 4 figures

Using terahertz time domain spectroscopy we demonstrate tunable polarization rotation and circular dichroism in intrinsically nonchiral planar terahertz metamaterials without twofold rotational symmetry. The observed effect is due to extrinsic chirality arising from the mutual orientation of the metamaterial plane and the propagation direction of the incident terahertz wave., Comment: 6 pages, 4 figures

We report an experimental observation of three distinct resonances in split ring resonators (SRRs) for both vertical and horizontal electric field polarizations at normal incidence by use of terahertz time domain spectroscopy. Breaking the symmetry in SRRs by gradually displacing the capacitive gap from the center towards the corner of the ring allows for an 85% modulation of the fundamental inductive-capacitive resonance. Increasing asymmetry leads to the evolution of an otherwise inaccessible high quality factor electric quadrupole resonance that can be exploited for bio-sensing applications in the terahertz region., Comment: 8 pages, 5 figures

We demonstrate thermally tunable superconductor hole array with active control over their resonant transmission induced by surface plasmon polaritons . The array was lithographically fabricated on high temperature YBCO superconductor and characterized by terahertz-time domain spectroscopy. We observe a clear transition from the virtual excitation of the surface plasmon mode to the real surface plasmon mode. The highly tunable superconducting plasmonic hole arrays may have promising applications in the design of low-loss, large dynamic range amplitude modulation, and surface plasmon based terahertz devices., Comment: 3 figures

We characterize the behaviour of split ring resonators made up of high-transition temperature YBCO superconductor using terahertz time domain spectroscopy. The superconductor metamaterial shows sharp change in the transmission spectrum at the fundamental inductive-capacitive resonance and the dipole resonance as the temperature dips below the transition temperature. Our results reveal that the high performance of such a metamaterial is limited by material imperfections and defects such as cracks, voids and secondary phases which play dominant role in partially impeding the flow of current causing dissipation of energy and electrical resistance to appear in the superconductor film., Comment: 6 pages, 3 figures

The invisibility cloak has been a long-standing dream for many researchers over the decades. By transforming space and light propagation, a three-dimensional (3D) object can be perceived as having reduced number of dimensions, in the form of points, lines, and thin sheets, making it "undetectable" judging from scattered field. Although a variety of cloaking devices have been reported at microwave and optical frequencies, the Terahertz (THz) domain remains unexplored. Moreover, it should be noted that all the previous experimental demonstrations are performed in a two-dimensional (2D) waveguide configuration. Although those works represent a critical step in validating the concept of the invisibility cloak, one would expect the cloaking device to be realized in 3D with the ability to cloak an object of realistic size. This requires the construction of an optically large cloaking device with features much smaller than the wavelength. Fabricating 3D structures with aspect ratio close to 100:1 is obviously a challenging task. Here, we report an experimental demonstration of a 3D THz ground plane cloak. Reflection terahertz time-domain spectroscopy (THz-TDS) was employed to characterize the cloaking samples. Two distinct reflection peaks can be clearly observed across a broad frequency range, which is caused by the reflection at the surface of the bump. The measured peak positions are consistent with the numerical simulation peak positions. By contrast, in the spectral map of the cloak sample, the wavefront is relatively smooth with a single peak.

Optical properties of planar thin film metamaterials were measured at room and liquid nitrogen temperatures using terahertz time-domain spectroscopy. The operation of metamaterials at cryogenic temperatures is anticipated to be a promising path towards low-loss metamaterials since nonradiative losses are strongly suppressed due to higher charge mobility. A 14% increase in the quality factor of the resonances was experimentally observed. It was limited by the high electron scattering rate due to defects in thin films. Supplementary simulations assuming metamaterials made of thick films reveal a temperature controlled behaviour and a 40% increase of the Q-factor at 10 K., Comment: 6 pages, 4 figures

Using terahertz time domain spectroscopy we investigate the normal incidence transmission through periodically and randomly arranged planar split ring resonators (SRRs). Introduction of positional disorder in metamaterials has no effect on the quality factor of the fundamental Inductive-Capacitive (LC) resonance. The dipole resonances undergo broadening and shift in their resonance frequencies. The experiment reveals that the randomly distributed SRR structures interact incoherently at LC resonance but couple coherently at the higher frequency dipole resonance.

We experimentally demonstrate at terahertz frequencies that a planar metamaterial exhibits a spectral response resembling electromagnetically induced transparency. The metamaterial unit cell consists of a split ring surrounded by another closed ring where their dimensions are such that their excitable lowest order modes have identical resonance frequencies but very different life times. Terahertz time-domain spectroscopy verifies that the interference of these two resonances results in a narrow transparency window located within a broad opaque region. In contrast to previous studies this enhanced transmission is achieved by independently exciting two resonances in which their coupling to the radiation field, and thus their linewidth, differs strongly. Rigorous numerical simulations prove that the transparency window is associated with a large group index and low losses, making the design potentially useful for slow light applications. This experiment opens an avenue to explore quantum mechanical phenomena using localized resonances in metallic structures

Terahertz time domain spectroscopy and rigorous simulations are used to probe the coupling between a dark and a bright plasmonic eigenmode in a metamaterial with broken symmetry. The metamaterial consists of two closely spaced split ring resonators that have their gaps in non-identical positions within the ring. For normal incidence and a fixed polarization both lowest order eigenmodes of the split ring resonators can be excited; although one of them has to be regarded as dark since coupling is prohibited because of symmetry constraints. Emphasis in this work is put on a systematic evaluation of the coupling effects depending on a spectral tuning of both resonances.

Negative index metamaterials (NIMs) give rise to unusual and intriguing properties and phenomena, which may lead to important applications such as superlens, subwavelength cavity and slow light devices. However, the negative refractive index in metamaterials normally requires a stringent condition of simultaneously negative permittivity and negative permeability. A new class of negative index metamaterials - chiral NIMs, have been recently proposed. In contrast to the conventional NIMs, chiral NIMs do not require the above condition, thus presenting a very robust route toward negative refraction. Here we present the first experimental demonstration of a chiral metamaterial exhibiting negative refractive index down to n=-5 at terahertz frequencies, with only a single chiral resonance. The strong chirality present in the structure lifts the degeneracy for the two circularly polarized waves and relieves the double negativity requirement. Chiral NIM are predicted to possess intriguing electromagnetic properties that go beyond the traditional NIMs, such as opposite signs of refractive indices for the two circular polarizations and negative reflection. The realization of terahertz chiral NIMs offers new opportunities for investigations of their novel electromagnetic properties, as well as important terahertz device applications., Comment: 15 pages, 4 figures