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A laser pulse composed of a fundamental and an appropriately phased second harmonic can drive a time-dependent current of photoionized electrons that generates broadband THz radiation. Over the propagation distances relevant to many experiments, dispersion causes the relative phase between the harmonics to evolve. This "dephasing" slows the accumulation of THz energy and results in a multi-cycle THz pulse with significant angular dispersion. Here, we introduce a novel optical configuration that compensates the relative phase evolution, allowing for the formation of a half-cycle THz pulse with almost no angular dispersion. The configuration uses the spherical aberration of an axilens to map a prescribed radial phase variation in the near field to a desired longitudinal phase variation in the far field. Simulations that combine this configuration with an ultrashort flying focus demonstrate the formation of a half-cycle THz pulse with a controlled emission angle and 1/4 the angular divergence of the multi-cycle pulse created by a conventional optical configuration.

Ultrafast laser irradiation can induce spontaneous self-organization of surfaces into dissipative structures with nanoscale reliefs. These surface patterns emerge from symmetry-breaking dynamical processes that occur in Rayleigh-B\'enard-like instabilities. In this study, we demonstrate that the coexistence and competition between surface patterns of different symmetries in two dimensions can be numerically unraveled using the stochastic generalized Swift-Hohenberg model. We originally propose a deep convolutional network to identify and learn the dominant modes that stabilize for a given bifurcation and quadratic model coefficients. The model is scale-invariant and has been calibrated on microscopy measurements using a physics-guided machine learning strategy. Our approach enables the identification of experimental irradiation conditions for a desired self-organization pattern. It can be applied generally to predict structure formation in situations where the underlying physics can be approximately described by a self-organization process and data is sparse and non-time series. Our work paves the way for supervised local manipulation of matter using timely-controlled optical fields in laser manufacturing.

"Flying focus" techniques produce laser pulses with dynamic focal points that travels distances much greater than a Rayleigh length. The implementation of these techniques in laser-based applications requires the design of optical configurations that can both extend the focal range and structure the radial group delay. This article describes a method for designing optical configurations that produce ultrashort flying focus pulses with arbitrary-trajectory focal points. The method is illustrated by several examples that employ an axiparabola for extending the focal range and either a reflective echelon or a deformable mirror-spatial light modulator pair for structuring the radial group delay. The latter configuration enables rapid exploration and optimization of flying foci, which could be ideal for experiments.

A laser pulse composed of a fundamental and properly phased second harmonic exhibits an asymmetric electric field that can drive a time-dependent current of photoionized electrons. The current produces an ultrashort burst of terahertz (THz) radiation. When driven by a conventional laser pulse, the THz radiation is emitted into a cone with an angle determined by the dispersion of the medium. Here we demonstrate that the programmable-velocity intensity peak of a spatiotemporally structured, two-color laser pulse can be used to control the emission angle, focal spot, and spectrum of the THz radiation. Of particular interest for applications, a structured pulse with a subluminal intensity peak can drive highly focusable, on-axis THz radiation.

10 {\mu}m lasing is studied in a compact CO2-He cell pressurized up to 15 atm when optically pumped by a ~50 mJ Fe:ZnSe laser tunable around 4.3 {\mu}m. The optimal pump wavelength and partial pressure of CO2 for generating 10 {\mu}m pulses are found to be ~4.4 {\mu}m and 0.75 atm, respectively. Without cavity optimization, the optical-to-optical conversion efficiency reached ~10% at a total pressure of 7 atm. The gain lifetime is measured to be ~1 {\mu}s at pressures above 10 atm, indicating the feasibility of using high-pressure optically pumped CO2 for the efficient amplification of picosecond 10 {\mu}m pulses., Comment: 10 pages, 8 figures

The resonant nonlinear refraction of 4-5 $\mu$m light in CO and CO$_2$ gas at a peak intensity of 15 MW/cm$^2$ was demonstrated using time- and frequency-resolved measurements of self-focusing and self-defocusing. The nonlinearity of these molecular gases exhibits intensity-dependent sign reversals and a < 4 ns response time. A change from self-focusing to self-defocusing or vice-versa was observed to occur for Rabi frequencies that are comparable to the collisional linewidth. A density matrix model for the nonlinear susceptibility of a strongly driven two-level system provides a qualitative explanation for these results.

We study the necessary condition under which a resonantly driven exciton polariton superfluid flowing against an obstacle can generate turbulence. The value of the critical velocity is well estimated by the transition from elliptic to hyperbolic of an operator following ideas developed by Frisch, Pomeau, Rica for a superfluid flow around an obstacle, though the nature of equations governing the polariton superfluid is quite different. We find analytical estimates depending on the pump amplitude and on the pump energy detuning, quite consistent with our numerical computations.

We show that weakly incoherent optical beams propagating in a Kerr medium exhibit a universal algebraic coherence after a short propagation time, mimicking the quasi-long-range order of ultracold quantum Bose gases in two dimensions. If two plates are inserted in the medium, this optical quasi-condensate gives rise to a long-range Casimir-like force, attractive at large distances and repulsive at short distances., Comment: Published version

An approach for the optimization and synthesis of a phase-only faceted Fresnel type diffractive optical element (FDOE) generating 3D virtual images is proposed. The FDOE is a transmissive Fresnel type DOE array, which produces the perception of a customized floating 3D virtual image behind the FDOE when illuminated with a divergent monochromatic Light Emitter Diode (LED) source. Each DOE unit of the FDOE is optimized with a modified iterative Fourier transform algorithm (M-IFTA). Each unit of the FDOE locally deflects the incident light to the same position to form a designated view of the target plane. The FDOE is fabricated using our home-built parallel write photo-lithography machine. Numerical simulations and optical experiments are performed to verify the proposed design method. Photos of the generated image are also presented. This work can find applications in optical security, anti-counterfeiting, and holographic display.

We report on a versatile method to compensate the linear attenuation in a medium, independently of its microscopic origin. The method exploits diffraction-limited Bessel beams and tailored on-axis intensity profiles which are generated using a phase-only spatial light modulator. This technique for compensating one of the most fundamental limiting processes in linear optics is shown to be efficient for a wide range of experimental conditions (modifying the refractive index and the attenuation coefficient). Finally, we explain how this method can be advantageously exploited in applications ranging from bio-imaging light sheet microscopy to quantum memories for future quantum communication networks.

We report the fabrication and characterization of photonic structures using tapered optical nanofibers. Thanks to the extension of the evanescent electromagnetic field outside of the nanofiber two types of devices can be built: a ring interferometer and a knot resonator. We propose a general approach to predict the properties of these structures using the linear coupling theory. In addition, we describe a new source of birefringence due to the ovalization of a nanofiber under strong bending, known in mechanical engineering as the Brazier effect.

We report on the generation of a train of ~ 2 ps, 10 um laser pulses via multiple four-wave mixing and compression of an infrared laser beat-wave propagating in the negative group velocity dispersion region of bulk GaAs and a combination of GaAs and NaCl. The use of a 200 ps, 106 GHz beat-wave, produced by combining laser pulses amplified on the 10P(20) and 10P(16) transition of a CO2 laser, provides a novel method for generating high-power, picosecond, mid-IR laser pulses at a high repetition rate. By using 165 and 882 GHz beat-waves we show that cascaded phase-mismatched difference frequency generation plays a significant role in the four-wave mixing process in GaAs.

In a recent preprint (arXiv:1401.1128v1) Cilibrizzi and co-workers report experiments and simulations showing the scattering of polaritons against a localised obstacle in a semiconductor microcavity. The authors observe in the linear excitation regime the formation of density and phase patterns reminiscent of those expected in the non-linear regime from the nucleation of dark solitons. Based on this observation, they conclude that previous theoretical and experimental reports on dark solitons in a polariton system should be revised. Here we comment why the results from Cilibrizzi et al. take place in a very different regime than previous investigations on dark soliton nucleation and do not reproduce all the signatures of its rich nonlinear phenomenology. First of all, Cilibrizzi et al. consider a particular type of radial excitation that strongly determines the observed patterns, while in previous reports the excitation has a plane-wave profile. Most importantly, the nonlinear relation between phase jump, soliton width and fluid velocity, and the existence of a critical velocity with the time-dependent formation of vortex-antivortex pairs are absent in the linear regime. In previous reports about dark soliton and half-dark soliton nucleation in a polariton fluid, the distinctive dark soliton physics is supported both by theory (analytical and numerical) and experiments (both continuous wave and pulsed excitation)., Comment: 4 pages, 2 figures

We present a theoretical study of the hydrodynamic properties of a quantum gas of exciton-polaritons in a semiconductor microcavity under a resonant laser excitation. The effect of a spatially extended defect on the superfluid flow is investigated as a function of the flow speed. The processes that are responsible for the nucleation of vortices and solitons in the wake of the defect are characterized, as well as the regimes where the superfluid flow remains unperturbed. Specific features due to the non-equilibrium nature of the polariton fluid are put in evidence.