4 results on '"Lebugle, Maxime"'
Search Results
2. Simultaneous two-color snapshot view on ultrafast charge and spin dynamics in a Fe-Cu-Ni tri-layer
- Author
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Rösner, Benedikt, Vodungbo, Boris, Chardonnet, Valentin, Döring, Florian, Guzenko, Vitaliy A., Hennes, Marcel, Kleibert, Armin, Lebugle, Maxime, Lüning, Jan, Mahne, Nicola, Merhe, Aladine, Naumenko, Denys, Nikolov, Ivaylo P., Lopez-Quintas, Ignacio, Pedersoli, Emanuele, Ribič, Primož R., Savchenko, Tatiana, Watts, Benjamin, Zangrando, Marco, Capotondi, Flavio, David, Christian, and Jal, Emmanuelle
- Subjects
Condensed Matter - Materials Science ,Physics - Instrumentation and Detectors ,Physics - Optics - Abstract
Ultrafast phenomena on a femtosecond timescale are commonly examined by pump-probe experiments. This implies multiple measurements where the sample under investigation is pumped with a short light pulse and then probed with a second pulse at various time delays to follow its dynamics. Recently, the principle of streaking extreme ultraviolet (XUV) pulses in the temporal domain has enabled recording the dynamics of a system within a single pulse. However, separate pump-probe experiments at different absorption edges still lack a unified timing, when comparing the dynamics in complex systems. Here we report on an experiment using a dedicated optical element and the two-color emission of the FERMI XUV free-electron laser to follow the charge and spin dynamics in composite materials at two distinct absorption edges, simultaneously. The sample, consisting of ferromagnetic Fe and Ni layers, separated by a Cu layer, is pumped by an infrared laser and probed by a two-color XUV pulse with photon energies tuned to the M edges of these two transition metals. The experimental geometry intrinsically avoids any timing uncertainty between the two elements and unambiguously reveals an approximately 100 fs delay of the magnetic response with respect to the electronic excitation for both Fe and Ni. This delay shows that the electronic and spin degrees of freedom are decoupled during the demagnetization process. These observations underline the importance of simultaneous investigation of the temporal response of both charge and spin in multi-component materials. In a more general scenario, the experimental approach can be extended to continuous energy ranges, promising the development of jitter-free transient absorption spectroscopy in the XUV and soft X-ray regimes.
- Published
- 2020
- Full Text
- View/download PDF
3. Bloch Oscillations of Einstein-Podolsky-Rosen States
- Author
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Lebugle, Maxime, Gräfe, Markus, Heilmann, René, Perez-Leija, Armando, Nolte, Stefan, and Szameit, Alexander
- Subjects
Quantum Physics ,Condensed Matter - Other Condensed Matter ,Physics - Optics - Abstract
Bloch Oscillations (BOs) of quantum particles manifest themselves as periodic spreading and re-localization of the associated wave functions when traversing lattice potentials subject to external gradient forces. Albeit BOs are deeply rooted into the very foundations of quantum mechanics, all experimental observations of this phenomenon so far have only contemplated dynamics of one or two particles initially prepared in separable local states, which is well described by classical wave physics. Evidently, a more general description of genuinely quantum BOs will be achieved upon excitation of a Bloch-oscillator lattice system by nonlocal states, that is, containing correlations in contradiction with local realism. Here we report the first experimental observation of BOs of two-particle Einstein-Podolsky-Rosen states (EPR), whose associated N-particle wave functions are nonlocal by nature. The time evolution of two-photon EPR states in Bloch-oscillators, whether symmetric, antisymmetric or partially symmetric, reveals unexpected transitions from particle antibunching to bunching. Consequently, the initial state can be tailored to produce spatial correlations akin to bosons, fermions or anyons. These results pave the way for a wider class of photonic quantum simulators., Comment: 21 pages, 6 figures
- Published
- 2015
4. Simultaneous two-color snapshot view on ultrafast charge and spin dynamics in a Fe-Cu-Ni tri-layer
- Author
-
Rösner, Benedikt, Vodungbo, Boris, Chardonnet, Valentin, Döring, Florian, Guzenko, Vitaliy A., Hennes, Marcel, Kleibert, Armin, Lebugle, Maxime, Lüning, Jan, Mahne, Nicola, Merhe, Aladine, Naumenko, Denys, Nikolov, Ivaylo P., Lopez-Quintas, Ignacio, Pedersoli, Emanuele, Ribič, Primož R., Savchenko, Tatiana, Watts, Benjamin, Zangrando, Marco, Capotondi, Flavio, David, Christian, Jal, Emmanuelle, Laboratoire de Chimie Physique - Matière et Rayonnement (LCPMR), Institut de Chimie du CNRS (INC)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS), and Université Pierre et Marie Curie - Paris 6 (UPMC)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)
- Subjects
charge dynamics ,Condensed Matter - Materials Science ,[PHYS.PHYS.PHYS-OPTICS]Physics [physics]/Physics [physics]/Optics [physics.optics] ,fel ,Physics - Instrumentation and Detectors ,ultrafast ,Materials Science (cond-mat.mtrl-sci) ,FOS: Physical sciences ,Instrumentation and Detectors (physics.ins-det) ,spin dynamics ,Experimental Methodologies ,[PHYS.PHYS.PHYS-GEN-PH]Physics [physics]/Physics [physics]/General Physics [physics.gen-ph] ,ARTICLES ,[PHYS.COND.CM-GEN]Physics [physics]/Condensed Matter [cond-mat]/Other [cond-mat.other] ,lcsh:QD901-999 ,lcsh:Crystallography ,[PHYS.PHYS.PHYS-INS-DET]Physics [physics]/Physics [physics]/Instrumentation and Detectors [physics.ins-det] ,ComputingMilieux_MISCELLANEOUS ,Physics - Optics ,Optics (physics.optics) - Abstract
Ultrafast phenomena on a femtosecond timescale are commonly examined by pump-probe experiments. This implies multiple measurements, where the sample under investigation is pumped with a short light pulse and then probed with a second pulse at various time delays to follow its dynamics. Recently, the principle of streaking extreme ultraviolet (XUV) pulses in the temporal domain has enabled recording the dynamics of a system within a single pulse. However, separate pump-probe experiments at different absorption edges still lack a unified timing, when comparing the dynamics in complex systems. Here, we report on an experiment using a dedicated optical element and the two-color emission of the FERMI XUV free-electron laser to follow the charge and spin dynamics in composite materials at two distinct absorption edges, simultaneously. The sample, consisting of ferromagnetic Fe and Ni layers, separated by a Cu layer, is pumped by an infrared laser and probed by a two-color XUV pulse with photon energies tuned to the M-shell resonances of these two transition metals. The experimental geometry intrinsically avoids any timing uncertainty between the two elements and unambiguously reveals an approximately 100 fs delay of the magnetic response with respect to the electronic excitation for both Fe and Ni. This delay shows that the electronic and spin degrees of freedom are decoupled during the demagnetization process. We furthermore observe that the electronic dynamics of Ni and Fe show pronounced differences when probed at their resonance, while the demagnetization dynamics are similar. These observations underline the importance of simultaneous investigation of the temporal response of both charge and spin in multi-component materials. In a more general scenario, the experimental approach can be extended to continuous energy ranges, promising the development of jitter-free transient absorption spectroscopy in the XUV and soft X-ray regimes.
- Full Text
- View/download PDF
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