1. Identifying f-electron symmetries of UTe2 with O-edge resonant inelastic x-ray scattering
- Author
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Liu, Shouzheng, Xu, Yishuai, Kotta, Erica C, Miao, Lin, Ran, Sheng, Paglione, Johnpierre, Butch, Nicholas P, Denlinger, Jonathan D, Chuang, Yi-De, and Wray, L Andrew
- Subjects
Physical Sciences ,Condensed Matter Physics ,Chemical sciences ,Engineering ,Physical sciences - Abstract
The recent discovery of spin-triplet superconductivity emerging from a nonmagnetic parent state in UTe2 has stimulated great interest in the underlying mechanism of Cooper pairing. Experimental characterization of short-range electronic and magnetic correlations is vital to understanding these phenomena. Here we use resonant inelastic x-ray scattering (RIXS), x-ray absorption spectroscopy (XAS), and atomic-multiplet-based modeling to shed light on the active debate between 5f26d1-based models with singlet crystal field states versus 5f3-based models that predict atomic Kramers doublets and much greater 5f itinerancy. The XAS and RIXS data are found to agree strongly with predictions for a 5f26d1-like valence electron configuration with weak intradimer magnetic correlations, and provide a context for interpreting recent investigations of the electronic structure and superconducting pairing mechanism.
- Published
- 2022