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Surface waves supported by structured metallic surfaces, i.e. metasurfaces, have drawn wide attention recently. They are promising for various applications ranging from integrated photonic circuits to imaging and bio-sensing in various frequency regimes. In this work, we show that surface states with diverse polarization configurations can be supported by a metasurface consisting of a single layer of bianisotropic metamaterial elements. The structure possesses D2d symmetry, which includes mirror symmetry in the xz and yz plane, and C2 rotational symmetry along y = +-x axis. Due to this unique symmetry, the metasuface supports both transverse electric (TE) and transverse magnetic (TM) waves along kx and ky directions, while a purely longitudinal mode and an elliptically polarized transverse electromagnetic (TEM) mode along ky = +-kx directions. The versatility of the surface modes on the metasurface may lead to new surface wave phenomena and device applications.

Cascaded optical field enhancement (CFE) can be realized in some specially designed multiscale plasmonic nanostructures, where the generation of extremely strong field at nanoscale volume is crucial for many applications, for example, surface enhanced Raman spectroscopy (SERS). Here, we propose a strategy of realizing a high-quality plasmonic nanoparticle-in-cavity (PIC) nanoantenna array, where strong coupling between a nanoparticle dark mode with a high order nanocavity bright mode can produce Fano resonance at a target wavelength. The Fano resonance can effectively boost the CFE in the PIC, with a field enhancement factor up to 5X10^2. A cost-effective and reliable nanofabrication method is developed with room temperature nanoimprinting lithography to manufacture high-quality PIC arrays. This technique guarantees the generation of only one gold nanoparticle at the bottom of each nanocavity, which is crucial for the generation of the expected CFE. As a demonstration of the performance and application of the PIC array, it is used as active SERS substrate for detecting 4-aminothiophenol molecules. The SERS enhancement factor up to 2X10^7 is obtained experimentally, verifying the field enhancement and potential of this device., Comment: 19 pages and 4 figures