1. Large electro-optic response of bulk ferroelectric crystals enhanced by piezoelectric resonance in the high frequency range
- Author
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Qingxin Meng, Zhongxiang Zhou, Dechang Jia, Jun Li, Yang Li, Robert McIntosh, Ruyan Guo, and Amar S. Bhalla
- Subjects
Phase transition ,Materials science ,02 engineering and technology ,Low frequency ,7. Clean energy ,01 natural sciences ,Tantalate ,symbols.namesake ,Optics ,0103 physical sciences ,General Materials Science ,010306 general physics ,business.industry ,Mechanical Engineering ,021001 nanoscience & nanotechnology ,Condensed Matter Physics ,Ferroelectricity ,Piezoelectricity ,Mechanics of Materials ,symbols ,Optoelectronics ,Photonics ,0210 nano-technology ,business ,Raman spectroscopy ,Microwave - Abstract
Electro-optic (EO) devices with high EO coefficients at radio and microwave frequencies are integral components of the photonics industry. This work determines the EO effect of ferroelectric Li-doped niobium-rich potassium tantalate niobate (K 0.95 Li 0.05 Ta 1- x Nb x O 3 ; KLTN) single crystals using improved dynamic EO measurement. The phase transitions of KLTN crystals were investigated via variable-temperature Raman spectroscopy. A full view of the surface displacement and velocity for the KLTN sample at the resonant frequency was studied using an ultra-frequency vibrometer. The KLTN sample with x = 0.60 exhibits the enhanced effective EO coefficient (γ c ) ∼ 217 pm/V near the piezoelectric resonant peaks, which is comparable with the value at low frequency. The piezoelectric enhanced EO property of KLTN single crystals can be attributed to nonlinear polarization and nonzero stress, and showing promising for designing practical optical-piezoelectric-mechanism coupling devices.
- Published
- 2018
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