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Experimental works performed on the Dubna gas-filled magnetic recoil separator (GFS) to study the reactions of formation of 294Ts and 294Og nuclides and the properties of their radioactive decay are described. Future possibilities of synthesizing new elements with Z = 119 and Z = 120 and performing experiments to study the properties of heavier isotopes of known superheavy nuclei Lv (Z = 116), Ts (Z = 117), and Og (Z = 118) are discussed.

We have studied the dependence of the production cross-sections of the isotopes 282,283112 and 286–288114 on the excitation energy of the compound nuclei 286112 and 290114. The maximum cross-sections of the xn-evaporation channels for the reaction 238U(48Ca,xn)286-x 112 were measured to be: σ 3n = 2.5 -1.1 +1.8 pb and σ 4n = 0.6 -0.5 +1.6 pb; for the reaction 242Pu(48Ca,xn)290-x 114: σ 2n ∼ 0.5 pb, σ 3n = 3.6 -1.7 +3.4 pb and σ 4n = 4.5 -1.9 +3.6 pb. In the reaction 233U(48Ca, 2-4n)277–279 112 we measured an upper cross-section limit of σ xn ≤ 0.6 pb. An increase of σ ER in the reactions of actinide targets with 48Ca can be due to the expected increase of the survivability of the excited compound nucleus upon closer approach to the closed neutron shell N = 184. The observed nuclear decay properties of the nuclides with Z = 104–118 are compared with theoretical nuclear mass calculations and the systematic trends of α-decay properties. As a whole, they give a consistent pattern of decay of the 18 even-Z neutron-rich nuclides with Z = 104–118 and N = 163–177.

neutron-rich isotopes 242,244 Pu, 243 Am, 245,248 Cm and 249 Cf with 48 Ca projectiles. The decay properties of the synthesized nuclei are consistent with the consecutive α-decays originating in the decays of parent nuclides 286,287,288,289 114, 287,288 115, 290,291,293 116 and 294 118 produced in the 2n- to 5n-evaporation channels. The present observations can be considered to be experimental evidence of the existence of the “island of stability” of superheavy elements.

This paper presents results of the experiments aimed at producing long-lived superheavy elements located near the spherical-shell closures with Z ⩾ 114 and N ⩾ 172 in the 244Pu + 48Ca and 248Cm + 48Ca reactions. The large measured α-particle energies of the newly observed nuclei, together with the long decay times and spontaneous fission terminating the chains, offer evidence of the decay of nuclei with high atomic numbers. The decay properties of the synthesized nuclei are consistent with the consecutive α-decays originating from the parent nuclides 288, 289114 and 292116, produced in the 3n and 4n evaporation channels with cross-sections of about a picobarn. The present observations can be considered as experimental evidence of the existence of the “island of stability” of superheavy elements.

This article reports the results of experiments aimed at producing hypothetical long-lived superheavy elements located near the spherical-shell closures with Z≥114 and N≥72. For the synthesis of superheavy nuclei, we used a combination of neutron-rich reaction partners, with a 244Pu target and a 48Ca projectile. The sensitivity of the present experiment exceeded by more than two orders of magnitude previous attempts at synthesizing superheavy nuclides in reactions of 48Ca projectiles with actinide targets. We observed new decay sequences of genetically linked alpha decays terminated by spontaneous fission. The high measured alpha-particle energies, together with the long decay times and spontaneous fission terminating the chains, offer evidence for the decay of nuclei with high atomic numbers. The decay properties of the synthesized nuclei are consistent with the consecutive alpha decays originating from the parent nuclides 288,289114, produced in the 3n-and 4n-evaporation channels with cross sections of about a picobarn. The present observations can be considered experimental evidence for the existence of the “island of stability” of superheavy elements and are discussed in terms of modern theoretical approaches.

The heavy-element research program of the Dubna gas-filled recoil separator requires the use of rather exotic, strongly radioactive targets which can withstand long-term, high-intensity heavy-ion bombardments. A number of targets with thicknesses of 0.1–0.8 mg/cm2 deposited on various backings by different techniques such as electrospraying, mechanical painting with organic solutions, as well as molecular plating or electrodeposition from organic solutions were tested. The best results were obtained for electroplated targets deposited on 1.5 μm Ti backings. Isotopically enriched targets of 235,236,238U, 242,244Pu, and 248Cm mounted on rotating disks were irradiated by ions ranging from neon to argon with intensities up to 2 × 1013pps delivered by the U400 cyclotron. During two months of irradiation the total beam dose of the 34S ions applied to the target of 244Pu reached 2.5 × 1019. Collaborative Dubna-Livermore experiments were performed in 1993–1995 by employing the Dubna gas-filled recoil separator and resulted in the discovery of the new nuclides 262104, 265106, 266106, 267108, and 273110. The experiments aimed at the synthesis of element 114 are under preparation. Target fabrication methods and experimental results for nuclear physics studies at Coulomb energies are described.

In bombardments of ${}^{238}$U targets with 186-MeV ${}^{34}$S projectiles we discovered the $\ensuremath{\alpha}$-decaying nuclide ${}^{267}$108 with a half-life of ${19}_{\ensuremath{-}10}^{+29}$ ms, ${E}_{\ensuremath{\alpha}}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}9.74$ to 9.87 MeV, and a production cross section of about 2.5 pb. The new nuclide was identified by measuring correlations in energy, time, and position to establish genetic links between its implantation in a position-sensitive silicon detector and subsequent $\ensuremath{\alpha}$ decay followed by $\ensuremath{\alpha}$ decays of known descendant nuclides.

In bombardments of 248Cm with 22Ne we discovered two new isotopes, 265106 and 266106, by establishing genetic links between α decays of the 106 nuclides and spontaneous fission (SF) or α decays of the daughter (or granddaughter) nuclides. For 266106 we measured Eα = 8.63 ± 0.05 MeV followed by the SF decay of 262104 for which we measured a half-life value of 1.2+1.00.5 s. For 265106 we measured Eα = 8.71–8.91 MeV. We estimated α half-lives of 10–30 s for 266106 and 2–30 s for 265106 with SF branches of approximately 50% or less. The decay properties of 266106 indicate a large enhancement in the SF stability of this N = 160 nuclide and confirm the existence of the predicted deformed shells N = 162 and Z = 108.

Thirty‐four new nuclides with Z = 104–116, 118 and N = 161–177 have been synthesized in the complete‐fusion reactions of 238U, 237Np, 242,244Pu, 243Am, 245,248Cm, and 249Cf targets with 48Ca beams. The masses of evaporation residues were identified through measurements of the excitation functions of the xn‐evaporation channels and from cross bombardments. The decay properties of the new nuclei agree with those of previously known heavy nuclei and with predictions from different theoretical models. A discussion of self‐consistent interpretations of all observed decay chains originating from the parent isotopes 282,283112, 282113, 286–289114, 287,288115, 290–293116, and 294118 is presented. Decay energies and lifetimes of the neutron‐rich superheavy nuclei as well as their production cross sections indicate a considerable increase in the stability of nuclei with the approach to the theoretically predicted nuclear shells with N = 184 and Z = 114.

Thirty‐four new nuclides with Z = 104–116, 118 and N = 161–177 have been synthesized in the complete‐fusion reactions of 238U, 237Np, 242,244Pu, 243Am, 245,248Cm, and 249Cf targets with 48Ca beams. The masses of evaporation residues were identified through measurements of the excitation functions of the xn‐evaporation channels and from cross bombardments. The decay properties of the new nuclei agree with those of previously known heavy nuclei and with predictions from different theoretical models. A discussion of self‐consistent interpretations of all observed decay chains originating from the parent isotopes 282,283112, 282113, 286–289114, 287,288115, 290–293116, and 294118 is presented. Decay energies and lifetimes of the neutron‐rich superheavy nuclei as well as their production cross sections indicate a considerable increase in the stability of nuclei with the approach to the theoretically predicted nuclear shells with N = 184 and Z = 114.

The reaction of 249Bk with 48Ca has been investigated with an aim of synthesizing and studying the decay properties of isotopes of the new element 117. The experiments were performed at five projectile energies (in two runs, in 2009-2010 and 2012) and with a total beam dose of 48Ca ions of about 9x1019 The experiments yielded data on a-decay characteristics and excitation functions of the produced nuclei that establish these to be 293117 and 294117 – the products of the 4n- and 3n-evaporation channels, respectively. In total, we have observed 20 decay chains of Z=117 nuclides. The cross sections were measured to be 1.1 pb for the 3n and 2.4 pb for the 4n-reaction channel. The new 289115 events, populated by α decay of 117, demonstrate the same decay properties as those observed for 115 produced in the 243Am(48Ca,2n) reaction thus providing cross-bombardment evidence. In addition, a single decay of 294118 was observed from the reaction with 249Cf – a result of the in-growth of 249Cf in the 249Bk target. The observed decay chain of 294118 is in good agreement with decay properties obtained in 2002-2005 in the experiments with the reaction 249Cf(48Ca,3n)294118. The energies and half-lives of the odd-Z isotopes observed in the 117 decay chains together with the results obtained for lower-Z superheavy nuclei demonstrate enhancement of nuclear stability with increasing neutron number towards the predicted new magic number N=184.

This paper presents results of experiments aimed at producing long-lived superheavy elements located near the spherical shell closures with Z ≥114 and N ≥172 in the reactions of neutron-rich isotopes 244Pu, 245,248Cm and 249Cf with 48Ca projectiles. The decay properties of the synthesized nuclei are consistent with the consecutive α-decays originating in the decays of parent nuclides 289114, 290,291,293116 and 294118 produced in the 2n and 3n-evaporation channels. The present observations can be considered to be experimental evidence of the existence of the “island of stability” of superheavy elements.

This paper presents results of the experiments aimed at producing long-lived superheavy elements located near the spherical-shell closures with Z ⩾ 114 and N ⩾ 172 in the 244Pu + 48Ca and 248Cm + 48Ca reactions. The large measured α-particle energies of the newly observed nuclei, together with the long decay times and spontaneous fission terminating the chains, offer evidence of the decay of nuclei with high atomic numbers. The decay properties of the synthesized nuclei are consistent with the consecutive α-decays originating from the parent nuclides 288, 289114 and 292116, produced in the 3n and 4n evaporation channels with cross-sections of about a picobarn. The present observations can be considered as experimental evidence of the existence of the “island of stability” of superheavy elements.

In preparation for recent experiments on the synthesis of superheavy nuclei with $Z=114$ in the reaction ${}^{244}\mathrm{Pu}{+}^{48}\mathrm{Ca},$ we modified the Dubna gas-filled recoil separator and its detection system and carried out bombardments of lead targets with ${}^{48}\mathrm{Ca}$ projectiles. We studied excitation functions of the reactions ${}^{206}\mathrm{Pb}{(}^{48}\mathrm{Ca},1\ensuremath{-}4n)$ and ${}^{204,207,208}\mathrm{Pb}{(}^{48}\mathrm{Ca},2n).$ Maximum cross sections for the evaporation of 1--4 neutrons in the complete fusion reaction ${}^{206}\mathrm{Pb}{+}^{48}\mathrm{Ca}$ were measured to be ${\ensuremath{\sigma}}_{1n}=60 \mathrm{nb},$ ${\ensuremath{\sigma}}_{2n}=500 \mathrm{nb},$ ${\ensuremath{\sigma}}_{3n}=30 \mathrm{nb},$ and ${\ensuremath{\sigma}}_{4n}=0.3 \mathrm{nb}.$ In the bombardment of an enriched ${}^{204}\mathrm{Pb}$ target, we simultaneously obtained excitation functions of the ${}^{204,206,207,208}\mathrm{Pb}{(}^{48}\mathrm{Ca},2n)$ reactions induced on the isotopic admixtures present in the target material. The maximum cross sections for the evaporation of two neutrons from the compound nuclei ${}^{256}\mathrm{No},$ ${}^{255}\mathrm{No},$ and ${}^{252}\mathrm{No}$ were measured to be 2.1 $\ensuremath{\mu}\mathrm{b},$ 1.3 $\ensuremath{\mu}\mathrm{b},$ and 10 nb, respectively. The spontaneously fissioning even-even isotope ${}^{250}\mathrm{No},$ with a half-life ${T}_{1/2}=36 \ensuremath{\mu}\mathrm{s},$ was identified for the first time in this experiment. In the reaction ${}^{207}\mathrm{Pb}{+}^{34}\mathrm{S},$ we measured the excitation function for the production of the 21-ms spontaneously fissioning isotope ${}^{238}\mathrm{Cf},$ confirming our preliminary identification of this nuclide based on the results of cross bombardments.

We present the observation of the first decay event of the new nuclide {sup 292}116 in the running experiment on the synthesis of Z=116 nuclei in the reaction {sup 248}Cm+{sup 48}Ca. The experiment is in progress at FLNR, JINR, Dubna.

118 s); for the spontaneous fission (T1/257.522.9 114 s), the total energies deposited in the detector array were 213 62 and 221 62 MeV. The decay properties of the synthesized nuclei are consistent with the consecutive a decays originating from the parent even-even nucleus 288 114, produced in the 4n-evaporation channel with a cross section of about 1 pb. 288 114 and 284 112 are the heaviest known a-decaying even-even nuclides, following the production of 260 Sg and 266 Sg (Z5106) and the observation of a decay of 264 Hs (Z5108). The observed radioactive properties of 288 114 and the daughter nuclides match the decay scenario predicted by the macroscopic-microscopic theory.