1. Moir��-localized interlayer exciton wavefunctions captured by imaging its electron and hole constituents
- Author
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Karni, Ouri, Barr��, Elyse, Pareek, Vivek, Georgaras, Johnathan D., Man, Michael K. L., Sahoo, Chakradhar, Bacon, David R., Zhu, Xing, Ribeiro, Henrique B., O'Beirne, Aidan L., Hu, Jenny, Al-Mahboob, Abdullah, Abdelrasoul, Mohamed M. M., Chan, Nicholas S., Karmakar, Arka, Winchester, Andrew J., Kim, Bumho, Watanabe, Kenji, Taniguchi, Takashi, Barmak, Katayun, Mad��o, Julien, da Jornada, Felipe H., Heinz, Tony F., and Dani, Keshav M.
- Subjects
Chemical Physics (physics.chem-ph) ,Materials Science (cond-mat.mtrl-sci) ,FOS: Physical sciences ,Applied Physics (physics.app-ph) ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,Optics (physics.optics) - Abstract
Interlayer excitons (ILXs) - electron-hole pairs bound across two atomically thin layered semiconductors - have emerged as attractive platforms to study exciton condensation, single-photon emission and other quantum-information applications. Yet, despite extensive optical spectroscopic investigations, critical information about their size, valley configuration and the influence of the moir�� potential remains unknown. Here, we captured images of the time- and momentum-resolved distribution of both the electron and the hole that bind to form the ILX in a WSe2/MoS2 heterostructure. We thereby obtain a direct measurement of the interlayer exciton diameter of ~5.4 nm, comparable to the moir�� unit-cell length of 6.1 nm. Surprisingly, this large ILX is well localized within the moir�� cell to a region of only 1.8 nm - smaller than the size of the exciton itself. This high degree of localization of the interlayer exciton is backed by Bethe-Salpeter equation calculations and demonstrates that the ILX can be localized within small moir�� unit cells. Unlike large moir�� cells, these are uniform over large regions, thus allowing the formation of extended arrays of localized excitations for quantum technology., 4 figures
- Published
- 2021
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