1. A high performance self-powered photodetector based on a 1D Te–2D WS2 mixed-dimensional heterostructure
- Author
-
Peiting Wen, Wei Gao, Jingbo Li, Nengjie Huo, Lixiang Han, and Mengmeng Yang
- Subjects
Materials science ,business.industry ,General Engineering ,Photodetector ,Bioengineering ,Heterojunction ,02 engineering and technology ,General Chemistry ,Photovoltaic effect ,010402 general chemistry ,021001 nanoscience & nanotechnology ,01 natural sciences ,Atomic and Molecular Physics, and Optics ,0104 chemical sciences ,Photovoltaics ,Rise time ,Electric field ,Optoelectronics ,General Materials Science ,Quantum efficiency ,0210 nano-technology ,business ,Dark current - Abstract
One-dimensional (1D)–two-dimensional (2D) van der Waals (vdWs) mixed-dimensional heterostructures with advantages of an atomically sharp interface, high quality and good compatibility have attracted tremendous attention in recent years. Herein, a mixed-dimensional vertical heterostructure is constructed by transferring mechanically exfoliated 2D WS2 nanosheets on epitaxially grown 1D tellurium (Te) microwires. According to the theoretical type-II band alignment, the device exhibits a photovoltaic effect and serves as an excellent self-powered photodetector with a maximum open-circuit voltage (Voc) up to ∼0.2 V. Upon 635 nm light illumination, the photoresponsivity, external quantum efficiency and detectivity of the self-powered photodetector (SPPD) are calculated to be 471 mA W−1, 91% and 1.24 × 1012 Jones, respectively. Moreover, the dark current of the SPPD is highly suppressed to the sub-pA level due to the large lateral built-in electric field, which leads to a high Ilight/Idark ratio of 104 with a rise time of 25 ms and decay time of 14.7 ms. The abovementioned properties can be further enhanced under a negative bias of −2 V. In brief, the 1D Te–2D WS2 mixed-dimensional heterostructures have great application potential in high performance photodetectors and photovoltaics.
- Published
- 2021
- Full Text
- View/download PDF