1. Magnetotransport properties of La 1−x Ca x MnO 3 (0.52 ≤ x ≤ 0.75): Signature of phase coexistence
- Author
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Bojana Korin-Hamzić, Florian Fischgrabe, Vasily Moshnyaga, Emil Tafra, Matija Čulo, Silvia Tomić, Mario Basletić, and Amir Hamzić
- Subjects
010302 applied physics ,Physics ,Colossal magnetoresistance ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed matter physics ,Magnetoresistance ,Metals and Alloys ,FOS: Physical sciences ,Surfaces and Interfaces ,Manganite ,01 natural sciences ,Variable-range hopping ,3. Good health ,Surfaces, Coatings and Films ,Electronic, Optical and Magnetic Materials ,Condensed Matter - Strongly Correlated Electrons ,Manganites ,Charge order ,Magnetotransport ,CMR ,Phase coexistence ,Ferromagnetism ,Phase (matter) ,0103 physical sciences ,Materials Chemistry ,Antiferromagnetism ,010306 general physics ,Phase diagram - Abstract
We report the temperature and magnetic field dependence of transport properties in epitaxial films of the manganite La$_{1-x}$Ca$_{x}$MnO$_{3}$ in the overdoped region of the phase diagram for $x > 0.5$, where a charge--ordered (CO) and an antiferromagnetic (AF) phase are present. Resistivity, magnetoresistance and angular dependence of magnetoresistance were measured in the temperature interval $4.2 ~\mathrm{K} < T < 300 ~\mathrm{K}$, for three concentrations $x = 0.52, 0.58$ and $0.75$ and in magnetic fields up to 5 T. The semiconductor/insulator--like behavior in zero field was observed in the entire temperature range for all three concentrations \textit{x} and the electric conduction, at lower temperatures, in the CO state obeys 3D Mott's variable--range hopping model. A huge negative magnetoresistance for $x = 0.52$ and $x = 0.58$, a metal--insulator transition for $B > 3 ~\mathrm{T}$ for $x = 0.52$ and the presence of anisotropy in magnetoresistance for $x = 0.52$ and $x = 0.58$ show the fingerprints of colossal magnetoresistance (CMR) behavior implying the existence of ferromagnetic (FM) clusters. The declining influence of the FM clusters in the CO/AF part of the phase diagram with increasing $x$ contributes to a possible explanation that a phase coexistence is the origin of the CMR phenomenon., 33 pages, 7 figures, 1 table, accepted in Thin Solid Films
- Published
- 2017
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