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Controlling the morphology of inorganic nanocrystals is important because many of their electronic attributes are highly sensitive to shape and aspect ratio. FePt nanocrystals have potential as advanced magnetic materials for ultrahigh-density memory. This is due to their high shape and/or magnetocrystalline anisotropy, which allows bits as small as 3 nm to be thermally stable over typical data storage periods of 10 years. Herein, nanocrystals were simply fabricated by simultaneous reduction of platinum acetylacetonate and thermal decomposition of iron pentacarbonyl in properly chosen conditions of solvent/surfactant proportions and temperature for rational design of their shape and magnetic properties. This work has combined magnetometry measurements and micromagnetic simulations to illustrate the role of the external shape on the rotation of the magnetization vector for colloidal assemblies. [ABSTRACT FROM AUTHOR]

We exploit canted anisotropies as possible means to enhance spin-transfer-torque (STT) and reduce switching currents. The STTs in spin-valve structures with perpendicular, canted, and, as a reference, in-plane magnetic anisotropies were studied. For perpendicular magnetic anisotropy and canted spin valves the thicknesses and number of Co and Pt layers were varied to obtain different angles of the magnetic anisotropy with respect to the sample plane. Point contact measurements were used to measure the change in the switching-field of the magnetization with the change in the bias current applied to the point contact. A larger STT effect, as evidenced by a larger change in the switching magnetic field for the unit change in the dc bias current, was observed for the sample with 45° tilt in magnetization compared to a sample with 12° tilt. Tilted magnetization of the reference layer causes precessional switching, decreasing the switching energy and time. Micromagnetic simulations were performed to explain the experimental observations. [ABSTRACT FROM AUTHOR]