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The Pernambuco–Alagoas (PEAL) Domain, southern Borborema Province, northeastern Brazil, bears the most voluminous Cryogenian–Ediacaran granitic rocks in this province, which was formed during the convergence of the São Francisco Craton and the Borborem Province, during the western Gondwana amalgamation. New geochemical and isotopic data along those from the literature, for one of the largest intrusions, the Correntes composite batholith, at the southern part of this domain, indicate that the granitic rocks are intermediate to acid, oxidized, metaluminous to peraluminous, magnesian, and are high-K calc alkalic to shoshonitic with I-type signature. They are enriched in large-ion lithophile elements, exhibit lightly negative Eu in rare-earth element patterns and negative Ta–Nb, P, and Ti anomalies in spidergrams. Average initial 87Sr/86Sr is 0.7055 and rocks present values of whole-rock εNd (0.6 Ga) that fall into two groups. The pre-to syn-collisional, 635–628 Ma plutons present εNd (0.6 Ga) values from +1.3 to −2.5, with Nd model ages varying from 1.29 to 0.92 Ga, while the late-to post-collisional, 602–580 Ma, plutons show more negative values (−8.2 to −9.5), and older Nd model ages from 1.95 to 1.81 Ga. This Nd-isotope pattern is also observed in other plutons of the southern PEAL Domain and indicates a change in the lower crust source rock with time, with larger contributions of crustal components in the late-to post-collisional rocks. The chemical and isotopic characteristics of the studied granitic rocks and other granitic batholiths in the southern PEAL Domain are compatible with modern magmatic arcs of continental active margins. We propose that in earlier stages of convergence, melting has further affected the younger (Stenian –Tonian), likely less refractory rocks associated with abundance of volatiles, whose segregation would have differentiated to form the oldest plutons. Slow cooling allowed the accumulation of heat from mantle-derived magma in the pre-collisional period, which, together with radiogenic heat from thickened crust, led to partial melting of older crustal rocks, and the formation of magmas whose segregation and differentiation of the melt would originate the younger plutons in this part of the PEAL Domain. Older plutons formed during a Cryogenian-Ediacaran flare-up event that occurred in the southern PEAL Domain. • A flare-up Cryogenian-Ediacaran magmatism ocurred during convergence between the São Francisco Craton and the PEAL Domain. • Early-to syn-collisional, 635–628 Ma, plutons are mostly derived from younger (Stenian-Tonian) sources. • Syn-collisional, 602–580 Ma, plutons are mostly derived from Paleoproterozoic sources. • Crustal reworking, with minor crustal growth, and granite genesis, occurred in the PEAL Domain during the Brasiliano orogeny. [ABSTRACT FROM AUTHOR]