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In nature, many mysterious creatures capable of deformation camouflage, color camouflage, and self‐healing have inspired scientists to develop various biomimetic soft robots. However, the systematic integration of all the above functionalities into a single soft actuator system still remains a challenge. Here we chemically introduce a multi‐stimuli‐responsive tetraarylsuccinonitrile (TASN) chromophore into a liquid crystal elastomer (LCE) network through a facile thiol‐ene photoaddition method. The obtained TASN‐LCE soft actuators not only exhibit reversible shape‐morphing and reversible color‐changing behavior in response to heat and mechanical compression, but also show excellent self‐healing, reprogramming and recycling characteristics. We hope that such a TASN‐LCE actuator system endowed with dynamic distortion, thermo‐ and mechano‐chromic camouflage, and self‐healing functionalities would pave the way for further development of multifunctional biomimetic soft robotic devices. [ABSTRACT FROM AUTHOR]

Keywords: Biomimetic actuator; Camouflage; Chromophore; Liquid crystal elastomer; Self-healing EN Biomimetic actuator Camouflage Chromophore Liquid crystal elastomer Self-healing 1 1 1 02/09/22 20220214 NES 220214 B Weiche Aktoren b In ihrem Forschungsartikel (e202115755) berichten Hong Yang, Quan Li et al. über die thermo- und mechanochrome Tarnung und Selbstheilung in biomimetischen weichen Aktoren basierend auf Flüssigkristallelastomeren. Frontispiz: Thermo- and Mechanochromic Camouflage and Self-Healing in Biomimetic Soft Actuators Based on Liquid Crystal Elastomers Biomimetic actuator, Camouflage, Chromophore, Liquid crystal elastomer, Self-healing. [Extracted from the article]