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We study experimentally the processes of parametric excitation in microscopic magnetically saturated disks of nanometer-thick Yttrium Iron Garnet. We show that, depending on the relative orientation between the parametric pumping field and the static magnetization, excitation of either degenerate or non-degenerate magnon pairs is possible. In the latter case, which is particularly important for applications associated with the realization of computation in the reciprocal space, a single-frequency pumping can generate pairs of magnons whose frequencies correspond to different eigenmodes of the disk. We show that, depending on the size of the disk and the modes involved, the frequency difference in a pair can vary in the range 0.1-0.8 GHz. We demonstrate that in this system, one can easily realize a practically important situation where several magnon pairs share the same mode. We also observe the simultaneous generation of up to six different modes using a fixed-frequency monochromatic pumping. Our experimental findings are supported by numerical calculations that allow us to unambiguously identify the excited modes. Our results open new possibilities for the implementation of reciprocal-space computing making use of low damping magnetic insulators., 18 pages, 4 figures

We present the parametric excitation of spin-wave modes in YIG micro-disks via parallel pumping. Their spectroscopy is performed using magnetic resonance force microscopy (MRFM), while their spatial profiles are determined by micro-focus Brillouin light scattering (BLS). We observe that almost all the fundamental eigenmodes of an in-plane magnetized YIG micro-disk, calculated using a micromagnetic eigenmode solver, can be excited using the parallel pumping scheme, as opposed to the transverse one. The comparison between the MRFM and BLS data on one side, and the simulations on the other side, provides the complete spectroscopic labeling of over 40 parametrically excited modes. Our findings could be promising for spin-wave-based computation schemes, in which the amplitudes of a large number of spin-wave modes have to be controlled., 6 pages, 4 figures

Magnonic nano-devices exploit magnons -- quanta of spin waves -- to transmit and process information within a single integrated platform that has the potential to outperform traditional semiconductor-based electronics for low power applications. The main missing cornerstone of this information nanotechnology is an efficient scheme for the direct amplification of propagating spin waves. The recent discovery of spin-orbit torque provided an elegant mechanism for propagation losses compensation. While partial compensation of the spin-wave damping has allowed for spin-wave signal modulation, true amplification - the exponential increase in the spin-wave intensity during propagation - has so far remained elusive. Here we evidence the operating conditions to achieve unambiguous amplification using clocked nanoseconds -long spin-orbit torque pulses in sub-micrometer wide magnonic waveguides, where the effective magnetization has been engineered to be close to zero to suppress the detrimental magnon-magnon scattering. As a result, we achieve an exponential increase in the intensity of propagating spin waves up to 500 % at a propagation distance of several micrometers. These results pave the way towards the implementation of energy efficient, cascadable magnonic architectures for wave-based information processing and complex on-chip computation., Comment: 22 pages, 5 figures

Transition-metal dichalcogenides (TMDCs) are an aspiring class of materials with unique electronic and optical properties and potential applications in spin-based electronics. Here, we use terahertz emission spectroscopy to study spin-to-charge current conversion (S2C) in the TMDC NbSe$_2$ in ultra-high-vacuum-grown F|NbSe$_2$ thin-film stacks, where F is a layer of ferromagnetic Fe or Ni. Ultrafast laser excitation triggers an ultrafast spin current that is converted into an in-plane charge current and, thus, a measurable THz electromagnetic pulse. The THz signal amplitude as a function of the NbSe$_2$ thickness shows that the measured signals are fully consistent with an ultrafast optically driven injection of an in-plane-polarized spin current into NbSe$_2$. Modeling of the spin-current dynamics reveals that a sizable fraction of the total S2C originates from the bulk of NbSe$_2$ with the same, negative, sign as the spin Hall angle of pure Nb. By quantitative comparison of the emitted THz radiation from F|NbSe$_2$ to F|Pt reference samples and the results of ab-initio calculations, we estimate that the spin Hall angle of NbSe$_2$ for an in-plane polarized spin current lies between -0.2% and -1.1%, while the THz spin-current relaxation length is of the order of a few nanometers.

The laser ultrasonics technique perfectly fits the needs for non-contact, non-invasive, non-destructive mechanical probing of samples of mm to nm sizes. This technique is however limited to the excitation of low-amplitude strains, below the threshold for optical damage of the sample. In the context of strain engineering of materials, alternative optical techniques enabling the excitation of high amplitude strains in a non-destructive optical regime are seeking. We introduce here a non-destructive method for laser-shock wave generation based on additive superposition of multiple laser-excited strain waves. This technique enables strain generation up to mechanical failure of a sample at pump laser fluences below optical ablation or melting thresholds. We demonstrate the ability to generate nonlinear surface acoustic waves (SAWs) in Nb:SrTiO$_3$ substrates, at typically 1 kHz repetition rate, with associated strains in the percent range and pressures close to 100 kbars. This study paves the way for the investigation of a host of high-strength SAW-induced phenomena, including phase transitions in conventional and quantum materials, plasticity and a myriad of material failure modes, chemistry and other effects in bulk samples, thin layers, or two-dimensional materials.

We perform ultrafast pump-probe measurements on a nanometer-thick crystalline Bi-doped yttrium iron garnet film with perpendicular magnetic anisotropy. Tuning the photon energy of the pump laser pulses above and below the material's bandgap, we trigger ultrafast optical and spin dynamics via both one- and two-photon absorption. Contrary to the common scenario, the optically-induced heating of the system induces an increase up to 20% of the ferromagnetic resonance frequency. We explain this unexpected result in terms of a photo-induced modification of the magnetic anisotropy, i.e. of the effective field, identifying the necessary conditions to observe this effect. Our results disclose the possibility to optically increase the magnetic eigenfrequency in nanometer-thick magnets., 5 pages, 4 figures

A magnetic material combining low losses and large Perpendicular Magnetic Anisotropy (PMA) is still a missing brick in the magnonic and spintronic fields. We report here on the growth of ultrathin Bismuth doped Y$_{3}$Fe$_{5}$O$_{12}$ (BiYIG) films on Gd$_{3}$Ga$_{5}$O$_{12}$ (GGG) and substituted GGG (sGGG) (111) oriented substrates. A fine tuning of the PMA is obtained using both epitaxial strain and growth induced anisotropies. Both spontaneously in-plane and out-of-plane magnetized thin films can be elaborated. Ferromagnetic Resonance (FMR) measurements demonstrate the high dynamic quality of these BiYIG ultrathin films, PMA films with Gilbert damping values as low as 3 10$^{-4}$ and FMR linewidth of 0.3 mT at 8 GHz are achieved even for films that do not exceed 30 nm in thickness. Moreover, we measure Inverse Spin Hall Effect (ISHE) on Pt/BiYIG stacks showing that the magnetic insulator$'$s surface is transparent to spin current making it appealing for spintronic applications., 17 pages, 4 figures and 8 pages of Supp. informations

Strongly out-of-equilibrium regimes in magnetic nanostructures exhibit novel properties, linked to the nonlinear nature of magnetization dynamics, which are of great fundamental and practical interest. Here, we demonstrate that ferromagnetic resonance driven by microwave magnetic fields can occur with substantial spatial coherency at an unprecedented large angle of magnetization precessions, which is normally prevented by the onset of spin-wave instabilities and magnetization turbulent dynamics. Our results show that this limitation can be overcome in nanomagnets, where the geometric confinement drastically reduces the density of spin-wave modes. When the obtained deeply nonlinear ferromagnetic resonance regime is perturbed, the magnetization undergoes eigenoscillations around the steady state due to torques tending to restore the stable large-angle periodic trajectory. These eigenoscillations are substantially different from the usual spin-wave modes around the ground state because their existence is connected to the presence of a large coherent precession. They are experimentally investigated by a new spectroscopic technique based on the application of a second microwave excitation field that is tuned to resonantly drive them. This two-tone spectroscopy enables us to show that they consist in slow coherent magnetization nutations around the large-angle steady precession, whose frequencies are set by the balance of restoring torques. Our experimental findings are well accounted for by an analytical model derived for systems with uniaxial symmetry. They also provide a new means for controlling highly nonlinear magnetization dynamics in nanostructures, opening interesting applicative opportunities in the context of magnetic nanotechnologies., Y. L. thanks the French National Research Agency for funding under Contract No. ANR-14-CE26- 0021 (MEMOS), V. V. N. acknowledges the Russian Competitive Growth program of Kazan Federal University, and C. S. acknowledges the Labex NanoSaclay (ANR-10-LABX-0035) for support under the action “Rayonnement International.” This research was partially funded by the ANR-18-CE24-0021 (MAESTRO) project.

We demonstrate an enhanced, bidirectional, in-plane magnetic field tuning of the gyrotropic resonance frequency of a magnetic vortex within a disk by introducing a flat edge. When the core is in its vicinity, the flat edge locally reduces the core's directional dynamic stiffness for movement parallel to the edge. This strongly reduces the net dynamic core stiffness, leading to the gyrotropic frequency being significantly less than when the core is centered (or located near the round edge). This leads to the measurable range of gyrotropic frequencies being more than doubled and also results in a clear chirality-mediated bistability of the gyrotropic resonance frequency due to what is effectively a chirality-dependence of the core's confining potential., 6 pages, 5 figures

We report a study on spin conductance in ultra-thin films of Yttrium Iron Garnet (YIG), where spin transport is provided by propagating spin waves, that are generated and detected by direct and inverse spin Hall effects in two Pt wires deposited on top. While at low current the spin conductance is dominated by transport of thermal magnons, at high current, the spin conductance is dominated by low-damping non-equilibrium magnons thermalized near the spectral bottom by magnon-magnon interaction, with consequent a sensitivity to the applied magnetic field and a longer decay length. This picture is supported by microfocus Brillouin Light Scattering spectroscopy.

We study translational, breathing and twisting resonant modes of transverse magnetic domain walls pinned at notches in ferromagnetic nanostrips. We demonstrate that a mode's sensitivity to notches depends strongly on the characteristics of that particular resonance. For example, the frequencies of modes involving lateral motion of the wall are the ones which are most sensitive to changes in the notch intrusion depth (especially at the narrower, more strongly confined end of the domain wall). In contrast, the breathing mode, whose dynamics are concentrated away from the notches is relatively insensitive to changes in the notches' sizes. We also demonstrate a sharp drop in the translational mode's frequency towards zero when approaching depinning which is found, using a harmonic oscillator model, to be consistent with a reduction in the local slope of the notch-induced confining potential at its edge., 11 pages, 10 figures, additional data and analysis

Layered transition-metal dichalcogenides (TMDs) family are gaining increasing importance due to their unique electronic band structures, promising interplay among light, valley (pseudospin), charge and spin degrees of freedom. They possess large intrinsic spin-orbit interaction which make them most relevant for the emerging field of spin-orbitronics. Here we report on the conversion of spin current to charge current in MoS2 monolayer. Using spin pumping from a ferromagnetic layer (10 nm of cobalt) we find that the spin to charge conversion is highly efficient. Analysis in the frame of the inverse Rashba-Edelstein (RE) effect yields a RE length in excess of 4 nm at room temperature. Furthermore, owing to the semiconducting nature of MoS$_{2}$, it is found that back-gating allows electrical field control of the spin-relaxation rate of the MoS$_{2}$-metallic stack.

We report on an experimental study on the spin-waves relaxation rate in two series of nanodisks of diameter $\phi=$300, 500 and 700~nm, patterned out of two systems: a 20~nm thick yttrium iron garnet (YIG) film grown by pulsed laser deposition either bare or covered by 13~nm of Pt. Using a magnetic resonance force microscope, we measure precisely the ferromagnetic resonance linewidth of each individual YIG and YIG{\textbar}Pt nanodisks. We find that the linewidth in the nanostructure is sensibly smaller than the one measured in the extended film. Analysis of the frequency dependence of the spectral linewidth indicates that the improvement is principally due to the suppression of the inhomogeneous part of the broadening due to geometrical confinement, suggesting that only the homogeneous broadening contributes to the linewidth of the nanostructure. For the bare YIG nano-disks, the broadening is associated to a damping constant $\alpha = 4 \cdot 10^{-4}$. A 3 fold increase of the linewidth is observed for the series with Pt cap layer, attributed to the spin pumping effect. The measured enhancement allows to extract the spin mixing conductance found to be $G_{\uparrow \downarrow}= 1.55 \cdot 10^{14}~ \Omega^{-1}\text{m}^{-2}$ for our YIG(20nm){\textbar}Pt interface, thus opening large opportunities for the design of YIG based nanostructures with optimized magnetic losses., Comment: 4 pages, 3 figures