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Highlights: A flexible tribotronic artificial synapse with bioinspired neurosensory behaviour was demonstrated, which establishes an active interaction mechanism with the environment. The device can well exhibit tuneable synaptic behaviours by changing the mechanical input modes, including excitatory postsynaptic current, paired-pulse facilitation, and the hierarchical memorial process. The device has excellent mechanical flexibility that can exhibit stable synaptic functions even under strain conditions with a bending radius of 20 mm after 1000 bending cycles. As key components of artificial afferent nervous systems, synaptic devices can mimic the physiological synaptic behaviors, which have attracted extensive attentions. Here, a flexible tribotronic artificial synapse (TAS) with bioinspired neurosensory behavior is developed. The triboelectric potential generated by the external contact electrification is used as the ion-gel-gate voltage of the organic thin film transistor, which can tune the carriers transport through the migration/accumulation of ions. The TAS successfully demonstrates a series of synaptic behaviors by external stimuli, such as excitatory postsynaptic current, paired-pulse facilitation, and the hierarchical memory process from sensory memory to short-term memory and long-term memory. Moreover, the synaptic behaviors remained stable under the strain condition with a bending radius of 20 mm, and the TAS still exhibits excellent durability after 1000 bending cycles. Finally, Pavlovian conditioning has been successfully mimicked by applying force and vibration as food and bell, respectively. This work demonstrates a bioinspired flexible artificial synapse that will help to facilitate the development of artificial afferent nervous systems, which is great significance to the practical application of artificial limbs, robotics, and bionics in future. [ABSTRACT FROM AUTHOR]

Tribotronics has attracted great attention as a new research field that encompasses the control and tuning of semiconductor transport by triboelectricity. Here, tribotronics is reviewed in terms of active mechanosensation and human–machine interfacing. As a fundamental unit, contact electrification field‐effect transistors are analyzed, in which the triboelectric potential can be used to control electrical transport in semiconductors. Several tribotronic functional devices have been developed for active control and information sensing, which has demonstrated triboelectricity‐controlled electronics and established active mechanosensation for the external environment. In addition, the universal triboelectric power management strategy and the triboelectric nanogenerator‐based constant sources are also reviewed, in which triboelectricity can be managed by electronics in the reverse action. With the implantation of triboelectric power management modules, the harvested triboelectricity by various kinds of human kinetic and environmental mechanical energy can be effectively managed as a power supply for self‐powered microsystems. In terms of the research prospects for interactions between triboelectricity and semiconductors, tribotronics is expected to demonstrate significant impact and potential applications in micro‐electro‐mechanical systems/nano‐electro‐mechanical systems (MEMS/NEMS), flexible electronics, robotics, wireless sensor network, and Internet of Things. [ABSTRACT FROM AUTHOR]