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Considering the growing interest in magnetic materials for unconventional computing, data storage, and sensor applications, there is active research not only on material synthesis but also characterisation of their properties. In addition to structural and integral magnetic characterisations, imaging of magnetisation patterns, current distributions and magnetic fields at nano- and microscale is of major importance to understand the material responses and qualify them for specific applications. In this roadmap, we aim to cover a broad portfolio of techniques to perform nano- and microscale magnetic imaging using superconducting quantum interference devices, spin centre and Hall effect magnetometries, scanning probe microscopies, x-ray- and electron-based methods as well as magnetooptics and nanoscale magnetic resonance imaging. The roadmap is aimed as a single access point of information for experts in the field as well as the young generation of students outlining prospects of the development of magnetic imaging technologies for the upcoming decade with a focus on physics, materials science, and chemistry of planar, three-dimensional and geometrically curved objects of different material classes including two-dimensional materials, complex oxides, semi-metals, multiferroics, skyrmions, antiferromagnets, frustrated magnets, magnetic molecules/nanoparticles, ionic conductors, superconductors, spintronic and spinorbitronic materials.

Understanding magnetic phase transitions from stripe to skyrmion textures provide fundamental scientific insights into the details of the intermediate topologies through which the system evolves. The solitonic nature of spin texture in both stripe and skyrmion phases has been observed in materials with Dzyaloshinskii-Moriya interaction. Here we show that the field evolution in a dipolar interaction mediated Fe/Gd multilayer that exhibits achiral stripe textures behaves similar to a finite-sized chiral soliton lattice. As a function of magnetic field, the stripes exhibit discrete jumps in periodicity indicative of intermediate topologies as the stripes get wound into skyrmions.

Efficient imaging of biomolecules, two-dimensional materials, and electromagnetic fields depends on retrieval of the phase of transmitted electrons. We demonstrate a method to measure phase in a scanning transmission electron microscope (STEM) using a nanofabricated diffraction grating to produce multiple probe beams. The measured phase is more interpretable than phase-contrast scanning transmission electron microscopy techniques without an off-axis reference wave, and the resolution could surpass that of off-axis electron holography. We apply this technique, called STEM holography, to image nanoparticles, carbon substrates, and electric fields. The contrast observed in experiments agrees well with contrast predicted in simulations.

The dynamic response of dipole skyrmions in Fe/Gd multilayer films is investigated by ferromagnetic resonance measurements and compared to micromagnetic simulations. We detail thickness- and temperature-dependent studies of the observed modes as well as the effects of magnetic field history on the resonant spectra. Correlation between the modes and the magnetic phase maps constructed from real-space imaging and scattering patterns allows us to conclude that the resonant modes arise from local topological features such as dipole skyrmions but do not depend on the collective response of a close-packed lattice of these chiral textures. Using micromagnetic modeling, we are able to quantitatively reproduce our experimental observations which suggests the existence of localized spin-wave modes that are dependent on the helicity of the dipole skyrmion. We identify four localized spin-wave excitations for the skyrmions that are excited under either in-plane or out-of-plane rf fields. Lastly we show that dipole skyrmions and nonchiral bubble domains exhibit qualitatively different localized spin-wave modes.

The interesting physics and potential memory technologies resulting from topologically protected spin textures such as skyrmions have prompted efforts to discover new material systems that can host these kinds of magnetic structures. Here, we use the highly tunable magnetic properties of amorphous Fe/Gd multilayer films to explore the magnetic properties that lead to dipole-stabilized skyrmions and skyrmion lattices that form from the competition of dipolar field and exchange energy. Using both real space imaging and reciprocal space scattering techniques, we determined the range of material properties and magnetic fields where skyrmions form. Micromagnetic modeling closely matches our observation of small skyrmion features (∼50 to 70 nm) and suggests that these classes of skyrmions have a rich domain structure that is Bloch-like in the center of the film and more Néel-like towards each surface. Our results provide a pathway to engineer the formation and controllability of dipole skyrmion phases in a thin film geometry at different temperatures and magnetic fields.

We show that properly engineered amorphous Fe-Gd alloy thin films with perpendicular magnetic anisotropy exhibit bound pairs of like-polarity, opposite helicity skyrmions at room temperature. Magnetic mirror symmetry planes present in the stripe phase, instead of chiral exchange, determine the internal skyrmion structure and the net achirality of the skyrmion phase. Our study shows that stripe domain engineering in amorphous alloy thin films may enable the creation of skyrmion phases with technologically desirable properties.