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This study demonstrates an energy harvester that combines a piezoelectric nanogenerator and an electret-based electrostatic generator. The device consists of an in-house fabricated nanocomposite (polydimethylsiloxane/barium titanate/carbon nanotube) as a piezoelectric layer and a monocharged Teflon fluorinated ethylene propylene as an electret electrostatic layer. The mechanical impedance of the structure can be altered easily by changing the nanocomposite monomer/cross-linker ratio and optimizing various mechanical energy sources. The energy harvester's performance was characterized by performing measurements with different frequencies (5–20 Hz) under applied dynamic loading. A total volumetric power density of ∼8.8 μW cm−3 and a total stored energy of ∼50.2 μJ min−1 were obtained. These findings indicate that this versatile, lightweight, and low-cost energy harvester can be employed as a power supply source for microelectronics in applications, such as wearables. [ABSTRACT FROM AUTHOR]