Search

The mechanisms and by-product formation of electrochemical oxidation (EO) for As(III) oxidation in drinking water treatment using groundwater was investigated. Experiments were carried out using a flowthrough system, with an RuO 2 /IrO 2 MMO Ti anode electrode, fed with synthetic and natural groundwater containing As(III) concentrations in a range of around 75 and 2 µg/L, respectively. Oxidation was dependent on charge dosage (CD) [C/L] and current density [A/m 2 ], with the latter showing plateau behaviour for increasing intensity. As(III) concentrations of <0.3 µg/L were obtained, indicating oxidation of 99.9 % of influent As(III). Achieving this required a higher charge dosage for the natural groundwater (>40 C/L) compared to the oxidation in the synthetic water matrix (20 C/L), indicating reaction with natural organic matter or other compounds. As(III) oxidation in groundwater required an energy consumption of 0.09 and 0.21 kWh/m 3 , for current densities of 20 and 60 A/m 2 , respectively. At EO settings relevant for As(III) oxidation, in the 30-100 C/L CD range, the formation of anodic by-products, as trihalomethanes (THMs) (0.11-0.75 µg/L) and bromate (<0.2 µg/L) was investigated. Interestingly, concentrations of the formed by-products did not exceed strictest regulatory standards of 1 µg/L, applicable to Dutch tap water. This study showed the promising perspective of EO as electrochemical advanced oxidation process (eAOP) in drinking water treatment as alternative for the conventional use of strong oxidizing chemicals., Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2024. Published by Elsevier Ltd.)

Drinking water distribution systems (DWDSs) are used to supply hygienically safe and biologically stable water for human consumption. The potential of thermal energy recovery from drinking water has been explored recently to provide cooling for buildings. Yet, the effects of increased water temperature induced by this "cold recovery" on the water quality in DWDSs are not known. The objective of this study was to investigate the impact of cold recovery from DWDSs on the microbiological quality of drinking water. For this purpose, three pilot distribution systems were operated in parallel for 38 weeks. System 1 has an operational heat exchanger, mimicking the cold recovery system by maintaining the water temperature at 25 °C; system 2 operated with a non-operational heat exchanger and system 3 run without heat exchanger. The results showed no significant effects on drinking water quality: cell numbers and ATP concentrations remained around 3.5 × 10 5  cells/ml and 4 ng ATP/l, comparable observed operational taxonomic units (OTUs) (~470-490) and similar Shannon indices (7.7-8.9). In the system with cold recovery, a higher relative abundance of Pseudomonas spp. and Chryseobacterium spp. was observed in the drinking water microbial community, but only when the cold recovery induced temperature difference (ΔT) was higher than 9 °C. In the 38 weeks' old biofilm, higher ATP concentration (475 vs. 89 pg/cm 2 ), lower diversity (observed OTUs: 88 vs. ≥200) and a different bacterial community composition (e.g. higher relative abundance of Novosphingobium spp.) were detected, which did not influence water quality. No impacts were observed for the selected opportunisitic pathogens after introducing cold recovery. It is concluded that cold recovery does not affect bacterial water quality. Further investigation for a longer period is commended to understand the dynamic responses of biofilm to the increased temperature caused by cold recovery., (Copyright © 2020 The Authors. Published by Elsevier Inc. All rights reserved.)

The drinking water quality changes during the transport through distribution systems. Domestic drinking water systems (DDWSs), which include the plumbing between the water meter and consumer's taps, are the most critical points in which water quality may be affected. In distribution networks, the drinking water temperature and water residence time are regarded as indicators of the drinking water quality. This paper describes an experimental research on the influence of stagnation time and temperature change on drinking water quality in a full-scale DDWS. Two sets of stagnation experiments, during winter and summer months, with various stagnation intervals (up to 168 h of stagnation) were carried out. Water and biofilms were sampled at two different taps, a kitchen and a shower tap. Results from this study indicate that temperature and water stagnation affect both chemical and microbial quality in DDWSs, whereas microbial parameters in stagnant water appear to be driven by the temperature of fresh water. Biofilm formed in the shower pipe contained more total and intact cells than the kitchen pipe biofilm. Alphaproteobacteria were found to dominate in the shower biofilm (78% of all Proteobacteria), while in the kitchen tap biofilm Alphaproteobacteria, Betaproteobacteria and Gammaproteobacteria were evenly distributed., (Copyright © 2017 The Authors. Published by Elsevier Ltd.. All rights reserved.)

The fate of H2O2 residual from advanced oxidation process (AOP) preceding managed aquifer recharge (MAR) is of concern because H2O2 could lead to undesired effects on organisms in the MAR aquatic and soil ecosystem. The objective of this study was to distinguish between factors affecting H2O2 decomposition in MAR systems, simulated in batch reactors with synthetic MAR water and slow sand filter sand. The results showed that pure sand and soil organic matter had no considerable effect on H2O2 decomposition, whereas naturally occurring inorganic substances on the surface of sand grains and microbial biomass are the two main factors accelerating H2O2 decomposition in MAR systems. Additionally, the results showed that the H2O2 decompositions with different initial concentrations fitted first-order kinetics in 2-6 h in a mixture of slow sand filter sand (as a substitute for sand from a MAR system) and synthetic MAR water with high bacterial population. An estimation indicated that low concentrations of H2O2 (<3 mg/L) could decompose to the provisional standard of 0.25 mg/L in the first centimeters of MAR systems with the influent water containing high microbial biomass 38 ng ATP/mL., (Copyright © 2016 Elsevier Ltd. All rights reserved.)

Calcium carbonate pellets are produced as a by-product in the pellet softening process. In the Netherlands, these pellets are applied as a raw material in several industrial and agricultural processes. The sand grain inside the pellet hinders the application in some high-potential market segments such as paper and glass. Substitution of the sand grain with a calcite grain (100% calcium carbonate) is in principle possible, and could significantly improve the pellet quality. In this study, the grinding and sieving of pellets, and the subsequent reuse as seeding material in pellet softening were tested with two pilot reactors in parallel. In one reactor, garnet sand was used as seeding material, in the other ground calcite. Garnet sand and ground calcite performed equally well. An economic comparison and a life-cycle assessment were made as well. The results show that the reuse of ground calcite as seeding material in pellet softening is technologically possible, reduces the operational costs by €38,000 (1%) and reduces the environmental impact by 5%. Therefore, at the drinking water facility, Weesperkarspel of Waternet, the transition from garnet sand to ground calcite will be made at full scale, based on this pilot plant research.

Ongoing pollution and improving analytical techniques reveal more and more anthropogenic substances in drinking water sources, and incidentally in treated water as well. In fact, complete absence of any trace pollutant in treated drinking water is an illusion as current analytical techniques are capable of detecting very low concentrations. Most of the substances detected lack toxicity data to derive safe levels and have not yet been regulated. Although the concentrations in treated water usually do not have adverse health effects, their presence is still undesired because of customer perception. This leads to the question how sensitive analytical methods need to become for water quality screening, at what levels water suppliers need to take action and how effective treatment methods need to be designed to remove contaminants sufficiently. Therefore, in the Netherlands a clear and consistent approach called 'Drinking Water Quality for the 21st century (Q21)' has been developed within the joint research program of the drinking water companies. Target values for anthropogenic drinking water contaminants were derived by using the recently introduced Threshold of Toxicological Concern (TTC) approach. The target values for individual genotoxic and steroid endocrine chemicals were set at 0.01 μg/L. For all other organic chemicals the target values were set at 0.1 μg/L. The target value for the total sum of genotoxic chemicals, the total sum of steroid hormones and the total sum of all other organic compounds were set at 0.01, 0.01 and 1.0 μg/L, respectively. The Dutch Q21 approach is further supplemented by the standstill-principle and effect-directed testing. The approach is helpful in defining the goals and limits of future treatment process designs and of analytical methods to further improve and ensure the quality of drinking water, without going to unnecessary extents., (Copyright © 2013 Elsevier Ltd. All rights reserved.)

The heating of drinking water in households contributes significantly to the emission of greenhouse gases. As a water utility aiming to operate at a climate neutral level by 2020, Waternet needs to reduce its CO2 emission by 53 kton yr-1. To contribute to this ambition, a pilot project was carried out in Uilenstede, Amstelveen, the Netherlands, to recover the shower heat energy with a shower heat exchanger from Dutch Solar Systems. An experimental setup was built in the Waternet laboratory to evaluate the claimed efficiencies. The energy recovery efficiency observed in the lab was 61-64% under winter conditions and 57-62% under summer conditions, while the energy recovery efficiency observed in Uilenstede was 57% in December 2014. Based on the observations, 4% of the total energy consumption of households in Amsterdam (electricity and gas) can be recovered with a shower heat exchanger installed in all households in Amsterdam, which also means a 54 kton year-1 CO2 emission reduction can be achieved. [ABSTRACT FROM AUTHOR]

The city of Amsterdam is going to build a new housing estate: IJburg. About 18,000 houses will be built and finally 45,000 people will live in IJburg. An important objective is to realize a sustainable housing estate: the design is focused on water and energy saving, and theuse of sustainable building materials. An alternative water supply system, in which household water is used besides drinking water, may be an important contribution to this ambition. Household water can be used for toilet flushing, for washing clothes or for both. Amsterdam Water Supply developed five scenarios for such an alternative water supply system. Water saving and supply of two types of water are key elements in these scenarios. Based on a comprehensive selection in which public health aspects, technical feasibility, legislation, acceptance by the public, costs and environmental impact were used as criteria, the optimum scenario was chosen: a dual water system, supplying drinking water from the existing drinking water production plants, andsupplying household water for toilet flushing and washing, produced from a local surface water, the IJ-lake. [ABSTRACT FROM AUTHOR]

The efficiency of activated carbon for pesticide removal is negatively influenced by the presence of natural organic matter (NOM) in water. NOM molecules compete with pesticides for adsorption sites and NOMmolecules block pores thus preventing pesticides entering the micropores. To improve the efficiency of GAC-filtration several possibilities are available. By using nanofiltration as a pretreatment for granular activated carbon (GAC) filtration. GAC lifetime for pesticide removal can be increased by a factor of 100. In situations where, besides pesticides removal, hardness removal and/or colour removal is required the combination of nanofiltration and GAC filtration is an interesting option. Ozonation prior to GAC-filtration also results in an increase in GAC lifetime for pesticide removal: NOM molecules become more polar (less adsorbable), smaller and more biodegradable, which results in less competition and pore blocking and so in an increased adsorption capacity of the GAC for pesticides. In laboratory experimentsan increase in GAC lifetime for pesticide removal of about 30--70% was determined by using an ozone dose of about 1.4 mg/l (in the presence of 2 mg/l DOC). Recently, Kiwa has investigated the possibilities of activated carbon fibres (ACF) as an alternative for granular activated carbon. This product is less influenced by the presence of NOM as a result of the pore structure which contains mainly micropores. With relatively short empty bed contact times of 20--60 sec ACF showed pesticide breakthrough a factor of 3 to more than 8 later than GAC-filtration (EBCT 20 min). [ABSTRACT FROM AUTHOR]

Wastewater reuse is becoming increasingly important for supplementing drinking water supply needs and/or to reduce costs in many communities around the world. However, wastewater reuse can result in a potential transmission route for infectious agents. Therefore, the occurrence of Cryptosporidium was assessed in a treatment plant geared for the production of drinking water from wastewater effluent and the results were compared to those on an existing typical drinking water treatment plant operated by Waternet, the water cycle company of Amsterdam, The Netherlands, and its surrounding areas. The assessment was done using Monte-Carlo simulation and probability density functions to determine the occurrence of Cryptosporidium in raw surface water and wastewater effluent and the removal in different treatment steps. From the research conducted, it was concluded that under normal conditions, drinking water that meets Dutch drinking water quality standards could also be produced from treated wastewater effluent. However, additional redundancy should be built in to meet the standards under extreme operating conditions. [ABSTRACT FROM AUTHOR]