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The measurement of hydrogen concentration in fuel cell systems is an important prerequisite for the development of a control strategy to enhance system performance, reduce purge losses and minimize fuel cell aging effects. In this perspective paper, the working principles of hydrogen sensors are analyzed and their requirements for hydrogen control in fuel cell systems are critically discussed. The wide measurement range, absence of oxygen, high humidity and limited space turn out to be most limiting. A perspective on the development of hydrogen sensors based on palladium as a gas-sensitive metal and based on the organic magnetic field effect in organic light-emitting devices is presented. The design of a test chamber, where the sensor response can easily be analyzed under fuel cell-like conditions is proposed. This allows the generation of practical knowledge for further sensor development. The presented sensors could be integrated into the end plate to measure the hydrogen concentration at the anode in- and outlet. Further miniaturization is necessary to integrate them into the flow field of the fuel cell to avoid fuel starvation in each single cell. Compressed sensing methods are used for more efficient data analysis. By using a dynamical sensor model, control algorithms are applied with high frequency to control the hydrogen concentration, the purge process, and the recirculation pump.