1. Finite-temperature dynamics and the role of disorder in nearly critical Ni(Cl1−xBrx)2·4SC(NH2)2
- Author
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L. Facheris, Andrey Zheludev, Dominic Blosser, R. I. Bewley, K. Yu. Povarov, and Severian Gvasaliya
- Subjects
Physics ,Condensed matter physics ,Magnon ,Dynamic structure factor ,02 engineering and technology ,021001 nanoscience & nanotechnology ,01 natural sciences ,Inelastic neutron scattering ,Spin wave ,0103 physical sciences ,Antiferromagnetism ,010306 general physics ,0210 nano-technology ,Structure factor ,Critical exponent ,Energy (signal processing) - Abstract
Inelastic neutron scattering is used to investigate the temperature dependence of spin correlations in the 3-dimensional XY antiferromagnet $\mathrm{Ni}{({\mathrm{Cl}}_{1\ensuremath{-}x}{\mathrm{Br}}_{x})}_{2}\ifmmode\cdot\else\textperiodcentered\fi{}4\mathrm{SC}{({\mathrm{NH}}_{2})}_{2}, x=0.14(1)$, tuned close to the chemical-composition-induced soft-mode transition. The local dynamic structure factor shows $\ensuremath{\hbar}\ensuremath{\omega}/T$ scaling behavior characteristic of a quantum-critical point. The deviation of the measured critical exponent from spin wave theoretical expectations is attributed to disorder. Another effect of disorder is local excitations above the magnon band. Their energy, structure factor, and temperature dependence are well explained by simple strong-bond dimers associated with Br-impurity sites.
- Published
- 2020
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