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Magnetic systems governed by exchange interactions between magnetic moments harbor frustration that leads to ground state degeneracy and results in the new topological state often referred to as a frustrated state of matter (FSM). The frustration in the commonly discussed magnetic systems has a spatial origin. Here we demonstrate that an array of nanomagnets coupled by the real retarded exchange interactions develops a new state of matter, time frustrated matter (TFM). In a spin system with the time-dependent retarded exchange interaction, a single spin-flip influences other spins not instantly but after some delay. This implies that the sign of the exchange interaction changes, leading to either ferro- or antiferromagnetic interaction, depends on time. As a result, the system's temporal evolution is essentially non-Markovian. The emerging competition between different magnetic orders leads to a new kind of time-core frustration. To establish this paradigmatic shift, we focus on the exemplary system, a granular multiferroic, where the exchange transferring medium has a pronounced frequency dispersion and hence develops the TFM.

The Kugel--Khomskii model with entangled spin and orbital degrees of freedom is a good testing ground for many important features in quantum information processing, such as robust gaps in the entanglement spectra. Here, we demonstrate that the entanglement can be also robust under effect of temperature within a wide range of parameters. It is shown, in particular, that the temperature dependence of entanglement often exhibits a nonmonotonic behavior. Namely, there turn out to be ranges of the model parameters, where entanglement is absent at zero temperature, but then, with an increase in temperature, it appears, passes through a maximum, and again vanishes., Comment: 10 pages, 8 figures

Using the exact diagonalization technique, we determine the energy spectrum and wave functions for finite chains described by the two-spin (Kugel--Khomskii) model with different types of intersubsystem exchange terms. The found solutions provide a possibility to address the problem of quantum entanglement inherent to this class of models. We put the main emphasis on the calculations of the concurrence treated as an adequate numerical measure of the entanglement. We also analyze the behavior of two-site correlation functions considered as a local indicator of entanglement. We construct the phase diagrams of the models involving the regions of nonzero entanglement. The pronounced effect of external fields, conjugated to both spin variables on the regions with entanglement, could both enhance and weaken the entanglement depending on the parameters of the models.

We address quantum spin helical states in the strongly frustrated Heisenberg model. Contrary to conventional Dzyaloshinskii-Moriya approach we show that such states appear without central symmetry breaking. As an example, we demonstrate that the magnetic and thermodynamic properties of the quasi-two-dimensional square-lattice compound $\mathrm{(CuBr)Sr_{2}Nb_{3}O_{10}}$ can be interpreted within 2D $S = 1/2$ $J_1-J_2-J_3$ Heisenberg model. In this compound neutron experiment indicates helical spin order while central symmetry does hold.

The specific heat and susceptibilities for the two- and one-dimensional spin--orbital models are calculated in the framework of a spherically symmetric self-consistent approach at different temperatures and relations between the parameters of the system. It is shown that even in the absence of the long-range spin and orbital order, the system exhibits the features in the behavior of thermodynamic characteristics, which are typical of those manifesting themselves at phase transitions. Such features are attributed to the quantum entanglement of the coupled spin and orbital degrees of freedom., Comment: 7 pages, 9 figures, submitted to JETP Letters

Frustrated magnetic compounds, in particular low-dimensional, are topical research due to persistent uncover of novel nontrivial quantum states and potential applications. The problem of this field is that many important results are scattered over the localized parameter ranges, while areas in between still contain hidden interesting effects. We consider $J_1-J_2-J_3$ Heisenberg model on the square lattice and use the spherically symmetric self-consistent approach for spin-spin Green's functions in "quasielastic" approximation. We have found a new local order in spin liquids: antiferromagnetic isotropical helices. On the structure factor we see circular concentric dispersionless structures, while on any radial direction the excitation spectrum has "roton" minima. That implies nontrivial magnetic excitations and consequences in magnetic susceptibility and thermodynamics. On the $J_1-J_2-J_3$ exchange parameters globe we discover a crossover between antiferromagnetic-like local order and ferromagnetic-like; we find stripe-like order in the middle. In fact, our "quasielastic" approach allows investigation of the whole $J_1-J_2-J_3$ globe., Comment: 9 pages, 12 figures

We analyze the possible types of ordering in a boson--fermion model. The Hamiltonian is inherently related to the Bose--Hubbard model for vector two-species bosons in optical lattices. We show that such model can be reduced to the Kugel--Khomskii type spin--pseudospin model, but in contrast to the usual version of the latter model, we are dealing here with the case of spin $S=1$ and pseudospin $1/2$. We show that the interplay of spin and pseudospin degrees of freedom leads to a rather nontrivial magnetic phase diagram including the spin-nematic configurations. Tuning the spin-channel interaction parameter $U_s$ gives rise to quantum phase transitions. We find that the ground state of the system always has the pseudospin domain structure. On the other hand, the sign change of $U_s$ switches the spin arrangement of the ground state within domains from ferro- to aniferromagnetic one. Finally, we revisit the spin (pseudospin)-1/2 Kugel--Khomskii model and see the inverse picture of phase transitions., Comment: 8 pages, 9 figures (in press), Phys. Rev. B, 2017

Using the spherically symmetric self-consistent Green's function method, we consider thermodynamic properties of the $S=1/2$ $J_1$-$J_2$ Heisenberg model on the 2D square lattice. We calculate the temperature dependence of the spin-spin correlation functions $c_{\mathbf{r}}=\langle S_{\mathbf{0}}^{z}S_{\mathbf{r}}^{z}\rangle $, the gaps in the spin excitation spectrum, the energy $E$ and the heat capacity $C_{V}$ for the whole $J_{1}$--$J_{2}$-circle, i.e. for arbitrary $\varphi$, $J_1=cos(\varphi)$, $J_2=sin(\varphi)$. Due to low dimension there is no long-range order at $T\neq 0$, but the short-range holds the memory of the parent zero-temperature ordered phase (antiferromagnetic, stripe or ferromagnetic). $E(\varphi)$ and $C_{V}(\varphi)$ demonstrate extrema "above" the long-range ordered phases and in the regions of rapid short-range rearranging. Tracts of $c_{\mathbf{r}}(\varphi)$ lines have several nodes leading to nonmonotonic $c_{\mathbf{r}}(T)$ dependence. For any fixed $\varphi$ the heat capacity $C_{V}(T)$ always has maximum, tending to zero at $T\rightarrow 0$, in the narrow vicinity of $\varphi = 155^{\circ}$ it exhibits an additional frustration-induced low-temperature maximum. We have also found the nonmonotonic behaviour of the spin gaps at $\varphi=270^{\circ}\pm 0$ and exponentially small antiferromagnetic gap up to ($T\lesssim 0.5$) for $\varphi \gtrsim 270^{\circ}$., Comment: 16 pages, 9 figures

Possible types of elementary excitations in the symmetric spin-orbital model on the a square lattice are analyzed using a spherically symmetric self-consistent approach. The excitation spectra are calculated. The behavior of the corresponding correlation functions depending on the temperature and parameters of the model is studied. A schematic phase diagram is plotted. It is shown that the thermodynamics of the system is mainly determined by elementary excitations with the entangled spin and orbital degrees of freedom., Comment: 5 pages, 5 figures

For the frustrated two-dimensional $S=1/2$ antiferromagnetic Heisenberg model close to quantum phase transition we consider the singlet ground states retaining both translational and SU(2) symmetry. Besides usually discussed checkerboard, spin-liquid and stripe states an unconventional state with two coexisting long-range orders appears to be possible at sufficiently large damping of spin excitations. The problem is treated in the frames of self-consistent spherically symmetric approach., Comment: 11 pages, 5 figures

The self-consistent treatment of real and imaginary renormalizations in the dynamic spin susceptibility for the frustrated Heisenberg model reproduces for cuprates at low doping: a spin spectrum, a saddle point for q near (pi/2,pi/2), nearly constant q-integrated susceptibility for energy less than 150 meV and a scaling law. Frustration increase (optimally doped case) leads to a stripe scenario with a saddle point at q near (pi,pi/2) and $\chi_{2D}(\omega)$ peak near 30meV. The obtained $\chi (\mathbf{q},\omega)$ describes neutron scattering results and leads to well-known temperature transport anomalies in doped cuprates., Comment: 4 pages, 4 figures, submitted to Phys.Rev.Lett