1. Phonon anomalies with doping in superconducting oxychlorides Ca2-xCuO2Cl2
- Author
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Lebert, Blair W., Yamamoto, Hajime, Azuma, Masaki, Heid, Rolf, Tsutsui, Satoshi, Uchiyama, Hiroshi, Baron, Alfred Q. R., Baptiste, Benoît, and d'Astuto, Matteo
- Subjects
Superconductivity (cond-mat.supr-con) ,Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,Condensed Matter - Superconductivity ,Condensed Matter::Superconductivity ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons - Abstract
We measure the dispersion of the Cu-O bond-stretching phonon mode in the high-temperature superconducting parent compound Ca$_2$CuO$_2$Cl$_2$. Our density functional theory calculations predict a cosine-shaped bending of the dispersion along both the ($\xi$00) and ($\xi\xi$0) directions, while comparison with previous results on Ca$_{1.84}$CuO$_2$Cl$_2$ show it only along ($\xi$00), suggesting an anisotropic effect which is not reproduced in calculation at optimal doping. Comparison with isostructural La$_{2-x}$Sr$_x$CuO$_4$ suggests that these calculations reproduce well the overdoped regime, however they overestimate the doping effect on the Cu-O bond-stretching mode at optimal doping.
- Published
- 2019
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