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Aviation aims to reduce its climate effect by exploiting the potential of identifying alternative climate optimized aircraft trajectories. Such climate-optimized trajectories require a dedicated meteorological service in order to inform on those regions of the atmosphere where aviation emissions have a large effect on climate, for example, by contrail formation or nitrogen-oxide (NOx)-induced ozone formation. With the algorithmic Climate Change Functions (aCCFs) prototypes of a mathematical formulation for the temporal and spatial climate effects of aviation emissions in the atmosphere is provided, which relies solely on numerical weather prediction at the time and location of emissions. Based on the recently published consistent set of aCCF-V1.0, we here introduce newly derived calibration factors for the individual non-CO2 effects of aviation (NOx, water vapour, contrail cirrus) and establish version V1.0A of aCCFs (aCCF-V1.0A). ACCF-V1.0A represents an updated formulation of aCCF while exploring the current level of scientific understanding of individual climate effects of aviation emissions by evaluating quantitative estimates of climate effects with the state-of-the-art climate-response model AirClim. Individual scaling factors (i.e. AirClim calibration factors) are provided for the respective non-CO2 effects comprising contrail cirrus, water vapour and NOx-induced climate effects on ozone and methane, resulting uniformly in lower estimates in aCCF-V1.0A for all species compared to the earlier version aCCF-V1.0. [ABSTRACT FROM AUTHOR]

Using climate-optimized flight trajectories is one essential measure to reduce aviation's climate impact. Detailed knowledge of temporal and spatial climate sensitivity for aviation emissions in the atmosphere is required to realize such a climate mitigation measure. The algorithmic Climate Change Functions (aCCFs) represent the basis for such purposes. This paper presents the first version of the Algorithmic Climate Change Function submodel (ACCF 1.0) within the European Centre HAMburg general circulation model (ECHAM) and Modular Earth Submodel System (MESSy) Atmospheric Chemistry (EMAC) model framework. In the ACCF 1.0, we implement a set of aCCFs (version 1.0) to estimate the average temperature response over 20 years (ATR20) resulting from aviation CO 2 emissions and non-CO 2 impacts, such as NO x emissions (via ozone production and methane destruction), water vapour emissions, and contrail cirrus. While the aCCF concept has been introduced in previous research, here, we publish a consistent set of aCCF formulas in terms of fuel scenario, metric, and efficacy for the first time. In particular, this paper elaborates on contrail aCCF development, which has not been published before. ACCF 1.0 uses the simulated atmospheric conditions at the emission location as input to calculate the ATR20 per unit of fuel burned, per NO x emitted, or per flown kilometre. In this research, we perform quality checks of the ACCF 1.0 outputs in two aspects. Firstly, we compare climatological values calculated by ACCF 1.0 to previous studies. The comparison confirms that in the Northern Hemisphere between 150–300 hPa altitude (flight corridor), the vertical and latitudinal structure of NO x -induced ozone and H 2 O effects are well represented by the ACCF model output. The NO x -induced methane effects increase towards lower altitudes and higher latitudes, which behaves differently from the existing literature. For contrail cirrus, the climatological pattern of the ACCF model output corresponds with the literature, except that contrail-cirrus aCCF generates values at low altitudes near polar regions, which is caused by the conditions set up for contrail formation. Secondly, we evaluate the reduction of NO x -induced ozone effects through trajectory optimization, employing the tagging chemistry approach (contribution approach to tag species according to their emission categories and to inherit these tags to other species during the subsequent chemical reactions). The simulation results show that climate-optimized trajectories reduce the radiative forcing contribution from aviation NO x -induced ozone compared to cost-optimized trajectories. Finally, we couple the ACCF 1.0 to the air traffic simulation submodel AirTraf version 2.0 and demonstrate the variability of the flight trajectories when the efficacy of individual effects is considered. Based on the 1 d simulation results of a subset of European flights, the total ATR20 of the climate-optimized flights is significantly lower (roughly 50 % less) than that of the cost-optimized flights, with the most considerable contribution from contrail cirrus. The CO 2 contribution observed in this study is low compared with the non-CO 2 effects, which requires further diagnosis. [ABSTRACT FROM AUTHOR]