1. Directly visualizing the momentum-forbidden dark excitons and their dynamics in atomically thin semiconductors
- Author
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Chakradhar Sahoo, Michael K. L. Man, Xiaoqin Li, Bala Murali Krishna Mariserla, Julien Madéo, Tony F. Heinz, Ting Cao, Marshall Campbell, Vivek Pareek, Keshav M. Dani, Arka Karmakar, E Laine Wong, Abdullah Al-Mahboob, and Nicholas S. Chan
- Subjects
Exciton ,Degrees of freedom (physics and chemistry) ,FOS: Physical sciences ,02 engineering and technology ,Electron ,01 natural sciences ,Momentum ,Condensed Matter::Materials Science ,chemistry.chemical_compound ,Mesoscale and Nanoscale Physics (cond-mat.mes-hall) ,0103 physical sciences ,Monolayer ,Coulomb ,Tungsten diselenide ,010306 general physics ,Condensed Matter::Quantum Gases ,Physics ,Condensed Matter - Materials Science ,Multidisciplinary ,Condensed Matter - Mesoscale and Nanoscale Physics ,Condensed matter physics ,Condensed Matter::Other ,business.industry ,Materials Science (cond-mat.mtrl-sci) ,Condensed Matter::Mesoscopic Systems and Quantum Hall Effect ,021001 nanoscience & nanotechnology ,Semiconductor ,chemistry ,0210 nano-technology ,business - Abstract
Resolving the momentum degree of freedom of excitons - electron-hole pairs bound by the Coulomb attraction in a photoexcited semiconductor, has remained a largely elusive goal for decades. In atomically thin semiconductors, such a capability could probe the momentum forbidden dark excitons, which critically impact proposed opto-electronic technologies, but are not directly accessible via optical techniques. Here, we probe the momentum-state of excitons in a WSe2 monolayer by photoemitting their constituent electrons, and resolving them in time, momentum and energy. We obtain a direct visual of the momentum forbidden dark excitons, and study their properties, including their near-degeneracy with bright excitons and their formation pathways in the energy-momentum landscape. These dark excitons dominate the excited state distribution - a surprising finding that highlights their importance in atomically thin semiconductors., Comment: 34 pages
- Published
- 2020
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