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From a review of the available literature, a database of experimental shape factors from measured beta spectra was created in previous work. Classical assumptions applied in beta spectra calculations which avoid the determination of the electron and nuclear wave functions were tested by comparison with each measured spectrum present in the database. From this systematic comparison, it was demonstrated that the typical assumption λ k =1 is inappropriate for all forbidden unique transitions. Moreover, the equally common ξ -approximation was also proved to be incorrect for about half of the listed first forbidden non-unique transitions and for all second non-unique ones. In present work, this study has been performed once again using an improved analytical screening correction. General results from previous study still remain the same. Except for allowed transitions, the mean energies in current nuclear databases are expected to be erroneous. Some selected beta spectra are also given to illustrate these results. [ABSTRACT FROM AUTHOR]

Metallic magnetic calorimeters have been used for several years for the determination of the shapes of beta spectra. Experimental spectra of the beta decays of $$^{63}$$ Ni and $$^{241}$$ Pu exhibit, at very low energy, strong deviations from standard theoretical calculations including corrections for screening, radiative, and nuclear size effects. These discrepancies can be attributed to the atomic exchange effect. In particular the spectrum of $$^{63}$$ Ni measured with an electroplated $$^{63}$$ Ni source is in excellent agreement with theory including the exchange effect. This underlines the quality of the experimental spectrum as well as the correctness of the calculation of the exchange effect. [ABSTRACT FROM AUTHOR]

Nuclear decay data measurements were performed in the frame of a EURAMET project. Two specific goals were addressed: (1) High-precision measurements of ^238U alpha-particle emission probabilities and (2) experimental characterization of the shape of beta spectra using cryogenic detectors. In the paper, specific lessons learned from the metrological work are highlighted. This includes effects of source preparation on the quality of alpha and beta spectrometry, the influence of exchange effects on beta spectra and the use of a magnet system to eliminate coincidence effects by conversion electrons in alpha-particle spectra. [ABSTRACT FROM PUBLISHER]

Abstract: Metallic magnetic calorimeters are a specific type of cryogenic detectors that have been shown to enable precise measurement of the shape of low energy beta spectra. The aim of their use at LNHB is the determination of the shape factors of beta spectra. The beta source is enclosed in the detector absorber, allowing for very high detection efficiency. It has turned out that the type of source is of crucial importance for the correctness of the measured spectrum. Spectra of 63Ni measured with several sources prepared by drying a NiCl2 solution differ from one another and from theory, whereas spectra measured with electroplated sources are reproducible and agree with theory. With these latter measurements we could confirm the atomic exchange effect down to very low energy (200eV). [Copyright &y& Elsevier]

Abstract: The LNE-LNHB is developing metallic magnetic calorimeters, a specific type of cryogenic detectors, for beta spectrometry. The aim is the determination of the shape factors of beta spectra. Our latest detector has been designed to measure the spectrum of 241Pu, a pure beta emitter with an endpoint energy of 20.8keV. In this paper, the detection principle of metallic magnetic calorimeters is explained and a detailed description is given of the realization of the detector enclosing a 241Pu source inside the detector absorber. A spectrum resulting from our first measurement is shown and compared with a theoretical spectrum. [Copyright &y& Elsevier]