1. Coatable Li4SnS4 Solid Electrolytes Prepared from Aqueous Solutions for All-Solid-State Lithium-Ion Batteries.
- Author
-
Choi, Young Eun, Park, Kern Ho, Kim, Dong Hyeon, Oh, Dae Yang, Kwak, Hi Ram, Lee, Young‐Gi, and Jung, Yoon Seok
- Subjects
LITHIUM-ion batteries ,AQUEOUS solutions ,ELECTROLYTES ,ENERGY storage ,ELECTRIC batteries - Abstract
Bulk-type all-solid-state lithium-ion batteries (ASLBs) for large-scale energy-storage applications have emerged as a promising alternative to conventional lithium-ion batteries (LIBs) owing to their superior safety. However, the electrochemical performance of bulk-type ASLBs is critically limited by the low ionic conductivity of solid electrolytes (SEs) and poor ionic contact between the active materials and SEs. Herein, highly conductive (0.14 mS cm
−1 ) and dry-air-stable SEs (Li4 SnS4 ) are reported, which are prepared using a scalable aqueous-solution process. An active material (LiCoO2 ) coated by solidified Li4 SnS4 from aqueous solutions results in a significant improvement in the electrochemical performance of ASLBs. Side-effects of the exposure of LiCoO2 to aqueous solutions are minimized by using predissolved Li4 SnS4 solution. [ABSTRACT FROM AUTHOR]- Published
- 2017
- Full Text
- View/download PDF