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The 30 at.% Ho: BaY2F8 crystals were grown by the Czochralski method, and their spectroscopic properties are analyzed systematically by standard Judd–Ofelt theory. The Judd–Ofelt intensity parameters are estimated to be Ω2 = 6.74 × 10−20 cm2, Ω4 = 1.20 × 10−20 cm2, and Ω6 = 0.66 × 10−20 cm2, and the fluorescence branching ratios and radiative lifetimes for a series of excited state manifolds are also determined. The emission cross sections with our measured infrared luminescence spectra, especially important for 4.1 μm, are calculated to be about 4.37 × 10−21 cm2. The crystal quality is preliminarily tested through a mid-infrared laser emission experiment. [ABSTRACT FROM AUTHOR]