1. Simple control of carbon mass loading in capacitive deionization for efficient deionized water production.
- Author
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Shi, Mingxing, Ji, Guangwei, Cui, Xiangjing, Liu, Chun, Hong, Xianyong, Ding, Zhoutian, Qiang, Hua, Wang, Fengyun, and Xia, Mingzhu
- Subjects
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DEIONIZATION of water , *CARBON-black , *CARBON , *ADSORPTION capacity - Abstract
[Display omitted] • The universal low carbon mass loading was used in capacitive deionization (CDI) for efficient deionized (DI) water production. • Partial desalination performance weakened with increasing carbon mass loading. • CDI cells using YEC-8–5.81 as electrodes produced DI water with a low conductivity of 1.89 μS/cm. • Carbons with a suitable micro- meso pore distribution and high specific capacitance may be a better choice. • 82.2% DI water recovery was achieved under stopped flow (SF) discharge mode. High-purity deionized (DI) water can be widely used in high-end manufacturing fields, but its efficient and energy-saving production is a huge challenge. Here, simple carbon mass loading control was developed for efficient DI water production via advanced capacitive deionization (CDI). Supercapacitor carbon (YEC-8) electrodes with diverse mass loading of 2.50, 5.81, 12.63 and 24.72 mg/cm2 were prepared for desalination. As expected, YEC-8–2.50 acquired the optimal CDI performance. High mass loading of 12.63 and 24.72 mg/cm2 not only caused an overt property drop but also serious wasted materials. Competitively, YEC-8–5.81 achieved a similar volumetric adsorption capacity (VAC) to YEC-8–2.50 as well as made up for the lack of total mass of YEC-8–2.50 and the resultant solution conductivity was as low as 1.89 μS/cm (grade III DI water). This strategy has been successfully extended to other carbon materials and carbons with suitable micro- meso pore distribution and high specific capacitance may be a better choice. Besides, the reverse effect of acetylene black (AB) mass on desalination was verified. To gain a high water recovery (W R), stopped flow (SF) discharge was introduced and realized a high W R of 82.2 %. Meanwhile, cycling tests indicated its splendid cycling stability. This study provides a universal direction for using low mass loading strategy for efficient DI water production. [ABSTRACT FROM AUTHOR]
- Published
- 2022
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