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We generalize the family of approximate momentum average methods to formulate a numerically exact, convergent hierarchy of equations whose solution provides an efficient algorithm to compute the Green's function of a particle dressed by bosons suitable in the entire parameter regime. We use this approach to extract ground-state properties and spectral functions. Our approximation-free framework, dubbed the generalized Green's function cluster expansion (GGCE), allows access to exact numerical results in the extreme adiabatic limit, where many standard methods struggle or completely fail. We showcase the performance of the method, specializing three important models of charge-boson coupling in solids and molecular complexes: the molecular Holstein model, which describes coupling between charge density and local distortions, the Peierls model, which describes modulation of charge hopping due to intersite distortions, and a more complex Holstein+Peierls system with couplings to two different phonon modes, paradigmatic of charge-lattice interactions in organic crystals. The GGCE serves as an efficient approach that can be systematically extended to different physical scenarios, thus providing a tool to model the frequency dependence of dressed particles in realistic settings., 13 pages, 6 figures main text + 1 figure appendices

Recent theoretical research on tensor gauge theories led to the discovery of an exotic type of quasiparticles, dubbed fractons, that obey both charge and dipole conservation. Here we describe physical implementation of dipole conservation laws in realistic systems. We show that fractons find a natural realization in hole-doped antiferromagnets. There, individual holes are largely immobile, while dipolar hole pairs move with ease. First, we demonstrate a broad parametric regime of fracton behavior in hole-doped two-dimensional Ising antiferromagnets viable through five orders in perturbation theory. We then specialize to the case of holes confined to one dimension in an otherwise two-dimensional antiferromagnetic background, which can be realized via the application of external fields in experiments, and prove ideal fracton behavior. We explicitly map the model onto a fracton Hamiltonian featuring conservation of dipole moment. Manifestations of fractonicity in these systems include gravitational clustering of holes. We also discuss diagnostics of fracton behavior, which we argue is borne out in existing experimental results., 5 pages main text + 1 page supplementary information, 2 figures main text

We use the Density Matrix Renormalization Group method to study a one-dimensional chain with Peierls electron-phonon coupling, which describes the modulation of the electron hopping by lattice distortions. We demonstrate that this system is stable against phase separation in the dilute density limit. We only find phase separation numerically for large couplings for which the linear approximation for the electron-phonon coupling becomes invalid; this behavior can be stabilized in a narrow sliver of the physical parameter space if the dispersion of the phonons is carefully tuned. These results indicate that in the dilute electron density limit, Peierls bipolaron liquids are generically stable, unlike in other models of electron-phonon coupling. We show that this behavior extends to finite carrier concentrations of up to quarter filling. This stability of low-density, light-mass bipolaron liquids in the Peierls model opens a path to high-$T_c$ superconductivity based on a bipolaronic mechanism, in higher dimensions., 4 pages main text + 5 pages supplementary materials, 4 figures main text + 6 figures supplementary materials

We investigate the formation of trimers in an infinite one-dimensional lattice model of hard-core particles with single-particle hopping $t$ and and nearest-neighbour two-body $U$ and three-body $V$ interactions of relevance to Rydberg atoms and polar molecules. For sufficiently attractive $U\leq-2t$ and positive $V>0$ a large trimer is stabilized, which persists as $V\rightarrow \infty$, while both attractive $U\leq0$ and $V\leq0$ bind a small trimer. The excited state above this small trimer is also bound and has a large extent; its behavior as $V\rightarrow -\infty$ resembles that of the large ground-state trimer. These large bound states appear to admit a continuum description. Furthermore, we find that in the limit $V>>t$, $U, Comment: 6 pages, 7 figures

Penning ionization releases electrons in a state-selected Rydberg gas of nitric oxide entrained in a supersonic molecular beam. Subsequent processes of electron impact avalanche, bifurcation, and quench form a strongly coupled, spatially correlated, ultracold plasma of ${\mathrm{NO}}^{+}$ ions and electrons that exhibits characteristics of self-organized criticality. This plasma contains a residue of nitric oxide Rydberg molecules. A conventional fluid dynamics of ion-electron-Rydberg quasi-equilibrium predicts rapid decay to neutral atoms. Instead, the NO plasma endures for a millisecond or more, suggesting that quenched disorder creates a state of suppressed electron mobility. Supporting this proposition, a 60-MHz radio frequency field with a peak-to-peak amplitude less than 1 V ${\mathrm{cm}}^{\ensuremath{-}1}$ acts dramatically to mobilize electrons, causing the plasma to dissipate by dissociative recombination and Rydberg predissociation. An evident density dependence shows that this effect relies on collisions, giving weight to the idea of arrested relaxation as a cooperative property of the ensemble.

Fractons are a type of emergent quasiparticle which cannot move freely in isolation, but can easily move in bound pairs. Similar phenomenology is found in boson-affected hopping models, encountered in the study of polaron systems and hole-doped Ising antiferromagnets, in which motion of a particle requires the creation or absorption of bosonic excitations. We show that boson-affected hopping models can provide a natural realization of fractons, either approximately or exactly, depending on the details of the system. We first consider a generic one-dimensional boson-affected hopping model, in which we show that single particles move only at sixth order in perturbation theory, while motion of bound states occurs at second order, allowing for a broad parameter regime exhibiting approximate fracton phenomenology. We explicitly map the model onto a fracton Hamiltonian featuring conservation of dipole moment via integrating out the mediating bosons. We then consider a special type of boson-affected hopping models with mutual hard-core repulsion between particles and bosons, accessible in hole-doped mixed-dimensional Ising antiferromagnets, in which the hole motion is one dimensional in an otherwise two-dimensional antiferromagnetic background. We show that this system, which is within the current reach of ultracold-atom experiments, exhibits perfect fracton behavior to all orders in perturbation theory, thereby enabling the experimental study of dipole-conserving field theories. We further discuss diagnostic signatures of fractonic behavior in these systems. In studying these models, we also identify simple effective one-dimensional microscopic Hamiltonians featuring perfect fractonic behavior, paving the way to future studies on fracton physics in lower dimensions., Comment: 15 pages main text + 3 pages appendices, 6 figures main text + 1 figure appendices

We consider the quench of an atomic impurity via a single Rydberg excitation in a degenerate Fermi gas. The Rydberg interaction with the background gas particles induces an ultralong-range potential that binds particles to form dimers, trimers, tetramers, etc. Such oligomeric molecules were recently observed in atomic Bose-Einstein condensates. In this work, we demonstrate with a functional determinant approach that quantum statistics and fluctuations have observable spectral consequences. We show that the occupation of molecular states is predicated on the Fermi statistics, which suppresses molecular formation in an emergent molecular shell structure. At large gas densities this leads to spectral narrowing, which can serve as a probe of the quantum gas thermodynamic properties., Comment: 10 pages main text + 3 pages appendices, 7 figures main text

It is widely accepted that phonon-mediated high-temperature superconductivity is impossible at ambient pressure, because of the very large effective masses of polarons/bipolarons at strong electron-phonon coupling. Here we challenge this belief by showing that strongly bound yet very light bipolarons appear for strong Peierls/Su-Schrieffer-Heeger interaction. These bipolarons also exhibit many other unconventional properties, e.g. at strong coupling there are two low-energy bipolaron bands that are stable against strong on-site Hubbard repulsion. Using numerical simulations and analytical arguments, we show that these properties result from the specific form of the phonon-mediated interaction, which is of "pair-hopping" instead of regular density-density type. This unusual effective interaction is bound to have non-trivial consequences for the superconducting state expected to arise at finite carrier concentrations, and should favor a large critical temperature., Comment: 6 pages, 5 figures

When dressed particles (polarons) exchange quantum phonons, the resulting interactions are generally attractive. If the particles have hard-core statistics and the coupling to phonons is through the kinetic energy terms, phonon-mediated interactions are repulsive. Here, we show that such repulsive phonon-mediated interactions bind dressed particles into bipolarons with unique properties. These bipolaron states appear in the gap between phonon excitations, above the two-polaron continuum. While thermodynamically unstable, the bipolaron is protected by energy and momentum conservation and represents a novel quasiparticle with a large dispersion and a negative effective mass near zero momentum. We discuss possible experimental implementation of the conditions for the formation of such repulsively bound bipolarons., Comment: 7 pages, 4 figures, 2 appendices

We argue that the quenched ultracold plasma presents an experimental platform for studying quantum many-body physics of disordered systems in the long-time and finite energy-density limits. We consider an experiment that quenches a plasma of nitric oxide to an ultracold system of Rydberg molecules, ions and electrons that exhibits a long-lived state of arrested relaxation. The qualitative features of this state fail to conform with classical models. Here, we develop a microscopic quantum description for the arrested phase based on an effective many-body spin Hamiltonian that includes both dipole-dipole and van der Waals interactions. This effective model appears to offer a way to envision the essential quantum disordered non-equilibrium physics of this system., 6 pages main text + 9 pages supplemental materials, 2 figures main text + 7 figures and 2 tables supplemental materials

We study two identical fermions, or two hard-core bosons, in an infinite chain and coupled to phonons by interactions that modulate their hopping as described by the Peierls/Su-Schrieffer-Heeger (SSH) model. We show that exchange of phonons generates effective nearest-neighbor repulsion between particles and also gives rise to interactions that move the pair as a whole. The two-polaron phase diagram exhibits two sharp transitions, leading to light dimers at strong coupling and the flattening of the dimer dispersion at some critical values of the parameters. This dimer (quasi)self-trapping occurs at coupling strengths where single polarons are mobile. This illustrates that, depending on the strength of the phonon-mediated interactions, the coupling to phonons may completely suppress or strongly enhance quantum transport of correlated particles., 6 pages main text + 8 pages supplementary material, 3 figures main text + 1 figure supplementary material

Spontaneous avalanche to plasma splits the core of an ellipsoidal Rydberg gas of nitric oxide. Ambipolar expansion first quenches the electron temperature of this core plasma. Then, long-range, resonant charge transfer from ballistic ions to frozen Rydberg molecules in the wings of the ellipsoid quenches the centre-of-mass ion/Rydberg molecule velocity distribution. This sequence of steps gives rise to a remarkable mechanics of self-assembly, in which the kinetic energy of initially formed hot electrons and ions drives an observed separation of plasma volumes. These dynamics adiabatically sequester energy in a reservoir of mass transport, starting a process that anneals separating volumes to form an apparent glass of strongly coupled ions and electrons. Short-time electron spectroscopy provides experimental evidence for complete ionization. The long lifetime of this system, particularly its stability with respect to recombination and neutral dissociation, suggests that this transformation affords a robust state of arrested relaxation, far from thermal equilibrium.

The exploration of large-scale many-body phenomena in quantum materials has produced many important experimental discoveries, including novel states of entanglement, topology and quantum order as found for example in quantum spin ices, topological insulators and semimetals, complex magnets, and high-$T_c$ superconductors. Yet, the sheer scale of solid-state systems and the difficulty of exercising exacting control of their quantum mechanical degrees of freedom limit the pace of rational progress in advancing the properties of these and other materials. With extraordinary effort to counteract natural processes of dissipation, precisely engineered ultracold quantum simulators could point the way to exotic new materials. Here, we look instead to the quantum mechanical character of the arrested state formed by a quenched ultracold molecular plasma. This novel class of system arises spontaneously, without a deliberate engineering of interactions, and evolves naturally from state-specified initial conditions, to a long-lived final state of canonical density, in a process that conflicts with classical notions of plasma dissipation and neutral dissociation. We take information from experimental observations to develop a conceptual argument that attempts to explain this state of arrested relaxation in terms of a minimal phenomenological model of randomly interacting dipoles of random energies. This model of the plasma forms a starting point to describe its observed absence of relaxation in terms of many-body localization (MBL). The large number of accessible Rydberg and excitonic states gives rise to an unconventional web of many-body interactions that vastly exceeds the complexity of MBL in a conventional few-level scheme. This experimental platform thus opens an avenue for the coupling of dipoles in disordered environments that will demand the development of new theoretical tools., Comment: 27 pages, 6 figures, 2 tables