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When thin films are patterned to realize nanoscale device geometries, maintaining their structural integrity is key to the quality of their functional properties. The introduction of new surfaces and interfaces by lateral modifications may alter material properties as well as the expected device functionality. In this study, two different techniques for nanoscale patterning of epitaxial thin films of La0.7Sr0.3MnO3 are used to investigate the effects on their ferromagnetic properties and film crystalline structure. Nanomagnets are realized as free- standing structures and embedded ferromagnets in a paramagnetic matrix, respectively. We find that the magnetic dichroism signal in x-ray spectomicroscopy is stronger along the edges of the embedded magnets close to TC. X-ray-diffraction measurements reveal a reduction of their in-plane lattice parameters. We discuss how in- plane stress from the nanomagnet surroundings can affect the magnetic properties in these structures. © 2020 The Author(s). Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).

Long-range magnetic ordering can be stabilized in arrays of single-domain nanomagnets through dipolar interactions. In these metamaterials, the magnetic properties are determined by geometric parameters such as the nanomagnet shape and lattice symmetry. Here, we demonstrate engineering of the anisotropy in a dipolar magnetic metamaterial by tuning of the lattice parameters. Furthermore, we show how a modified Kittel's law explains the resulting domain configurations of the dipolar ferromagnetic arrays.

Two-dimensional lattices of dipolar-coupled thin film ferromagnetic nanodisks give rise to emergent superferromagnetic (SFM) order when the spacing between dots becomes sufficiently small. In this paper, we define micron-sized arrays of permalloy nanodisks arranged on a hexagonal lattice. The arrays were shaped as hexagons, squares, and rectangles to investigate finite-size effects in the SFM domain structure for such arrays. The resulting domain patterns were examined using x-ray magnetic circular dichroism photoemission electron microscopy. At room temperature, we find these SFM metamaterials to be below their blocking temperature. Distinct differences were found in the magnetic switching characteristics of horizontally and vertically oriented rectangular arrays. The results are corroborated by micromagnetic simulations.

We have studied the impact of lattice geometry on the dynamic properties of close-spaced arrays of circular nanomagnets, also known as magnonic crystals. To this end, we prepared 2D nanomagnet arrays with both square and hexagonal lattice symmetries (300-nm disk diameter, 400-nm center-to-center distance) and performed broadband ferromagnetic resonance (FMR) measurements. Micromagnetic simulations were used to interpret distinct features of the measured resonance spectra. The FMR bias field was applied along two distinct principal directions for each lattice, and a sample with well-separated, decoupled disks was measured for reference. We found that the interdisk dipolar coupling has a strong impact on the FMR for these 2D magnonic crystals. Distinctly different oscillation modes were found for the individual nanomagnets, dependent on lattice symmetry and direction of the bias field. Moreover, we find that spectral peak splitting from excitation of edge and center modes, as well as the damping, depends on the lattice symmetry and the orientation of the bias field. These findings demonstrate that lattice geometry has a strong influence on the excited spin-wave spectrum and is a relevant design parameter for spintronic devices. © American Physical Society 2019. This is the authors accepted and refereed manuscript to the article.

A field-driven transformation of a domain pattern in a square micromagnet, defined in a thin film of La0.7Sr0.3MnO3, is discussed in terms of creation and annihilation of bulk vortices and edge-bound topological defects with half-integer winding numbers. The evolution of the domain pattern was mapped with soft x-ray photoemission electron microscopy and magnetic force microscopy. Micromagnetic modeling, permitting detailed analysis of the spin texture, accurately reproduces the measured domain state transformation. The simulations also helped stipulate the energy barriers associated with the creation and annihilation of the topological charges and thus to assess the stability of the domain states in this magnetic microstructure. (C) 2018 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license.