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6 pages; International audience; Isomeric states in 253No have been investigated by conversion-electron and gamma-ray spectroscopy with the GABRIELA detection system. The 31 micro second isomer reported more than 30 years ago is found to decay to the ground state of 253No by the emission of a 167 keV M2 transition. The spin and parity of this low-lying isomeric state are established to be 5/2+. The presence of another longer-lived isomeric state is also discussed.

We re-examine the well-known Wong formula for heavy-ion fusion cross sections. Although this celebrated formula yields almost-exact results for single-channel calculations for relatively heavy systems such as $^{16}\mathrm{O}+^{144}\mathrm{Sm}$, it tends to overestimate the cross section for light systems such as $^{12}\mathrm{C}+^{12}\mathrm{C}$. We generalize the formula to take account of the energy dependence of the barrier parameters and show that the energy-dependent version gives results practically indistinguishable from a full quantal calculation. We then examine the deviations arising from the discrete nature of the intervening angular momenta, whose effect can lead to an oscillatory contribution to the excitation function. We recall some compact, analytic expressions for these oscillations and highlight the important physical parameters that give rise to them. Oscillations in symmetric systems are discussed, as are systems where the target and projectile identities can be exchanged via a strong transfer channel.

Background: The nuclear structure of colliding nuclei is known to influence the fusion process. Couplings of the relative motion to nuclear shape deformations and vibrations lead to an enhancement of the sub-barrier fusion cross section in comparison with the predictions of one-dimensional barrier penetration models. This enhancement is explained by coupled-channels calculations including these couplings. The sub-barrier fusion cross section is also affected by nucleon transfer channels between the colliding nuclei.Purpose: The aim of the present experiment is to investigate the influence of the projectile and target nuclear structures on the fusion cross sections in the $^{40}\mathrm{Ca}+^{58}\mathrm{Ni}$ and $^{40}\mathrm{Ca}+^{64}\mathrm{Ni}$ systems.Methods: The experimental and theoretical fusion excitation functions as well as the barrier distributions were compared for these two systems. Coupled-channels calculations were performed using the ccfull code.Results: Good agreement was found between the measured and calculated fusion cross sections for the $^{40}\mathrm{Ca}+^{58}\mathrm{Ni}$ system. The situation is different for the $^{40}\mathrm{Ca}+^{64}\mathrm{Ni}$ system where the coupled-channels calculations with no nucleon transfer clearly underestimate the fusion cross sections below the Coulomb barrier. The fusion excitation function was, however, well reproduced at low and high energies by including the coupling to the neutron pair-transfer channel in the calculations.Conclusions: The nuclear structure of the colliding nuclei influences the fusion cross sections below the Coulomb barrier for both $^{40}\mathrm{Ca}+^{58,64}\mathrm{Ni}$ systems. Moreover, we highlighted the effect of the neutron pair-transfer channel on the fusion cross sections in $^{40}\mathrm{Ca}+^{64}\mathrm{Ni}$.

Precise fusion and quasi-elastic scattering excitation functions have been measured for the systems 40 Ca + 90,96 Zr at energies spanning the Coulomb barrier. From both the fusion and the quasi-elastic scattering data representations of the barrier distributions have been extracted. The barrier distributions of the two reactions are qualitatively very different. While the lighter system is well described by coupled-channels calculations including multi-phonon excitations, this coupling scheme fails completely for the heavier system, possibly due to multi-neutron transfer.

The rotational structure of ${}^{246}$Fm has been investigated using in-beam $\ensuremath{\gamma}$-ray spectroscopic techniques. The experiment was performed using the JUROGAMII germanium detector array coupled to the gas-filled recoil ion transport unit (RITU) and the gamma recoil electron alpha tagging (GREAT) focal plane detection system. Nuclei of ${}^{246}$Fm were produced using a 186 MeV beam of ${}^{40}$Ar impinging on a ${}^{208}$Pb target. The JUROGAMII array was fully instrumented with Tracking Numerical Treatment 2 Dubna (TNT2D) digital acquisition cards. The use of digital electronics and a rotating target allowed for unprecedented beam intensities of up to 71 particle-nanoamperes for prompt $\ensuremath{\gamma}$-ray spectroscopy at a level of approximately 11 nb. With all these major experimental advances a rotational band is observed in ${}^{246}$Fm.

International audience; The perceptive analysis of Rutherford, celebrated at this conference, turned the experiments of Geiger and Marsden into a measurement of the radius of the object that became known as the atomic "nucleus". We now know that the nucleus can have a range of radii that depend on its static and dynamical deformations. These deformations give rise to the distributions of reaction barriers that have been extensively studied over recent years. While fusion reactions are most often used for such studies, there are cases where, for physical or practical reasons, the scattering channels must be exploited. Despite the major advantages gained from modern experimental techniques, the resulting experiments are in spirit essentially the same as those performed over 100 years ago by Rutherford and his colleagues.

International audience; In the context of the creation of heavy evaporation residues, the interplay between capture, quasifission and true compound-nucleus fission is discussed. An approximate factorisation of the cross section into a compound nucleus term and an entrance-channel term is derived, with each of these terms being clearly defined.

Using the random matrix model, we discuss the effect of couplings to non-collective states on the penetrability of a one dimensional potential barrier. We show that these non-collective excitations hinder the penetrability and thus smear the barrier distribution at energies above the barrier, while they do not affect significantly the penetrability at deep subbarrier energies. The energy dependence of the Q-value distribution obtained with this model is also discussed., 4 pages, 2 figures. A talk given at the 10th international conference on nucleus-nucleus collisions (NN2009), Aug. 16-21, 2009, Beijing, China

An isomeric state in {sup 255}Lr with a half-life of t{sub 1/2} = 1.4(1) ms and E{sub x}>720-keV has been observed for the first time using the GABRIELA setup at the focal plane of the VASSILISSA separator. Based on its K-forbiddeness, the configuration of the state is most probably formed by coupling the valence proton to a two quasiparticle neutron excitation. Possible three quasiparticle configurations are discussed.

The 'experimental barrier distribution' provides a parameter-free representation of experimental heavy-ion capture cross sections that highlights the effects of entrance-channel couplings. Its relation to the s-wave transmission is discussed, and in particular it is shown how the full capture cross section can be generated from an l=0 coupled-channels calculation. Furthermore, it is shown how this transmission can be simply exploited in calculations of quasifission and evaporation-residue cross sections. The system {sup 48}Ca+{sup 154}Sm is studied in detail. A calculation of the compound-nucleus spin distribution reveals a possible energy dependence of barrier weights due to polarization arising from target and projectile quadrupole phonon states; this effect also gives rise to an entrance-channel 'extra-push'.

Near-barrier fusion excitation functions for the $^{14}\mathrm{C}$ and $^{18}\mathrm{O}+^{208}\mathrm{Pb}$ reactions have been analyzed in the framework of the barrier-passing model using different forms of the nuclear potential and the phenomenology of a fluctuating barrier. The best-fit fusion potentials were used to estimate cluster decay probabilities from the corresponding ground states of Ra and Th (i.e., for the inverse decay process). The analysis supports the ``\ensuremath{\alpha}-decay-like'' scenario for carbon and oxygen emission from these nuclei.

A precise fusion excitation function has been measured for 40 Ca+ 94 Zr at near- and sub-barrier energies, and the fusion barrier distribution has been extracted. Comparing with the existing data for 40,48 Ca+ 90,96 Zr shows that couplings to inelastic excitations determine the fusion cross sections and the shape of the barrier distributions near the barrier. At lower energies, the two systems possessing neutron-transfer channels with large positive Q-values ( 40 Ca+ 94,96 Zr) have remarkably similar cross sections, and both show a large enhancement with respect to the other systems and to coupled-channels calculations including up to three quadrupole and octupole phonons in the Zr targets.

Mass-energy and angular distributions of fission fragments for the $^{48}\mathrm{Ca}+^{144,154}\mathrm{Sm}\ensuremath{\rightarrow}^{192,202}\mathrm{Pb}$, $^{40}\mathrm{Ca}+^{154}\mathrm{Sm}\ensuremath{\rightarrow}^{194}\mathrm{Pb}$ reactions have been measured. Fusion suppression and the presence of quasifission at energies near and below the Coulomb barrier have been observed for the reactions with the deformed target $^{154}\mathrm{Sm}$. In the case of the spherical $^{144}\mathrm{Sm}$ target no evidence of quasifission has been found. Quasifission cross sections have been extracted from total fission-like events by analysis of their mass and angular distributions.

Large-angle quasielastic scattering has been studied in a high- Z 1 Z 2 nuclear reaction of the type leading to superheavy-element production by cold fusion. We show that despite the presence of strongly dissipative channels, and the complete absence of fusion, the notion of an external barrier distribution, determined by strong coupling to collective excitations of target and projectile, is still valid. Furthermore, our method allows us to deduce some properties of the deep-inelastic processes in this system.

In view of its large deformation, which should give rise to strong barrier structures, the 20 Ne projectile has been used to study the influence of neutron-transfer channels on the distribution of barrier heights. A previous experiment with a combination of projectiles 20,22 Ne suggested that the role of α-particle transfer channels is small. By an appropriate choice of targets (90 Zr and 92 Zr ), having very similar intrinsic structures (excited states and deformation parameters) but giving rise to different Q-values for neutron transfers, we highlight the role of these channels.

Excited states in {sup 249}Fm were populated via the {alpha} decay of {sup 253}No and the subsequent decay was observed with the GABRIELA detection system installed at the focal plane of the VASSILISSA recoil separator. The energies, spins, and parities of these states could be established through combined {alpha},{gamma}, and conversion-electron spectroscopy. The first members of the ground-state rotational band were identified. Their excitation energies as well as the observation of a cross-over E2 transition confirm the assignment of 7/2{sup +}624 for the ground state of {sup 249}Fm. Two excited states were also observed and their decay properties suggest that they correspond to the particle excitation 9/2{sup -}734 and hole excitation 5/2{sup +}622. The analysis suggests that the 279-keV transition de-exciting the 9/2{sup -} state has anomalous E1 conversion coefficients.

A new experiment to determine the thermonuclear cross section of the C-12(alpha,gamma)O-16 reaction has been performed in regular kinematics using an intense alpha-particle beam of up to 340 mu A from the Stuttgart DYNAMITRON. For the first time, a 4 pi-germanium-detector setup has been used to measure the angular distribution of the gamma rays at all angles simultaneously. It consisted of an array of nine EUROGAM high-purity Ge detectors in close geometry, actively shielded individually with bismuth germanate crystals. The C-12 targets were isotopically enriched by magnetic separation during implantation. The depth profiles of the implanted carbon in the C-12 targets were determined by Rutherford backscattering for purposes of cross-section normalization and absolute determination of the E1 and E2 S factors. Angular distributions of the gamma decay to the O-16 ground state were measured in the energy range E-c.m.=1.30-2.78 MeV and in the angular range (lab.) 30 degrees-130 degrees. From these distributions, astrophysical E1 and E2 S-factor functions vs energy were calculated, both of which are indispensable to the modeling of this reaction and the extrapolation toward lower energies. The separation of the E1 and E2 capture channels was done both by taking the phase value phi(12) as a free parameter and by fixing it using the results of elastic alpha-particle scattering on C-12 in the same energy range.

Fusion-evaporation cross sections were measured in the two systems {sup 48}Ca+{sup 90,96}Zr in an energy range from well below to well above the Coulomb barrier. The sub-barrier fusion of {sup 48}Ca+{sup 90}Zr is reproduced by coupled-channels calculations including the lowest quadrupole and octupole vibrations of {sup 90}Zr, and using a Woods-Saxon potential with a standard diffuseness parameter a = 0.68 fm. However, the fusion cross sections are overestimated above the barrier. The low-energy slope of the excitation function for {sup 48}Ca+{sup 96}Zr is steeper. This implies a larger diffuseness parameter a = 0.85 fm. Fusion cross sections are well fit in the whole energy range, and the effect of the strong octupole vibration in {sup 96}Zr is predominant. The extracted fusion barrier distributions are reasonably well reproduced by calculations for both systems. A comparison with previous data for {sup 40}Ca+{sup 90,96}Zr is made in an attempt to clarify the role of transfer couplings in sub-barrier fusion.

With the aid of the Geant4 Monte Carlo simulation package a new detection system has been designed for the focal plane of the recoil separator VASSILISSA situated at the Flerov Laboratory of Nuclear Reactions, JINR, Dubna. GABRIELA (Gamma Alpha Beta Recoil Investigations with the Electromagnetic Analyser VASSILISSA) has been optimised to detect the arrival of reaction products and their subsequent radioactive decays involving the emission of alpha- and beta-particles, fission fragments, gamma- and X-rays, and conversion electrons. The new detector system is described and the results of the first commissioning experiments are presented., 24 pages, Submitted to NIM A

The interest in the study of the fission process of superheavy nuclei mainly deals with the opportunity to obtain information about the cross-section of the compound nucleus (CN) formation at excitation energies E*\approx 15–30 MeV. It allows one to estimate the survival probability of the superheavy composite system after evaporation of 1–3 neutrons, i.e. in "cold" or "warm" fusion reactions. However, in order to solve this problem deeper understanding of the coalescence processes between colliding nuclei, the competition between fusion-fission and quasi-fission processes is needed. The characteristics of both processes, their manifestation in the experimental observables and the relative contribution to the capture cross-section in dependence on the excitation energies, reaction entrance channel etc were investigated for a wide range of target-projectile combinations. Results of the experiments devoted to the study of the fusion-fission and quasi-fission processes in the reactions of the formation of the superheavy nuclei with Z = 102–122 are presented. The heavy ions 26Mg, 48Ca, 50Ti, 58Fe and 64Ni were used as projectiles. The choice of the reactions with 48Ca and actinide-targets was inspired by the experiments on the production of the isotopes 283112, 289114 and 283116 in Dubna using the same reactions. The 50Ti, 58Fe and 64Ni projectiles were chosen since the corresponding projectile-target combinations lead to the synthesis of even heavier elements. The experiments were carried out at the U-400 accelerator of the Flerov Laboratory of Nuclear Reactions (JINR, Russia) and the XTU Tandem accelerator of the National Laboratory of Legnaro (LNL, Italy) using the time-of-flight spectrometer of fission fragments CORSET. The role of the shell effects, the influence of the entrance channel asymmetry and the deformations of colliding nuclei on the mechanism of the fusion-fission and the competitive process of quasi-fission are discussed. The recent results on synthesis of superheavy nuclei and the perspectives of the "hot" fusion reaction for the production of superheavy nuclei are considered.

In intermediate-mass systems, collective excitations of the target and projectile can greatly enhance the subbarrier capture cross section σ cap by giving rise to a distribution of Coulomb barriers. For such systems, capture essentially leads directly to fusion [formation of a compound nucleus (CN)], which then decays through the emission of light particles (neutrons, protons, and alpha particles). Thus, the evaporation-residue (ER) cross section is essentially equal to σ cap. For heavier systems, the experimental situation is significantly more complicated owing to the presence of quasifission (QF) (rapid separation into two fragments before the CN is formed) and by fusion-fission (FF) of the CN itself. Thus, three cross sections need to be measured in order to evaluate σ cap. Although the ER essentially recoil along the beam direction, QF and FF fragments are scattered to all angles and require the measurement of angular distributions in order to obtain the excitation function and barrier distribution for capture. Two other approaches to this problem exist. If QF is not important, one can still measure just the ER cross section and try to reconstruct the corresponding σ cap through use of an evaporation-model code that takes account of the FF degree of freedom. Some earlier results on σ cap obtained in this way will be reanalyzed with detailed coupled-channels calculations, and the “extra-push” phenomenon discussed. One may also try to obtain σ cap by exploiting unitarity, that is, by measuring instead the flux of particles corresponding to quasielastic (QE) scattering from the Coulomb barrier. Some new QE results obtained for the 86Kr + 208Pb system at iThemba LABS in South Africa will be presented.

International audience; A breakthrough was recently obtained in the analysis of the so-called Hyper-Long-HyperDeformed (HLHD) experiment made at the EUROBALL-IV γ-detector array (EB). The 64Ni + 64Ni ⇒ 128Ba* fusion reaction was studied at Ebeam = 255 and 261 MeV, reaching the highest angular momentum that the compound nuclei can accommodate. To date no discrete HD rotational bands have been identified. However, rotational patterns in the form of ridge-structures in three-dimensional (3D) rotational mapped spectra are identified with dynamic moments of inertia J(2) ranging from 71 to 1112 MeV-1 in 12 different nuclei selected by charged particle- and/or γ-gating. The four nuclei, 118Te, 124Cs, 125Cs and 124Xe found with moment of inertia J(2)≥100 2 MeV-1, are most likely hyperdeformed, the remaining nuclei with smaller values of J(2), are considered to be superdeformed, in qualitative agreement with recent theoretical calculations.

Motivated by the extreme deformation parameters of the projectile, we have measured quasi-elastic scattering for 20 Ne + 118 Sn. In contrast to calculations based on known collective states, the experimental barrier distribution is structureless. A comparison with the system 22 Ne + 118 Sn shows that this smoothing is unlikely to be due to nucleon- or α -transfer channels, and is more likely to be due to coupling to many other weak channels.

A recent publication reports that heavy-ion fusion cross sections at extreme subbarrier energies show a continuous change of their logarithmic slope with decreasing energy, resulting in a much steeper excitation function compared with theoretical predictions. We show that the energy dependence of this slope is partly due to the asymmetric shape of the Coulomb barrier, that is its deviation from a harmonic shape. We also point out that the large low-energy slope is consistent with the surprisingly large surface diffusenesses required to fit recent high-precision fusion data., 9 pages, 3 eps figures

We have studied the mass and energy distributions of fission fragments from the two reactions ${}^{12}\mathrm{C}{+}^{204}\mathrm{Pb}$ and ${}^{48}\mathrm{Ca}{+}^{168}\mathrm{Er}$ that lead to the same compound nucleus ${}^{216}{\mathrm{Ra}}^{*}.$ Despite the fact that the excitation energy was around 40 MeV in both cases, the contribution from asymmetric fission in the first reaction is only around 1.5% but is about 30% in the second. This marked increase in the yield of asymmetric products is connected to the quasifission process, in which important shell effects become evident. The mass-energy distributions are interpreted in terms of an independent decay mode competing with the normal fusion-fission process and possibly leading to a significant suppression of the fusion cross section itself.

Near-barrier excitation functions have been measured for evaporation-residue production and fission in the 12C + 204,206,208Pb and 48Ca + 168,170Er systems that lead to the compound nuclei 216,218,220Ra*. A Pronounced suppression of evaporation-residue production is observed for the more symmetric combinations, 48Ca + 168,170Er. We relate this to the significant quasifission components already observed for these systems.

Heavy-ion fusion barrier distributions are now routinely obtained directly from experimental data. Measurements of the total γ-ray multiplicity for the fusion channels of the 58 Ni + 60 Ni system, which has striking yet well understood barrier structures, confirm the theoretical predictions that very high spins can be populated at energies close to (and even below) the nominal Coulomb barrier. The mapping from multiplicities to spin populations shows that structures in the barrier distribution are still evident in the γ-ray results.

The extraction of representations of the fusion barrier distribution from backward-angle, quasi-elastic, elastic and transfer excitation functions is discussed. Such excitation functions have been measured for , and projectiles incident on a variety of targets. The results are compared with representations obtained from fusion excitation functions. Varying in their sensitivity, all representations show evidence of the barrier structure. Differences between the scattering and the fusion representations can be related to the effects of coupling to residual, weak reaction channels.

We study in detail the barrier distributions extracted from large-angle quasi-elastic scattering of heavy ions at energies near the Coulomb barrier. Using a closed-form expression for scattering from a single barrier, we compare the quasi-elastic barrier distribution with the corresponding test function for fusion. We examine the isocentrifugal approximation in coupled-channels calculations of quasi-elastic scattering and find that for backward angles, it works well, justifying the concept of a barrier distribution for scattering processes. This method offers an interesting tool for investigating unstable nuclei. We illustrate this for the $^{32}$Mg + $^{208}$Pb reaction, where the quadrupole collectivity of the neutron-rich $^{32}$Mg remains to be clarified experimentally., Comment: 26 pages, 10 eps figures